A simple unilateral homogenous PhOLEDs with enhanced efficiency and reduced efficiency roll-off

Shaoqing ZHUANG, Wenzhi ZHANG, Xiao YANG, Lei WANG

PDF(202 KB)
PDF(202 KB)
Front. Optoelectron. ›› 2013, Vol. 6 ›› Issue (4) : 435-439. DOI: 10.1007/s12200-013-0349-3
RESEARCH ARTICLE
RESEARCH ARTICLE

A simple unilateral homogenous PhOLEDs with enhanced efficiency and reduced efficiency roll-off

Author information +
History +

Abstract

In this paper, highly efficient phosphorescent organic lighting emitting diodes (PhOELDs) with low efficiency roll-off are demonstrated by using a unilateral homogenous device structure with wide band-gap material 4, 4', 4″-tri(N-carbazolyl)-triphenylamine (TCTA) as hole transporting layer and emitting layer (EML). The optimized blue device exhibits a high power efficiency of 40 lm/W, external quantum efficiency of 19.2% and current efficiency of 37.7 cd/A. More importantly, the device exhibits a low efficiency roll-off at 1000 cd/m2. In addition, the white homogenous PhOLEDs only exhibits the efficiency roll-off 5.6% and 17.5%, corresponding to the brightness of 1000 and 5000 cd/m2 respectively. These interesting results demonstrate that the simple unilateral homogenous device structure is a promising way to enhance the device efficiency and reduce the efficiency roll-off.

Keywords

enhance efficiency / efficiency roll-off / unilateral homogenous structures

Cite this article

Download citation ▾
Shaoqing ZHUANG, Wenzhi ZHANG, Xiao YANG, Lei WANG. A simple unilateral homogenous PhOLEDs with enhanced efficiency and reduced efficiency roll-off. Front Optoelec, 2013, 6(4): 435‒439 https://doi.org/10.1007/s12200-013-0349-3

References

[1]
Tang C W, VanSlyke S A. Organic electroluminescent diodes. Applied Physics Letters, 1987, 51(12): 913-915
CrossRef Google scholar
[2]
Fukase A, Dao K L T, Kido J. High-efficiency organic electroluminescent devices using iridium complex emitter and arylamine-containing polymer buffer layer. Ploymers for Advanced Technologies, 2002, 13(8): 601-604
CrossRef Google scholar
[3]
Tanaka D, Sasabe H, Li Y J, Su S J, Takeda T, Kido J. Ultra high efficiency green organic light-emitting devices. Japanese Journal of Applied Physics, 2007, 46(1): L10-L12
CrossRef Google scholar
[4]
Su S J, Tanaka D, Li Y J, Sasabe H, Takeda T, Kido J. Novel four-pyridylbenzene-armed biphenyls as electron-transport materials for phosphorescent OLEDs. Organic Letters, 2008, 10(5): 941-944
CrossRef Pubmed Google scholar
[5]
Kim H, Cho N S, Oh H Y, Yang J H, Jeon W S, Park J S, Suh M C, Kwon J H. Highly efficient red phosphorescent dopants in organic light-emitting devices. Advanced Materials, 2011, 23(24): 2721-2726
CrossRef Pubmed Google scholar
[6]
Fan C H, Sun P, Su T H, Cheng C H. Host and dopant materials for idealized deep-red organic electrophosphorescence devices. Advanced Materials, 2011, 23(26): 2981-2985
CrossRef Pubmed Google scholar
[7]
Malliaras G G, Scott J C. The roles of injection and mobility in organic light emitting diodes. Journal of Applied Physics, 1998, 83(10): 5399-5403
CrossRef Google scholar
[8]
Polikarpov E, Swensen J S, Chopra N, So F, Padmaperuma A B. An ambipolar phosphine oxide-based host for high power efficiency blue phosphorescent organic light emitting devices. Applied Physics Letters, 2009, 94(22): 223304
CrossRef Google scholar
[9]
Gong S, Chen Y, Luo J, Yang C, Zhong C, Qin J, Ma D. Bipolar tetraarylsilanes as universal hosts for blue, green, orange, and white electrophosphorescence with high efficiency and low efficiency roll-off. Advanced Functional Materials, 2011, 21(6): 1168-1178
CrossRef Google scholar
[10]
Chou H H, Cheng C H. A highly efficient universal bipolar host for blue, green, and red phosphorescent OLEDs. Advanced Materials, 2010, 22(22): 2468-2471
CrossRef Pubmed Google scholar
[11]
Xiao L, Su S J, Agata Y, Lan H, Kido J. Nearly 100% internal quantum efficiency in an organic blue-light electrophosphorescent device using a weak electron transporting material with a wide energy gap. Advanced Materials, 2009, 21(12): 1271-1274
CrossRef Google scholar
[12]
Lee J H, Huang C L, Hsiao C H, Leung M K, Yang C C, Chao C C. Blue phosphorescent organic light-emitting device with double emitting layer. Applied Physics Letters, 2009, 94(22): 223301
CrossRef Google scholar
[13]
Zhang X W, Li J, Khan M, Zhang L, Jiang X Y, Haq K, Zhu W Q, Zhang Z L. Improved chromaticity and electron injection in a blue organic light-emitting device by using a dual electron-transport layer with hole-blocking function. Semiconductor Science and Technology, 2009, 24(7): 075021
CrossRef Google scholar
[14]
Cai C, Su S J, Chiba T, Sasabe H, Pu Y J, Nakayama K, Kido J. Efficient low-driving-voltage blue phosphorescent homojunction organic light-emitting devices. Japanese Journal of Applied Physics, 2011, 50(4): 040204
CrossRef Google scholar
[15]
Tsuji H, Mitsui C, Sato Y, Nakamura E. Bis(carbazolyl)benzodifuran: a high-mobility ambipolar material for homojunction organic light-emitting diode devices. Advanced Materials, 2009, 21(37): 3776-3779
CrossRef Google scholar
[16]
Wang Q, Tao Y, Qiao X, Chen J, Ma D, Yang C, Qin J. High-performance, phosphorescent, top-emitting organic light-emitting diodes with p-i-n homojunctions. Advanced Functional Materials, 2011, 21(9): 1681-1686
CrossRef Google scholar
[17]
Jang S E, Yook K S, Lee J Y. High power efficiency in simplified two layer blue phosphorescent organic light-emitting diodes. Organic Electronics, 2010, 11(6): 1154-1157
CrossRef Google scholar
[18]
Qiao X, Tao Y, Wang Q, Ma D, Yang C, Wang L, Qin J, Wang F. Controlling charge balance and exciton recombination by bipolar host in single-layer organic light-emitting diodes. Journal of Applied Physics, 2010, 108(3): 034508
CrossRef Google scholar
[19]
Zhang H, Huo C, Zhang J, Zhang P, Tian W, Wang Y. Efficient single-layer electroluminescent device based on a bipolar emitting boron-containing material. Chemical Communications (Cambridge), 2006, (3): 281-283
CrossRef Google scholar
[20]
Seo J H, Lee S J, Seo B M, Moon S J, Lee K H, Park J K, Yoon S S, Kim Y K. White organic light-emitting diodes showing nearly 100% internal quantum efficiency. Organic Electronics, 2010, 11(11): 1759-1766
CrossRef Google scholar
[21]
Chen H, Lee J, Shiau C. Electromagnetic modeling of organic light-emitting devices. Journal of Lightwave Technology, 2006, 24(6): 2450-2457
CrossRef Google scholar
[22]
Su S J, Chiba T, Takeda T, Kido J. Pyridine-containing triphenylbenzene derivatives with high electron mobility for highly efficient phosphorescent OLEDs. Advanced Materials, 2008, 20(11): 2125-2130
CrossRef Google scholar

Acknowledgements

This research work was supported by the National Natural Science Foundation of China (Grant Nos. 21161160442 and 51203056), the National Basic Research Program of China (973 Program) (No. 2013CB922104), Wuhan Science and Technology Bureau (NO. 01010621227) and the Open Research Fund of State Key Laboratory of Polymer Physics and Chemistry.

RIGHTS & PERMISSIONS

2014 Higher Education Press and Springer-Verlag Berlin Heidelberg
AI Summary AI Mindmap
PDF(202 KB)

Accesses

Citations

Detail

Sections
Recommended

/