1. Institute for Advanced Study, Tsinghua University, Beijing 100084, China
2. Department of Physics, Fudan University, Shanghai 200438, China
PengfeiZhang.physics@gmail.com
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Received
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Published
2023-11-30
2024-03-25
2024-06-15
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Revised Date
2024-05-06
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Abstract
The spectral form factor (SFF) can probe the eigenvalue statistic at different energy scales as its time variable varies. In closed quantum chaotic systems, the SFF exhibits a universal dip-ramp-plateau behavior, which reflects the spectrum rigidity of the Hamiltonian. In this work, we explore the general properties of SFF in open quantum systems. We find that in open systems the SFF first decays exponentially, followed by a linear increase at some intermediate time scale, and finally decreases to a saturated plateau value. We derive general relations between (i) the early-time decay exponent and Lindblad operators; (ii) the long-time plateau value and the number of steady states. We also explain the effective field theory perspective of general behaviors. We verify our theoretical predictions by numerically simulating the Sachdev−Ye−Kitaev (SYK) model, random matrix theory (RMT), and the Bose−Hubbard model.
Yi-Neng Zhou, Tian-Gang Zhou, Pengfei Zhang.
General properties of the spectral form factor in open quantum systems.
Front. Phys., 2024, 19(3): 31202 DOI:10.1007/s11467-024-1406-7
The spectral form factor (SFF) has attracted much attention in recent years for its direct relation to the eigenvalue statistics at different energy scales and its utility as a robust diagnosis of quantum chaos [1-13]. The structure of SFF is a direct indicator of the energy spectrum correlation in quantum systems. As its time variable increases, it reveals the eigenvalue statistics at a smaller energy scale. The SFF among different models reveals the symmetry that those models preserve. It exhibits several universal properties including the initial decay, the increase at intermediate time scales which shows a linear ramp in models with spectrum rigidity, and finally the saturation to a plateau value. This dip-ramp-plateau structure is ubiquitous in quantum chaos systems [14-17].
However, the interaction and exchange between the system and environment are inevitable, and therefore it is natural to focus on the corresponding problem in open systems. Generalizing familiar concepts in closed systems to open systems has helped people discover much more interesting and novel physics. Recently, the development of entropy dynamics [18], entanglement phase transition [19-46], and operator complexity [47-50] in open quantum many-body systems have aroused much interest in condensed matter physicists. Also, there are explorations on the definitions and physical interpretations of the SFF in open systems or non-Hermitian Hamiltonians [51-58].
In this paper, we study the SFF in open quantum systems driven by the Lindblad master equation. The definition we use excludes possible exponential growth over time in general non-Hermitian systems [59]. For concreteness, we define the normalized SFF as the ratio between SFF with dissipation and that without dissipation. We find some general properties of the normalized SFF according to its early-time and late-time dynamics. More specifically, we find this normalized SFF has an early-time exponential decay behavior related to the Lindblad operators and late-time plateau behavior related to the number of steady states. We demonstrate the generality of these properties in open systems by studying three different models with dissipation: the random matrix model, the SYK model, and the Bose−Hubbard model. In the random matrix model and the Bose−Hubbard model, the numerical results agree well with our conjecture. Furthermore, using the path-integral method, we give a candidate semi-classical explanation of the SFF in systems with dissipation, and this is a novel perspective for understanding the general properties of the normalized SFF.
2 The definition of SFF in open systems
In the closed system, the SFF can be defined as the size fluctuation of the analytic continuation of the thermal partition function of the quantum system
with . From this expression, we see that SFF captures the energy level correlations of the full spectrum of the system, and the energy scale that it probes decreases as its time variable increases. At early time, SFF captures the energy level correlations at an energy scale much larger than the mean energy level spacing of the system, and it usually has a decay behavior, often called slope. This slope region is non-universal in different models for it sees the details of the energy spectrum of the system. However, it can be universally bounded, regardless of whether the system is chaotic or not [60]. At the intermediate time scale, SFF measures the energy level correlation in the same order as the mean energy level spacing, and in some models that have level repulsion, we see a linear ramp of SFF as time increases. Therefore, SFF can be used to diagnose spectral rigidity. A detailed study of the SFF in terms of spectral distances helps understand this ramp and the transition to the plateau [17]. Over a long time, the SFF often saturates to a constant plateau value determined by each single energy level. Also, there are some studies about the non-universal properties of the form factor in chaotic systems [61, 62].
In the open system, we consider the time evolution of the system driven by the Lindblad Master equation
Here, is the dissipation strength, and is the Lindblad jump operator. If we use the Choi−Jamiolkwski isomorphism [63, 64] to map the density matrix to a wave function defined on a doubled space as , then after this mapping the wave function in the doubled system satisfies a Schrodinger-like equation . Here, is defined on the doubled space with
Operators with subscripts and stand for operators acting on the left and the right systems respectively, “T” stands for the transpose, and represents the identity operator. Here, both and take the same form as the original Hamiltonian , although they act on different Hilbert spaces.
Similar to the SFF defined in the closed system in Eq. (1), we can define the SFF in the open system as
Here, we use the subscript to denote the SFF in open systems (that is the dissipation strength is non-zero). Also, we consider that this non-Hermitian Hamiltonian can be diagonalized, yielding a set of eigenstates denoted as . We represent them as which provides the second equality in Eq. (4). This spectrum originates from the Lindblad equation and is referred to as the Lindblad spectrum. When we set the dissipation strength in the Lindblad evolution as zero, we find that this definition is the same as that in the closed system Eq. (1). Our generalization to open quantum systems is consistent with the definition presented in Can’s work [51], referred to as the dissipative form factor. In Ref. [51], the primary focus is on Lindbladian terms with randomness, whereas our arguments remain valid for Lindbladian terms without randomness.
Since the imaginary part of the Lindblad spectrum is always non-negative, this SFF defined in Eq. (4) will not grow exponentially. Thus, although the Lindblad spectrum is complex, the SFF defined in Eq. (4) will decay exponentially in time till it reaches the steady state value. In addition, there is an alternative approach to defining the SFF in open systems that has a close relation to the definition Eq. (4), and the details of this discussion are included in the supplementary materials [65].
3 The general function of the normalized SFF
Let us now consider the behavior of the normalized SFF in open systems defined as
The motivation here is to find some general properties of this normalized SFF. We summarize some general properties of this normalized SFF including the early-time exponential decay behavior related to the Lindblad operators and the late-time plateau behavior related to the number of the steady state, and it is illustrated in Fig.1. We summarize these general properties below.
1) At the early time , the normalized SFF has an exponential decay behavior
Here and . is the Hilbert space dimension of the Hamiltonian .
2) The long-time behavior of this normalized SFF is a constant plateau whose value is given by
Below, we give some simple arguments for these general properties. At the short-time limit, we can perform a Taylor expansion in to the leading order:
This leads to
In the early-time regime, it is known that the correlation between the left and right systems in the doubled space is much smaller than the correlation within the same system [14], then we ignore the correlation contribution of the first term of the in Eq. (3) when evaluating the last line of Eq. (9). Using the fact that the second and the third terms of the commute with each other, we further obtain
This leads to the expression of in Eq. (6), and its detailed derivation is in the supplementary materials [65]. As time increases, the correlation between the left and right contours generally increases, thus the assumption above is not valid at the intermediate time. Therefore, the normalized SFF generally does not have this exponential decay behavior at the intermediate time scales .
The final plateau value of the normalized SFF can be understood by investigating Eq. (4). Only the steady state with zero-imaginary eigenvalue will give a non-vanishing contribution to the long-time plateau value of SFF, and this gives the expression Eq. (7). In addition, if there are more than one steady state, then Eq. (7) should be changed to . Here, is the total number of steady states.
Moreover, we can analyze the late-time regime using the effective field theory approach [11, 14]. The main idea is to approximate Green’s functions on the path-integral contour of the SFF by their counterparts on a Keldysh contour with an auxiliary imaginary time separation between forward and backward evolutions. The SFF defined in Eq. (4) can be written as the path-integral
Without any dissipation, the linear ramp can be understood as an integration over the zero mode and its conjugate variable . describes the relative time shift between forward and backward evolution branches and can be understood as the energy of the system. In closed systems, there is no coupling between two branches, and the effective action does not depend on . Consequently, the integral over from to leads to a linear slope. When the dissipation strength becomes small but finite, we find perturbatively
Here is the Wightmann Green’s function of operator with energy [14]
where is determined by the thermodynamic relation. This leads to a finite mass for , which increases linearly as time increases. In particular, as , the mode will be pinned at , which terminates the presence of the linear ramp. The role of different types of Lindblad operators in shaping the general properties of the normalized SFF can also be discussed [66].
4 Examples
In the following, we use the SYK model, the random matrix model, and the Bose−Hubbard model as examples to illustrate these general properties of the normalized SFF in the open system.
We comment here that the SYK model and the random matrix model are both good examples to analytically calculate the SFF since they both involve random averages over different realizations that rattle the energy eigenvalues. The random average smooths out the fluctuations that come from the oscillating terms in the SFF, thus making it a smooth function of time. In comparison, the SFF has extensive spikes in the Bose−Hubbard model that come from the zeros of the SFF, and we need to do the time slice average to get a smooth SFF curve.
4.1 SYK model
We consider the SFF of the SYK model [67-71] whose Hamiltonian is of the form
Here, is a random variable that satisfies the Gaussian distribution with mean zero and variance
and is the Majorana fermion operator. The Lindblad jump operators are chosen as the single Majorana Fermion operators.
We numerically compute the SFF for SYK model with in Fig.2, and there are several noteworthy features of this figure. First, we find that curves with different dissipation collapse well into a single line when they are plotted in terms of . Second, the early-time exponential decay in the SYK model is visible in Fig.2, and it agrees well with our analytical result at early time region . Third, the long-time value of the SFF curve is a non-vanishing plateau whose value is .
Furthermore, we can then write the SFF of the SYK model as a path-integral with the Lindblad operator chosen as the single Majorana fermion operator . Also, the dissipation strength is chosen as the constant . We can then solve the early-time saddle-point solutions of the effective action, and to the first-order of dissipation strength , the effective action at the saddle point is
Thus, we obtain the normalized SFF as . It has an exponential decay behavior at the early time. The details of the derivation of the SFF in the SYK model are included in the supplementary [65]. A similar analysis of the SFF in the Brownian SYK is also included, in which the normalized SFF also has an early-time exponential decay behavior [65]. Moreover, since the spectrum of the Majorana SYK model with N mod 8 is not 0 has a 2-fold degeneracy [4, 72], the final plateau value of the normalized SFF is instead of as shown in Fig.2.
4.2 The random matrix theory
We now consider the SFF in Gaussian unitary ensemble (GUE). The SFF we defined in Eq. (4) can be written in RMT as
with being a random matrix defined on doubled space. Here, and with and both are random Hermitian matrices. The bracket means an averaging with respect to the Gaussian distribution:
Then we consider the SFF in open systems in RMT. The SFF of open systems defined in Eq. (4) can be written as
In Fig.3, we present for the GUE of matrices with dimension . We find that without dissipation the SFF first dips below its plateau value and then climb back up in a linear fashion (this region is also called the ramp), joining onto the plateau as depicted in the right inset of Fig.3. Also, when we add a small dissipation, we find a similar dip-ramp behavior of the SFF, whereas it then decays to a plateau value that is lower than the case without dissipation. Moreover, the height of the plateau is of order without dissipation which is the mean level spacing, and the height of the plateau is of order with non-zero dissipation.
To understand this behavior of SFF with dissipation, we can directly calculate the normalized SFF, and the derivation details are included in the supplementary material [65]. We obtain the normalized SFF at early times
and this is an exponential decay behavior which is also visible in the numerical results in Fig.3, and it is in good agreement with at . On the other hand, in the long time limit , we find , and . This explains the difference between the final plateau value in the case with and without dissipation as depicted in Fig.3.
4.3 Bose−Hubbard model
We now consider the SFF of the 1D Bose−Hubbard model with dissipation. The Hamiltonian of the Bose−Hubbard model is
Here, is the strength of the nearest neighbor hopping, and is the strength of the on-site interaction. In an open system, we set as a time-independent dissipation strength. Also, we set the Lindblad jump operators as . Here , and is the total number of sites.
The normalized SFF of the Bose−Hubbard model is illustrated in Fig.4, and SFF is shown in the right inset. In our numerical simulation, we set which is in the quantum critical region of 1D BHM [73]. Previous simulations suggest that the system exhibits quantum many-body chaos [74], although it is debatable that the system is most chaotic near the criticality [75, 76]. Meanwhile, since the SFF has extensive spikes in the Bose−Hubbard model, we perform the time slice average to get a smooth SFF curve in Fig.4. This time average excludes possible non-general features, as discussed in Refs. [61, 62] for closed systems. The number of time points that we average over is . The details of this average are added in the supplementary [65]. The initial exponential decay curve obtained by Eq. (6) is also included for comparison. The early-time exponential decay of the normalized SFF is visible in the left inset of Fig.4, and it agrees well with the theoretical curve at .
5 Conclusion
In this letter, we have generalized the SFF to open quantum systems driven by the Lindblad master equation. We show that the normalized SFF of open systems generally has a dip-ramp structure and then decays to the plateau behavior at small dissipation strength. In particular, we unveil two general properties of the normalized SFF including the early-time exponential decay behavior determined by the Lindblad operators and the late-time plateau behavior that relates to the number of steady states. Our main tools are the SYK model, the random matrix model, and the Bose−Hubbard model. Using numerical techniques, we have obtained the behavior of SFF in these three models at all times. Then we are able to extract the general early-time and late-time behaviors of the normalized SFF, and we find good agreement between the numerics and analytical results.
Our work potentially opens up many interesting directions: firstly, the dynamics of the SFF of open systems have a close relationship with the Lindblad spectrum [77], and therefore the SFF can be used as a diagnosis of the structure of the Lindblad spectrum. Secondly, it will be interesting to study the intermediate time scales behavior of the SFF of the open system which might go through a phase transition and have some critical behaviors [54]. Thirdly, the SFF in open systems that we discussed here can be similarly measured in experiments [78-80] via generalization to the doubled space, and the detail is left to the appendix [65].
Meanwhile, the dynamical manifestations of level repulsion can be shown in the form of a drop in the value of the survival probability below its saturation point, which is known as the correlation hole [81-85]. Since the survival probability is the probability of finding the system in its initial state at a later time, this survival probability is the same as the SFF at inverse temperature when the initial state is chosen as the coherent Gibbs state of inverse temperature . Therefore, the dip-ramp behavior of the correlation hole has a close relation to the SFF. To generalize the study of survival probability in open quantum systems, we can replace the unitary evolution with an evolution governed by the Lindblad master equation. This results in an alternative definition of the SFF in open systems, which includes off-diagonal terms between eigenstates of the Hamiltonian, as discussed in the Electronic Supplementary Materials (Appendix A) [65]. Numerically, we verify that this new definition closely corresponds to the definition discussed in the main text for nearly the entire time regime. Consequently, we anticipate that the investigation of correlation holes can also be extended to open systems. A comprehensive study of this extension, however, will be postponed in future works.
Moreover, the Lindbladian description of open systems relies on the Markovian approximation of the environment. Consequently, time scales that exceed the Markovian approximation may not be accurately described by the Lindblad master equation. For open systems that reach their steady state within a time scale shorter than this Markovian approximation time scale, this is typically not a significant challenge. However, it is possible that in certain specific many-body systems, the steady state is not achieved within the time frame of the Markovian approximation. In such cases, our analysis of the long-time plateau behavior, which is related to the Lindblad operators, may not be entirely reliable as the Lindblad description is not suitable in this regime.
The Lindblad equation requires the Markovian−Born approximation and the secular approximation on the interaction term [86]. Building on previous studies of the Markovian approximation, for times , where represents the width of the bath system correlation spectrum, the Markovian approximation becomes applicable [87]. The Markovian approximation provides a description on a coarse-grained time scale with the assumption that environmental excitations decay over times that are not resolved. However, if the time duration is too long, environmental excitations will influence the original system, and this characteristic time scale depends on the relative degrees of freedom, temperature, and the detailed spectrum shape of the bath. Therefore, comparing the Heisenberg time and the failure time of the Markovian approximation is a specific problem that varies with different settings. Therefore, it is important to emphasize that the generality we have discussed in our paper is applicable within the time domain where the Markovian treatment of the environment holds. Time scales exceeding this domain require further exploration, and we leave this for future studies
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If we simply generalize the definition of the SFF for non-Hermitian systems as follows: Fγ(t)=1[ Z(0)]2∑ m,n e− i( ϵm− ϵn)t. where {ϵn} is the set of eigenvalues of the non-Hermitian system, and we denote the real and imaginary parts of the eigenvalues as αn and βn respectively. Since the energy eigenvalues of a general non-Hermitian system are complex, implying that the imaginary part βn is generally nonzero, from the definition we observe that Fγ(t)=1[ Z(0)]2∑ m,n e− i( αm− αn)te(βm−βn) t. Hence, for the set of m, n that satisfies βm −βn > 0, there will be an exponential growth term e(βm−βn) t in the above definition, resulting in the exponential growth of the SFF as time increases.
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In this supplementary, we show (A) alternative definitions of SFF; (B) the derivation of the pre-factor α in early decay region; (C, D, E) detailed calculation of SFF in three examples; (F) possible experimental realization of SFF.
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In general, we think the types of different Lindblad operators will not change the general properties of the normalized SFF regarding its short-time exponential decay and long-time plateau behavior. Since the argument we provide just below Eq. (9) does not resume some specific form of the Lindblad operators. Nevertheless, different Lindblad operators may lead to a different number of steady states, thereby altering the value of θ. For example, let us consider a Hamiltonian H with charge conservation, such as our Bose‒Hubbard model. In the main text, we focus on Lindblad operators that preserve the particle number, ensuring that charge conservation is a strong U(1) symmetry of the open system. In this scenario, there is at least one steady state in each charge sector, resulting in at least N + 1 steady states in the full Fock space with arbitrary particle numbers. (Note that our discussions in the main text focus on a single charge sector.) In contrast, when some Lindblad operators couple different charge sectors, the system exhibits only a weak U(1) symmetry. Consequently, there may be only one steady state even in the full Fock space.
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