Characterization of micro-mixing in a novel impinging streams reactor

Hui HU, Zhiming CHEN, Zhen JIAO

PDF(162 KB)
PDF(162 KB)
Front. Chem. Sci. Eng. ›› 2009, Vol. 3 ›› Issue (1) : 58-64. DOI: 10.1007/s11705-009-0106-8
RESEARCH ARTICLE
RESEARCH ARTICLE

Characterization of micro-mixing in a novel impinging streams reactor

Author information +
History +

Abstract

This paper presents an experimental investigation of a novel impinging stream reactor (ISR) with the aim of high mixing intensity. The integral mixing quality in the reactor was measured with the iodide-iodate reaction and showed excellent mixing performance. The impact of the operating parameters, such as fluxes, circulation and inter-nozzle distances, was investigated in terms of segregation index. The results showed that the increase of flux, the decrease of inter-nozzle distance and a suitable circulation can improve the micro-mixing efficiency. Based on turbulence theory, it was estimated that the characteristic micro-mixing time was 0.002—0.02 s, which was much shorter than that in the stirred tank reactor. The micro-mixing time was related to the segregation index, which was in good agreement with those in the literature.

Keywords

micro-mixing / impinging streams reactor / turbulent mixing / mass transfer

Cite this article

Download citation ▾
Hui HU, Zhiming CHEN, Zhen JIAO. Characterization of micro-mixing in a novel impinging streams reactor. Front Chem Eng Chin, 2009, 3(1): 58‒64 https://doi.org/10.1007/s11705-009-0106-8

References

[1]
Ji L J, Liu H F, Wang F C, Yu Z H. Residence time distribution of impinging stream reactor. Journal of East China University of Science and Technology, 2006, 32(1): 24-27 (in Chinese)
[2]
Wang S J, Mujumdar A S. Three-dimensional analysis of flow and mixing characteristics of a novel in-line opposing-jet mixer. Ind Eng Chem Res, 2007, 46: 632-642
CrossRef Google scholar
[3]
Florian S, Johannes G, Hans C S, Wolfgang P, Michael M. The low Reynolds number turbulent flow and mixing in a confined impinging jet reactor. Int J Heat and Fluid Flow, 2007, 28: 1429-1442
CrossRef Google scholar
[4]
Xiao Y, Chen Y, Wu Y. Determining micro-mixing characteristic time constant in SCISR with azo coupling reaction. Journal of South-Central University for Nationalities, 2005, 24(2): 5-8 (in Chinese)
[5]
Ou Yang C B, Liu Y Z, Qi G S, Yang L R. Function study on micro mixing in impinging stream-rotating packed bed reactor. Applied Chemical Industry, 2003, 31(5): 22-24
[6]
Norbert K, Thomas K, Michael E, Peter W. Convective mixing and chemical reactions in microchannels with high flow rates. Sensors and Actuators B, 2006, 117: 495-508
CrossRef Google scholar
[7]
Fournier M C, Falk L, Villermaux J. A new parallel competing reaction system for assessing micro-mixing efficiency: experimental approach. Chemical Engineering Science, 1996, 52(22): 5053-5064
CrossRef Google scholar
[8]
Zhang J W. Study of the flow field characteristic of submerged circulative impinging stream reactor. Dissertation for the Doctoral Degree. Shenyang: Northeast University, 2004, 20-22 (in Chinese)
[9]
Guichardon P, Falk L. Characterisation of micro-mixing efficiency by the iodide-iodate reaction system. Part I: experimental procedure. Chemical Engineering Science, 2000, 55: 4233-4243
CrossRef Google scholar
[10]
Palmer D A, Ramette R W, Mesmer R E. Triodide ion formation equilibrium and activity coefficients in aqueous solution. Journal of Solution Chemistry, 1984, 13(9): 673-683
CrossRef Google scholar
[11]
Allen T L, Keefer R M. The formation of hypoiodous acid and hydrated iodine cation by the hydrolysis of iodine. J Am Chem Soc, 1955, 77: 2957-2960
CrossRef Google scholar
[12]
Wei Y J, Liu C G, Mo L P. Ultraviolet absorption spectra of iodine , iodide ion and triiodide ion. Spectroscopy and Spectral Analysis, 2005, 25(1): 86-88 (in Chinese)
[13]
Bourne J R, Martin S. Fast reaction in rotor-stator mixers of different size. Chemical Engineering and Progressing, 1992, 31: 285-296
CrossRef Google scholar
[14]
Zhao Y C, Ying Y, Chen G W, Yuan Q. Characterization of micro-mixing in T-shaped micro-mixer. Journal of Chemical Industry and Engineering, 2006, 57(8): 1884-1890 (in Chinese)
[15]
Baldyga J, Bourne J R. Comparison of the engulfment and the interaction-by-exchange-with-the-mean micro-mixing models. Chemical Engineering Journal, 1990, 45(1): 25-31
CrossRef Google scholar
[16]
Liu P D, Futran M, Midler M, Paul E L. Particle size design of pharmaceuticals by continuously impinging jets precipitation. AIChE Meeting, Chicago, 1990
[17]
Amarjit J M, Donald J K. Micromixing effects in a two-impinging-jets precipitator. AIChE Journal, 1996, 42(7): 1801-1814
CrossRef Google scholar
[18]
Tamir A. Impinging stream reactor-fundamentals and application. Amsterdam: Elsevier, 1994: 39-54
[19]
Tamir A. Processes and phenomena in impinging-stream reactors. Chemical Engineering Progress, 1989, 85 (9): 53-61

RIGHTS & PERMISSIONS

2014 Higher Education Press and Springer-Verlag Berlin Heidelberg
AI Summary AI Mindmap
PDF(162 KB)

Accesses

Citations

Detail

Sections
Recommended

/