Manipulating atomic states via optical orbital angular-momentum

Xiong-jun LIU , Xin LIU , Leong-Chuan KWEK , Choo Hiap OH

Front. Phys. ›› 2008, Vol. 3 ›› Issue (2) : 113 -125.

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Front. Phys. ›› 2008, Vol. 3 ›› Issue (2) :113 -125. DOI: 10.1007/s11467-008-0024-0
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Manipulating atomic states via optical orbital angular-momentum
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Abstract

Optical orbital angular-momentum (OAM) has more complex mechanics than the spin degree of photons, and may have a broad range of application. Manipulating atomic states via OAM has become an interesting topic. In this paper, we first review the general theory of generating adiabatic gauge field in ultracold atomic systems by coupling atoms to external optical fields with OAM, and point out the applications of the generated adiabatic gauge field. Then, we review our work in this field, including the generation of macroscopic superposition of vortex-antivortex states and spin Hall effect (SHE) in cold atoms.

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orbital angular momentum / adiabatic Gauge field / vortex states / spin Hall effect / quantum state transfer / ultracold atoms

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Xiong-jun LIU, Xin LIU, Leong-Chuan KWEK, Choo Hiap OH. Manipulating atomic states via optical orbital angular-momentum. Front. Phys., 2008, 3 (2) : 113-125 DOI:10.1007/s11467-008-0024-0

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1 Introduction

Coherent optical control of the quantum state of atoms is the most important task in quantum optics and atomic physics, in terms of the application to quantum information science and discovering the basic features of quantum many-body physics. A direct control of atomic quantum states can be achieved by transferring the external optical information to atoms via atom-light interaction [1−19]. The technique of quantum state transfer between photons and atoms has vital importance in the practical quantum information technologies. As a result, developing appropriate techniques for coherent transfer of quantum states between photons and atoms has become one of the central topics of quantum information science and been widely studied in both theory and experiment in recent years. The elegant schemes of this field include, e.g. the coherent control of single-atom by high-Q cavity QED [1−5], and the quantum state transfer between photons and an ensemble of atoms through electromagnetically induced transparency (EIT) [6−22]. The applications of coherent manipulation of atomic quantum states are now widely investigated in quantum memory, quantum computing, and quantum teleportation [23−28].

On the other hand, it has been widely acknowledged that ultracold atomic gases have become an ideal play-ground to experimentally investigate many-body physics [29]. The remarkable controllability in the parameters of these systems allows a clean study of complexr physics in a controllable fashion. One of the most exciting advances in ultracold atomic gases is that rotating Bose-Einstein condensates (BECs) provide a conceptual link between the physics of trapped gases and the physics of condensed matter systems such as superfluids, type-II superconductors, and quantum-Hall effect (QHE) materials [30−36]. In the rotating BEC systems, the trap rotation provides an effective magnetic field for the electrically neutral atoms. For this, the Abrikosov lattice of quantized vortices [37] and the analog of the fractional quantum Hall effect (FQHE) can be studied.

Recent advances in the optical coherent manipulation of ultracold atoms suggest an alternative to create adiabatic gauge fields for the atomic systems by coupling the atoms to external optical fields which are spatially dependent in the amplitude and phase [38−41], e.g. optical fields with orbital angular-momentum (OAM). Optical OAM has more complex mechanics than the spin degree of photons, and can have a broad range of application [42, 43]. The simplest class of light field carrying OAM is an optical vortex, which is a beam of light whose phase varies in a corkscrew-like manner along the beam’s direction of propagation [45, 46]. The interacting Hamiltonian of atoms and optical field with OAM depends on the local spatial parameters, which results in an adiabatic gauge field for the motion of atoms under the adiabatic condition. Properly modifying the external optical fields yields different types of effective magnetic field, the curvature of the adiabatic gauge field. Different from the rotating BECs where only the constant and spin-independent effective magnetic field can be obtained [30], the effective magnetic field created using optical means has more freedom to be shaped and controlled, and then is very helpful to study new physics in ultracold atoms.

In this paper, we first review the basic idea of generating adiabatic gauge field in ultracold atomic system by coupling atoms to external optical fields with OAM, and point out the applications of the generated adiabatic gauge field. Then, we review our work in this field, including the generation of macroscopic superposition of vortex-antivortex states and spin Hall effect (SHE) in cold atoms.

The paper is organized as follows. In Section 2, we introduce the general discussion on the adiabatic gauge field for the ultracold atomic system; in Section 3, we give an example of the adiabatic gauge field in the three-level system; in Section 4, we discuss how to generate macroscopic superposition of vortex-antivortex states from a five-level M-type atomic system; in Section 5, we introduce an intriguing application of the created adiabatic gauge field: spin Hall effect in ultracold atoms; concluding remarks are given in Section 6.

2 Adiabatic gauge field in quantum system

2.1 Unitary transformation

The idea that adiabatic gauge fields can be generated in quantum systems was first proposed by Wilczek and Zee more than twenty years ago [47]. In this section, we shall review the general theory of the adiabatic gauge fields created in the quantum N-level systems. For convenience, we denote H0(r) as the unperturbed Hamiltonian that describes the N internal levels |χk〉(k=1,2,⋯,N) for the system, and Ek as the eigenvalue of the corresponding energy level. In the presence of perturbation Hamiltonian HI that can be created through e.g. external trap potentials, laser-induced coupling for atomic systems, etc., the dynamics of the quantum system can be studied via perturbation theory. Without loss of generality, in this paper we consider the case of a weak perturbation so that HI does not induce the energy shift to the energy levels of internal Hamiltonian, but causes the coupling between different eigenstates |χk〉. For this we can generally expand the wave function for the system according to Ψ˜(r,t)=∑k=1NΨk(r)exp(−iEkt/ℏ)|χk〉, where Ek is the eigenvalue of the corresponding internal energy level. Denoting by Ψ = (Ψ1, Ψ2, · · ·, ΨN)T, the coupling between states Ψk by the interaction Hamiltonian can be given by

(1)iℏ∂Ψ∂t=[−ℏ22m∇2+V(r)]Ψ+HI(r)Ψ

where V(r) is the external trap potential, and the interacting Hamiltonian HI depends on the local parameters, e.g. the spatial position r. The diagonalization of the interacting Hamiltonian can be done through a local unitary transformation U(r),

(2)Ψ=U(r)Φ, HId=U†HIU

where Φ = (Φ1, Φ2, · · ·, ΦN) is the diagonalized basis of the interacting Hamiltonian, and HId is diagonal on this basis. The diagonal elements (HId)kk = Ek represents the eigenvalue of Φk. Note that the specific form of the unitary transformation U(r) shall be solely determined by the interacting Hamiltonian. Substituting the transformation (2) into Eq. (1) we obtain the equation of evolution for Φ that

(3)iℏ∂Φ∂t=−ℏ22mU†∇2UΦ+U†V(r)UΦ+HId(r)Φ

The form of the above equation can be simplified by introducing the gauge potential

(4)A(r)=iℏceU†(r)∇U(r)

with e the electric charge constant.

Relying on the above definition of the gauge potential and after a straightforward calculation we find that the Eq. (3) can be rewritten as follows:

(5)iℏ∂Φ∂t=12m[iℏ∇+ecA(r)]2Φ+V′(r) Φ+HId(r) Φ

where V′=U†V(r)U. Since U(r) considered here is a local unitary transformation on the N-dimensional Hilbert space, it is an N × N parameter-dependent matrix. As a result, the gauge defined based on Eq. (4) is non-Abelian and of the N × N matrix form (of the SU (N) symmetry). The non-Abelian gauge field is associated with the curvature (effective magnetic field) that is given by

(6)Fμν=∂μAν−∂νAμ−iec[Aμ,Aν]

with the magnetic field Bj = 1/2ϵjklFkl. One should keep in mind that to this step we do not apply the adiabatic condition in the equation of motion. The gauge field defined in Eq. (4) is a pure gauge and it is easy to verify that Fµν = 0. It is noteworthy that the non-Abelian pure gauge may have nontrivial significance by resulting in a phase to the wave function Φ:

(7)Φ(r,t)→Peieℏc∫A⋅dlΦ(r,t)

where P is the operator of chronological ordering. The above phase factor is known as Wilson loop integral [48]. This phase factor can be non-zero even for a pure gauge, since for the non-Abelian gauge field we have ∇×A≠B=0. To find the possible observable physics for this phase factor is an interesting issue in gauge field theory.

2.2 Adiabatic condition

In this paper, however, we are interested in the case that the adiabatic condition can be applied and then the adiabatic gauge field is obtained [49]. Under the adiabatic condition, the adiabatic gauge potential is generally associated with a non-zero curvature

(8)Fμν≠0

To have more sense of the adiabatic gauge field obtained above, we consider two special cases in the following.

First, let us suppose that the system is nondegenerate, i.e., En is different for different eigenstates Φn. Besides, the coupling between each two states, say Φj and Φk, induced by the off-diagonal element Ajk(r) satisfies

(9)|P⋅Ajkm(Ej−Ek)|≪1

the adiabatic condition is then approved and the transition between different states in Eq. (5) can be ignored. The non-Abelian gauge field is reduced from SU(N) symmetry to N independent U(1) Abelian gauge fields with

(10)Aj(r)=iℏce(U†(r)∇U(r))jj=iℏ〈Φj|∇|Φj〉, j=1,2,⋯,N

and the corresponding scalar potential after applying the adiabatic condition:

(11)ϕj(r)=12m∑k≠jAjk⋅Akj, j=1,2,⋯,N

In the dynamical equation of evolution (5), all components of the column vector Φ become decoupled to each other and now yield

(12)iℏ∂Φj∂t=12m[iℏ∇+ecAj(r)]2Φj+V¯j'(r)Φj

with Vj'(r) = V'(r)+ϕj+Ej. The curvature of U(1) gauge fields is given by

(13)Fμν(j)=∂μAν(j)−∂νAμ(j)

which is generally non-zero.

Another interesting possibility is that the system has degeneracy. Without loss of generality, we suppose Φ1, Φ2, · · ·, Φm(m < N) consist of the degenerate subspace of the system, with energy eigenvalue Eg that differs from the eigenvalues of all remaining states. Similarly, when

(14)|P⋅Aijm(Eg−Ej)|≪1

where i = 1, 2, · · ·, m and j = m + 1, m + 2, · · ·, N. Then we denote reduced column vector Φ′ = ( Φ1, Φ2,⋯, Φm)T, which satisfies the equation:

(15)iℏ∂Φ′∂t=12m[iℏ∇+ecA'(r)]2 Φ′+[V′(r)+ϕ′+Eg] Φ′

where A′(r) is still non-diagonal U(m) gauge field and Ajk'(r)=iℏce(U†(r)∇U(r))jk. The scalar field ϕ′ is also an m × m matrix with the elements ϕjk'=12m∑l>mAjl· Alk. The curvature can also be calculated with the Eq. (6), but now it is generally nonzero.

3 Example of adiabatic gauge field: three-level atomic system

As an example, in this section we calculate the adiabatic gauge field in the three-level Λ-type atomic system which couples to two external laser fields.

The three-level Λ-type system is shown in Fig. 1. The transition |c〉→|a〉 is resonantly coupled by a pump field with the Rabi-frequency Ω1 = Ω1(0)exp(ik1⋅r), where Ω1(0)(r) is the slowly spatially varying amplitude and k1 is the wave-vector. The probe field, whose Rabi frequency Ω2=Ω2(0)(r)ei[ϕ(r)+k2⋅r] with Ω2(0)(r) the slowly spatially varying amplitude, couples resonantly the transition |b〉 → |a〉, where k2 is wave-vector of the probe field. ϕ(r) is the spatially-dependent phase. Defining the flip operators as σ^μν=|μ〉〈ν| with the level indices µ, ν = a, b, c, the Hamiltonian in the present system reads

(16)H=H0+HIH0=−ℏ22me∇2+V(r)HI=−(ℏΩ2σ^ab+ℏΩ1σ^ac)+h.c.

where V (r) is the external trap potential. To facilitate the subsequent discussion, H0 is written in r-representation other using flip operators in Eq. (16). The interaction Hamiltonian HI can be diagonalized with the local unitary transformation: H˜I=U(r)HIU†(r) with

(17)U(r)=(1212sinθe−iS(r)12cosθ0cosθ−sinθeiS(r)12−12sinθe−iS(r)−12cosθ)

where S = (k2−k1) · r + ϕ(r) and the mixing angle tan θ(r) = |Ω2/Ω1|. Under this unitary transformation, the three eigenstates of HI are easily obtained as

(18)|Φ+〉=12(|a〉+sinθe−iS(r)|b〉+cosθ|c〉)|Φ0〉=cosθ|b〉−sinθeiS(r)|c〉|Φ−〉=12(|a〉−sinθe−iS(r)|b〉−cosθ|c〉)

with the corresponding eigenvalues E± = ∓ℏ2Ω0 and E0 = 0 where Ω0=|Ω1|2+|Ω2|2. It is interesting that |Ψ0〉, typically known as the dark state for a three-level Λ system [6, 7, 9, 10, 19−22], is a coherent superposition of two ground states, excluding the excited state. Dark state is also a central idea for the electromagnetically induced transparency (EIT), a prevailing modern technique in recent years to realize the slow light and quantum memory for photons [6−14].

According to the definition given in the previous section, by a straightforward calculation we find that the 3 × 3 matrix A in the three-level system has the following form:

(19)A=ℏce(12sin2θ∇S(i12∇θ+122sin2θ∇S)e−iS−12sin2θ∇S(−i12∇θ+122sin2θ∇S)eiS−sin2θ∇S(i12∇θ−122sin2θ∇S)eiS−12sin2θ∇S(−i12∇θ−122sin2θ∇S)e−iS12sin2θ∇S)

which generally is a SU(3) non-Abelian gauge potential. Noting that the present system is non-degenerate, we have particular interest in the case when the adiabatic condition is satisfied. For this we require

(20)|v⋅Aαβ(Eα−Eβ)|≪1, α≠β=+,−,0

which can be satisfied for sufficient large Rabi-frequency and small motion velocity. Under this condition we ignore the off diagonal elements of the gauge potential. A most interesting result can be achieved by applying the probe field with orbital angular momentum (OAM) ℏl. In this way, the spatially-dependent phase of the probe field has the form: ϕ(r) = l arctan(y/x). Furthermore, we consider the special situation that the Rabifrequency rate between the probe and pump fields satisfies |Ω2Ω1| = λρ ∝ ρ with ρ = x2+y2 the distance from z axis, and |Ω2|≪|Ω1|, i.e., the probe field is much weaker than the pump field. The diagonal elements of gauge potential (19) follows the three constant effective magnetic fields

(21)B++=B−−=ℏlcλ2/ee^z, B00=−2ℏlcλ2/ee^z

This result clearly shows that atoms in the dark state (|Φ0〉) and in the bright states (|Φ±〉) experience the opposite magnetic fields, respectively in +z and −z direction. Such a situation will result in the different Landau-level structure for dark-state and bright-state particles (Fig. 2). If we further apply an effective electric field in say x direction, we can find atoms in | Φ0〉 move in the+y direction, while the atoms in | Φ±〉 move in the −y direction. This is in fact the basic idea in generating spin current in atoms [50, 51].

An interesting extension from the above situation can be done by considering the four-level atomic tripod system [41], where there are three ground states. Two independent dark states in the tripod level configuration consist of the degenerate subspace of the system. According to our general discussion in Section 2, this will result in a U (2) non-Abelian gauge field in the atomic adiabatic dynamics. The possibility of realization of monopole gauge field is also discussed in Ref. [41].

4 Generation of macroscopic superposition of vortex-antivortex states

By now we have shown that applying laser fields with OAM can generate effective magnetic fields for the orbital motion of atoms. This result can be understood as the coherent transfer of OAM between optical fields and atoms. A natural idea following this result is that one can generate atomic vortex states by transferring the optical vortex to atoms. As is well-known, in cold atoms such as Bose-Einstein condensates (BECs) in dilute gases, the stable existence of quantized vortices is one of the most striking and fascinating signatures of superfluidity [52]. Many works have been done on the nucleation of vortex lattices in a BEC cloud by stirring the BEC cloud via rotating external trap potentials [30]. On the other hand, excitation of vortices in BECs, using the optical vortex beams, has been proposed recently using Raman techniques [53−55]. In this section we introduce the scheme, first proposed in Ref. [56] and in Ref. [57], for creation of macroscopic superpositions of vortex-antivortex states through coherent transfer of OAM between laser fields and cold atoms.

Consider an ensemble of condensed atoms with internal five-level M type configuration interacting with four laser beams (Fig. 3). Two strong control lasers respectively drive the transitions |2〉 → |4〉 and |3〉 →|5〉 with Rabi frequencies Ωc1 = Ωc1(0)exp(ikc1 ⋅ r) and Ωc2 = Ωc2(0)exp(ikc2 ⋅ r), where kcj is the wavevector. The probe fields, Ωp1 = Ωp1(0)ei(lϕ+kp1⋅r) and Ωp2 = Ωp2(0)ei(l′ϕ+kp1⋅r), respectively couple the transitions |1〉 → |4〉 and |1〉 → |5〉 with the wave-vectors kpj = kpjz^(j = 1,2). Ωcj(0) and Ωpj(0)(j = 1,2) are the slowly varying amplitudes. Similarly, here we have allowed the two probe photons to have orbital angular momentum ℏl and ℏl′, respectively. It is convenient to introduce the time-slowly-varying amplitudes Ψ2 = Φ2e−i(ωp1−ωc1)t, Ψ4 = Φ4e−iωp1t, Ψ3 = Φ3e−i(ωp2−ωc2)t, and Ψ5 = Φ5e−iωp2t. Hence, the equations of motion for the matter fields are given by

(22)iℏ∂Φ1∂t=−ℏ22m∇2Φ1+V1(r)Φ1+(U11|Φ1|2+U12|Φ2|2+U13|Φ3|2)Φ1+ℏΩp1*Ψ4+ℏΩp2*Φ5

(23)iℏ∂Φ2∂t=(ϵ12−ℏ22m∇2)Φ2+V2(r)Φ2+(U21|Φ1|2+U22|Φ2|2+U32|Φ3|2)Φ1+ℏΩc1*Φ4

(24)iℏ∂Φ3∂t=(ϵ13−ℏ22m∇2)Φ3+V3(r)Φ3+(U31|Φ1|2+U32|Φ2|2+U33|Φ3|2)Φ1+ℏΩc2* Φ5

(25)iℏ∂Φ4∂t=(ϵ14−ℏ22m∇2)Φ4+V4(r)Φ4+ℏΩc1Φ2+ℏΩp1Φ1

(26)iℏ∂Φ5∂t=(ϵ15−ℏ22m∇2)Φ5+V5(r)Φ5+ℏΩc2Φ3+ℏΩp2 Φ1

where Vi(r)(i = 1, 2, 3, 4, 5) are the external potentials, the scattering length aij characterizes the atom-atom interactions via Uij = 4πℏ2aij/m of which for simplicity we assume the scattering length aij = a0 is constant. ϵ14=ℏ(ω41−ωp1) and ϵ15=ℏ(ω51−ωp2) are energies of single-photon detunings, while ϵ12=ℏ(ω21−ωp1−ωs1) and ϵ13 = ℏ(ω31 − ωp2 − ωs2) are energies of the two-photon detunings. To solve the above equations, we shall consider the dark-state condition, i.e., the atoms are approximately restricted on the dark state of the five-level system:

(27)|ΨD〉=Ωc1Ωc2Ω02|1〉−Ωp1Ωc2Ω02|2〉−Ωc1Ωp2Ω02|3〉

where Ω0=(|Ωc1Ωc2|2+|Ωp1Ωc2|2+|Ωc1Ωp2|2)1/4. Since the dark state excludes excited state, the collisions between two excited states and lower states are safely neglected.

It is noteworthy that here our purpose is a little different from that discussed in the former sections. We shall not calculate the adiabatic dynamics of the dark state, but study the dynamics of the coherently generated states Φ2 and Φ3. However, since the dark state is not the unitary transformation of the three ground states, generally the dynamics of Φ2,3 cannot solely be determined through Eq. (27) even if we can solve the adiabatic motion of the dark state. To solve this problem, we assume that the two-photon detunings ϵ12 and ϵ13 are sufficiently small and the strengths of the probe fields are much smaller than that of the control fields, one arrives at the adiabatic Raman passage relating Φ2 and Φ3 to Φ1 [38] through the Eq. (27). In the first order we find

(28)Φ2=−ξ1 Φ1, Φ3=−ξ2 Φ1

where the ratio coefficients ξ1==−Ωp1Ωc1 and ξ2=−Ωp2Ωc2. This result is also the lowest solution of Eqs. (25) and (26). The subsequent derivation for equations of motion for Φ1, Φ2 and Φ3 straightforward. For example, substituting the above relation into the Eqs. (23) and (24), respectively, yields

(29)Φ4=−(ℏΩc1*)−1{[iℏ∂∂t−(ϵ12−ℏ22m∇2)+V2(r)]ξ1−1 Φ1−(U21|+U22|ξ1|−2|+U32|ξ2|−2|) Φ1|2} Φ1

(30)Φ5=−(ℏΩc2*)−1{[iℏ∂∂t−(ϵ13−ℏ22m∇2)+V3(r)]ξ2−1 Φ1+(U31|+U32|ξ1|−2+U33|ξ2|−2|) Φ1|2} Φ1

Together with the above results, from the Eq. (22) we can obtain the equation of motion for the field Φ1. Similarly, from the Eq. (22) and Eq. (24) [or Eq. (23)], one can derive the relations between fields Φ4,5 and Φ2 (or Φ3), and then substituting them into the Eq. (23) [or Eq. (24)] we can obtain the equation of motion for the field Φ2 (or Φ3). Finally, we find the equations of motion for the matter fields Φ1, Φ2 and Φ3 given by

(31)iℏ∂∂tΦα=12m(iℏ∇+Aα]2Φα+VαeffΦα+U|Φ1|2Φα, α=1,2,3

where we have ignored nonlinear terms involving Φ2 or Φ3 for small |ξj|, the nonlinear interaction strength U = 4πℏ2a0/m and the effective vectors read

(32)A1=ℏΞ1−1(ξ1*∇ξ1+ξ2*∇ξ2)

(33)A2=ℏΞ2−1[1/ξ2*∇(1/ξ2)+ξ1*/ξ2*∇(ξ1/ξ2)]

(34)A3=ℏΞ3−1[1/ξ1*∇(1/ξ1)+ξ2*/ξ1*∇(ξ2/ξ1)]

with Ξ1=1+|ξ1|2+|ξ2|2, Ξ2=1+1/|ξ2|2+|ξ1|2/|ξ2|2 and Ξ3 = 1 + 1/|ξ1|2 + |ξ2|2/|ξ1|2, and the effective trap potentials V1eff = iℏ Ξ1−1[V1+|ξ1|2V2 +|ξ2|2V3 +(2mΞ1)−1|A1|2], V2eff = iℏ Ξ2−1[V2+(ϵ21 + V1)/|ξ2|2 −V3|ξ1|2/|ξ2|2+(2mΞ2)−1|A2|2] and V3eff=iℏ Ξ3−1[V3+(ϵ31+V1)/|ξ1|2−V2|ξ2|2/|ξ1|2+(2mΞ3)−1|A3|2]. One can find that the effective vectors Aα(α = 1, 2, 3) is generally non-Hermitian, which is easily understood by recalling that Φ1,2,3 are not eigenstates while dark state is. The Hermitian contribution is due to the changes in the phase of ξ1,2, while the non-Hermitian part results from the changes of the amplitude of ξ1,2. Denoting dimensionless function ξj = eiRj Ωpj(0)/Ωcj(0)(j = 1,2) with the phases R1=(kp1−kc1)⋅r+lϕ and R2=(kp2−kc2)⋅r+l′ϕ, and under the condition |∇|ξj|2|≪||ξj|2∇Rj|, we can neglect the non-Hermitian part. The effective vectors can then be rewritten as

(35)A1=ℏ Ξ1−1(|ξ1|2∇R1+|ξ2|2∇R2)

(36)A2=−ℏ Ξ2−1(|1/ξ2|2∇R2−|ξ1|2/|ξ2|2∇(R1−R2))

(37)A3=ℏΞ3−1(|1/ξ1|2∇R1−|ξ2|2/|ξ1|2∇(R2−R1))

When |ξ1|2 = |ξ2|2, i.e., the ratio between the Rabi frequencies Ωp1(0) and Ωc1(0) equals that between Ωp2(0) and Ωc2(0), and the photons of two input probe fields have opposite orbital angular momentum, i.e. l = −l′, it is easy to verify A1 = 0 and A2 = −A3 = A =−ℏl∇ϕ. The Eqs. (31) can be recast into

(38)iℏ∂∂t(Φ2Φ3)=12m(iℏ∇+qσ3A)2(Φ2Φ3)+(V2eff00V3eff)⋅(Φ2Φ3)+U|Φ1|2(Φ2Φ3)

where σ3 is the pauli matrix, q = +1, and

(39)iℏ∂∂tΦ1=−12mℏ∇2Φ1+V1eff(r)Φ1

The results (38) and (39) can be interpreted as that the three categories of condensates with effective electric charges q1 = 0 and q2 =−q3 = q = +1, respectively, interact with an effective U (1) gauge field A. In other words, by employing two probe lights that respectively have orbital angular momentum ±lℏ in the ±z direction, we obtain an effective two-flavor (oppositely charged) condensate which has attracted special attention in recent years [59, 60]. Alternatively, if we call Φ2 and Φ3 as (pseudo-)spin up |↑〉 and down |↓〉 state, the above result can be understood that different spin states experience opposite effective gauge fields. For the present purpose, since |ξj|2≪1, the small depletion of atoms in state |1〉 can be neglected, and then Eq. (38) is linearized by putting | Φ1|≈ρ(r) with ρ(r) the total density of the condensate. In this way, the lowest order solution of Eq. (38) is given by

(40)Φ2(r,t)=−Ωp1(0)Ωc1(0)ρ(r)exp[iS2(r,t)]

(41)Φ3(r,t)=−Ωp2(0)Ωc2(0)ρ(r)exp[iS3(r,t)]

where the phases S2(r,t) = q2ℏ∫0rA ⋅ dr′ + S02(r,t) and S3(r,t)=q3ℏ∫0rA⋅dr′+S03(r,t) with S02(r, t) = k¯2⋅r−∫0tdt′{V2eff[r+K¯2(t′−t)]+Uρ[r+K¯2(t′−t)]} and S03(r,t)=k¯3⋅r−∫0tdt′{V3eff [r+K¯3(t′−t)]+Uρ[r+K¯3(t′−t)]}. K¯2=ℏk¯2/m=ℏ(kp1−kc1)/m and K¯3=ℏk¯3/m=ℏ(kp2−kc2)/m are the corresponding recoil velocities. The velocity spread of the two generated BECs can be obtained as vj(r)=ℏ∇rSj(r,t)/m (j=2,3). By a straightforward calculation one can verify that the loop integration of the velocity yields ∮z=0∈Cjvj(r′)⋅dr′=±2πℏl/m (j=2,3), where the sign of right-hand side of the above equation takes + (for j = 2) or − (for j = 3). z = 0∈Cj means that the integration path Cj encircles the z-axis. The above results indicate that the orbital angular momenta of input probe fields are fully transferred into the generated BECs Φ2 and Φ3.

A simple but interesting application of the above results is that if the input probe lights are the components of a superposition of opposite OAM states (vortex qubits): | + l〉 ± | − l〉, we can obtain the macroscopic superposition of vortex-antivortex states for the matter fields through the above coherent transfer technique of vortex states. Creation of a general superposition of the OAM states of light has been studied in Ref. [57], and the created vortex qubits for BECs are supposed to have interesting fundamental and practical applications [58].

5 Spin Hall effect in atoms

Spin hall effect (SHE) has recently attracted much attention since its prediction in solid systems with spin-orbit coupled structures [61−66], with the concomitant creation of spin currents and study of quantized spin hall conductance. The physics of SHE in semiconductors can be understood in the following way: In the presence of spin-orbit coupling, the applied electric field leads to a transverse motion (perpendicular to the electric field) of spins, with the spin-up and spin-down carriers transporting opposite to each other; thus, a spin current is created perpendicular to the electric field. Quantized SHE was predicted in metallic graphene [67, 68], mercury telluride-cadmium telluride semiconductor systems [69] and in semiconductors with a strain gradient structure [70]. In the latter cases, quantum SHE is essentially the phenomenon in which particles in different spin directions experience opposite effective gauge fields formed through spin-orbit couplings, resulting in a non-vanishing quantized spin hall conductance and a vanishing charge hall conductance.

According to the discussion in the former sections, we know the effective gauge field on atoms can be readily generated through atom-light couplings. Properly adjusting the parameters of external laser fields, one can reach the situation that different atomic spin states (angular-momentum states) experience opposite gauge fields, leading to SHE in atomic systems. Such an idea was first proposed in Refs. [50] and [51].

Figure 4 shows the level configuration of an ensemble of cold Fermi atoms interacting with two external light fields. The ground (|g±,±12〉) and excited (|e±,±12〉) states are hyperfine angular momentum states (atomic spins) with their total angular momenta Fg = Fe = 1/2. The laser fields are characterized by the Rabi-frequencies Ω1 = Ω10 exp[i(k1 · r + l1ϑ)] and Ω2 = Ω20 exp[i(k2 · r + l2ϑ)]. Here, the phase ϑ = arctan(y/x). For simplicity, in the following discussion we replace the notations |α±,±12〉  by  |α±〉 (α=e,g). The r-representation atomic wave function is denoted by Φα(r, t). Similar to former discussions, we introduce the slowly-varying amplitudes of atomic wave-functions by (setting ωg± = 0): Ψg± = Φg±, Ψe+ = Φe+(r,t)e−i[k2⋅r−(ωe+−Δ1)t], Ψe− = Φe−(r,t)e−i[k1⋅r−(ωe−−Δ2)t], where ℏωα is the energy of the state |α〉, ∆1 and ∆2 are respectively the detuning of σ+ and σ− light fields. The Hamiltonian of the present system can be written as H = H0 + H1 + H2, where

(42)H0=∑α=e±g±∫d3r Ψα*[−ℏ22m∇2+V(r)] ΨαH1=ℏΔ1∫d3r Ψe+*Se+e+ Ψe++ℏ∫d3r( Ψe+* Ω10eil1 ϑ S1+ Ψg− +h.a.)H2=ℏΔ2∫d3r Ψe−*Se−e− Ψe−+ℏ∫d3r( Ψe−* Ω20eil2 ϑ S2+ Ψg+ +h.a.)

with atomic operators Se±e± = |e±〉〈e±|, S1+ =|e+〉〈g−|,S2+ = |e−〉〈g+|, S1+† = S1− and S2+† = S2−. V(r) is the external trap potential. The collisions (s-wave scattering) between cold Fermi atoms are negligible. The interaction part of the Hamiltonian can be diagonalized with the following local unitary transformation:

(43)U(r)=(U100U2)

with

(43)Uj=(cosθjsinθjeiljϑ(r)−sinθje−iljϑ(r)cosθj), j=1,2

Under this transformation, the four eigenstates of interaction Hamiltonian can be obtained as [|ψ+〉,|ψ−〉]T=U1[|e+〉,|g−〉]T and [|ϕ+〉,|ϕ−〉]T = U2[|e−〉,|g+〉]T. The mixing angles θj are defined according to tan θ1 = Eψ−/Eψ+ and tan θ2 = Eϕ−/Eϕ+, where the eigenvalues of |ψ±〉 and |ϕ±〉 can be calculated by: Eψ± = (Δ1 ±Δ12+4Ω102)/2 and Eϕ±=(Δ2±Δ22+4Ω202)/2.

In order to suppress the spontaneous emission of the excited states, we shall consider the large detuning case, i.e. Δj2≫Ωj02. By calculating all values up to the order of Ωj02/Δj2, one can verify that tan θj = Ωj0 /∆j, and Eψ,ϕ+≫Eψ,ϕ−. According to the Eq. (9), atomic motion may lead to the transitions between ground eigenstates and excited ones. For example, the element of transition between |ψ+〉 and ψ−〉 can be calculated by

(44)τ±=|〈ψ+|∂t|ψ−〉|∼|v¯f⋅∇θ1(r)+12sin2θ1v¯f⋅∇ϑ1(r)|

where v¯f is the fermi velocity of the atomic system. For our purpose we require τ± ≪ |Eψ+ − Eψ−| so that the coupling between ground states and excited states can be neglected. Then, we introduce the adiabatic condition that the population of the higher levels |ψ+〉 and |ϕ+〉 is adiabatically eliminated, say, meanwhile the total system is restricted to the ground eigenstates

(45)|Ψ〉=cosγ|ψ−〉+sinγ|ϕ−〉=cosγ|S↓〉+sinγ|S↑〉

where, to facilitate further discussions, we have put the effective spin states: |S↓〉 = |ψ−〉, |S↑〉 = |ϕ−〉 with their z-component effective spin polarizations Sz↑=ℏ2(cos2θ2−sin 2θ2)≈ℏ/2 and Sz↓=ℏ2(sin2 θ1−cos2 θ1)≈−ℏ/2. The parameter γ describes the possibility of an atom in states |S↓〉 and |S↑〉, and can be determined by the initial condition. It is easy to see that the probability of excited states is much smaller than that of the ground states for |S↑,↓〉 (sin2θj≪cos2θj), therefore the atomic decay can be safely neglected in the present situation.

Under the above adiabatic condition, the local transformation U(r) can lead to a diagonalized SU(2) gauge potential:

(46)ec(A↓00A↑)=iℏ(〈S↓|∇|S↓〉00〈S↑|∇|S↑〉)

where e > 0 is the positive effective charge of an atom and c is the vacuum light speed. Accordingly, the effective (scalar) trap potentials read Vα(r) = V(r)− ℏ|Δj|−1Ωj02−(2m)−1|ℏ〈Sα|∇|Sα〉|2 with j = 1 (for α =↓) and j = 2 (for α =↑). Especially, we have

(47)A↓=−A↑=ℏlce−1Ω02Δ2(xe^y−ye^x)/ρ2

and

(48)Veff(r)=V↑,↓(r)=V(r)−ℏΩ02/Δ−ℏ2l2Ω04(2mΔ4ρ2)

with ρ = x2+y2, when we choose ∆1 = ∆2 = ∆, Ω10 = Ω20 = Ω0 and l1 =−l2 = l, i.e., the angular momenta of the two light fields are opposite in direction. This result is intrinsically interesting: by coupling the atomic spin states to radiation, we find the atomic system can be described as an ensemble of charged particles with opposite spins experiencing opposite magnetic fields but the same electric field. With the help of gauge and trap potentials, we can rewrite the Hamiltonian in the following effective form:

(49)H=∫d3r Ψs↓*[12m(ℏ∂k+iecAk)2] Ψs↓+∫d3r Ψs↑* [12m(ℏ∂k−iecAk)2] Ψs↑+∫d3r(V↓|Ψs↓|2+V↑|Ψs↑|2)

where Ψs↓(r) = cosγ〈r|S↓〉 and Ψs↑(r) = sinγ〈r|S↑〉 are spin wave functions in r-representation.

The spin current in the present system has several important properties. First, it satisfies the conservation law. The spin density in the present system is calculated according to

(50)S(r,t)=Ψs↓*S↓Ψs↓+Ψs↑*S↑Ψs↑

with S↑↓=(Sx↑↓,Sy↑↓,Sz↑↓). On the other hand, the spin current density Jk(r,t)=(Jksx,Jksy,Jksz) is defined by

(51)Jk=−iℏmS↓(Ψs↓*D1kΨs↓−Ψs↓D1k*Ψs↓*)−iℏmS↑(Ψs↑*D2kΨs↑−Ψs↑D2k*Ψs↑*)

where D1k=∂k+iecAk and D2k=∂k−iecAk are the covariant derivative operators. By a straightforward calculation we can verify the following continuity equation:

(52)∂tS(r,t)+∂kJk=Akσze^z×Jk(r,t)

where σz is the pauli matrix. It is easy to see for the sz-component spin current, that the right hand side of Eq. (52) equals zero. Thus, the spin current Jksz is conserved. Note that there is no spin-orbit coupling in the present atomic system and that it can be verified that the orbit-angular momentum current is also conserved. These results confirm the conservation law for sz-component of total angular momentum current of atoms. Second, the spin current in the present system may exhibit interesting topological properties. For convenience, we denote

(53)Ψsα=2mηζα, α=↑,↓

where the complex ζα=|ζα|e−iφα with |ζ↓|2+|ζ↑|2=1. The modulus η is related to the total atomic density which is assumed to be constant in our case. Then the sz-component of Eq. (51) can be recast into

(54)Jksz=−iℏ2η2(ζ↓∂kζ↓*−ζ↓*∂kζ↓+ζ↑*∂kζ↑−ζ↑∂kζ↑*)    −2ℏ2η2ecAk=ℏ2η2[∂k(φ1−φ2)−(|ζ↓|2−|ζ↑|2)∂k(φ1+φ2)]    −2ℏ2η2ecAk

Furthermore, we introduce the unit vector field by λ = (ζ¯,σζ), where ζ=(ζ↓,ζ↑*)T and σ = (σx, σy, σz). It then follows that λ1=ζ↓*ζ↑*+ζ↓ζ↑, λ2 = i(ζ↓ζ↑ − ζ↓*ζ↑*) and λ3=|ζ↓|2−|ζ↑|2. Based on these variables we can finally find the following result:

(55)(∇×Jsz)m=−2ℏ2η2ecBm−12ℏ2η2ϵmklλ⋅(∂kλ×∂lλ)

The contribution λ·(∂kλ × ∂lλ) indicates a topological term in the spin current induced by optical fields. Note each value of λ represents a point in the two-dimensional sphere S2. The variation of λ depends on the relative density of the two spin components γ(r) and the sum of the phase spreadings φ↑(r) + φ↓(r). It is easy to verify that λ can cover the entire surface S2 for the parameter distributions in the interaction region: φ1 + φ2: 0→2n1π and γ: 0→n2π/2 with integers n1,n2⩾1. We then obtain a map between the unit vector field λ and the spatial vectors F: λ→r/r so that the closed-surface integral

(55)∮s(∇×Jsz)⋅dS∼∮sdsmϵmklrr⋅(∂krr×∂lrr)∼4πn

where n is the winding number. In physics, such mapping degree corresponds to the formation of a local inhomogeneity in the densities of the spin-up and spin-down atoms. The Hamiltonian (49) can also be understood as a system with two-flavor oppositely charged particles interacting with one external effective magnetic field. Such model has a wide range of application in, e.g. two-band superconductivity [73, 74], etc. For instance, under certain conditions liquid metallic hydrogen might allow for the coexistence of superconductivity with both electronic and protonic Cooper pairs [75]. Faddeev et al. have discovered a series of nontrivial topological properties in these systems [59, 60]. Again, based on our technique, we develop an optical way to realize a two-flavor artificially charged system, which may allow for a deeper understanding of the basic physical mechanisms in cold atomic systems.

For practical application, an important goal is to create a pure spin current injection, i.e., there is no accompanying massive current. For this we use two columnar spreading light fields that [43, 44] Ω01(r) = Ω02(r) = fρ with f > 0. Furthermore, we set the potential V(r) = 12ν(ρ + x0e^x)2 with the coefficient ν=(1+ℏl2f22mΔ3)2ℏf2Δ, say, we use a two-dimensional harmonic potential centered at ρ=−x0e^x [76]. Then we reach a set of uniform magnetic field

(56)B↓(−B↑)=ℏlcef2Δ2e^z

and electric fields

(57)E=−∇Veff(r)=−(1+ℏl2f24mΔ3)2ℏf2x0eΔe^x

respectively in z(−z) and x directions. Atoms in different spin states |Sα〉 experience the opposite magnetic fields Bα but the same electric field E. This may lead to a Landau level structure for each spin orientation. Together with the applied in-plane electric field, one can obtain a pure spin current in the y direction, while the massive current is zero. To exactly calculate the spin currents, we need to calculate the eigenstates of the present system. The Hamiltonian for a single atom in state |Sα〉 can be written as:

(58)Hα=H0α+H′, α=↓,↑H′=−eExH0α=ℏ2eB2mc(Rα2+Pα2)+12mpz2

with R↑↓ = (ceB)1/2(px−ecAx↑↓),P↑↓ = (ceB)1/2(py−ecAy↑↓) and B = |B↑,↓|. One can verify that [Rα,Pβ] = iℏδαβ, so the eigenfunction of H0α is Hermite polynomial, written as μnkα(R) with the Landau level Enk,α = (n+1/2)ℏω+ℏk2/2m and ω = eB/mc. In the weak field case, the spin/massive current carried by an atom can be calculated to the first-order correction with perturbation theory on the state |μnkα〉 (linear response)

(59)(jsz,my)nk,α=〈μnkα|jsz,my|μnkα〉+(∑n′α′〈μn′kα′|H′|μnkα〉〈μnkα|jsz,my|μn′kα′〉En,α−En′,α′+h.a.)

where the spin current operator is

(60)(jszy)α=ℏ2(Szαvyα+vyαSzα)

with vyα=[y,Hα]/ih=(eB/m2c)1/2Pα and the massive current operator jm = mvy. The two terms in the right hand side of the above equation respectively refer to the zeroth and first-order correction. It is easy to see that 〈μnkα|jsz,my|μn′kα′〉 = 0 when n′≠n±1, thus only the terms with n′ = n ± 1 contribute to the above equation.

If the space-spreading lengths of the atoms in x and z directions are Lx and Lz, respectively, the average current density for the total system is given by

(61)Jsz,my=1LxLz∫dE[(jsz,m(0))nk,α+(jsz,m(1))nk,α]f(E)

with f (E) the Fermi distribution function. For 6Li atoms we consider the initial condition that sin2 γ = cos2 γ = 1/2, i.e., the atoms have the equal possibility in state |S↓〉 and |S↑〉, which is familiar in optical traps [77]. Note that under the present definitions the perturbation part can be rewritten as H′=iℏE(ecB)1/2∂∂R. Substituting this result into Eqs. (60) and (61) we get

(62)Jszy=na(ℏ+ℏ2l2f24mΔ3)Δx0l

where na = 2mη2 is the density of atoms, whereas the massive current Jm = 0. In fact, under the present interaction of external effective electric and magnetic fields, the atoms with opposite velocities in y direction have opposite spin polarizations (see Fig. 5). Thus, the massive current vanishes whereas a pure spin current is obtained. This result allows us to create conserved spin currents without using atomic beams.

To observe SHE in present cold atomic systems, a spin-sensitive measurement [78] can be used. After the spin current is created, the spin-up and spin-down atoms will respectively accumulate in opposite sides along the y direction of the atom chip. Experimentally, one can detect such spatially separated spin accumulation via, e.g. fluorescence measurement. For 6Li atoms, one could perform resonant Raman transitions from the accumulated spin state Sz = −1/2 to 22P1/2(F = 3/2, m =−3/2) and from Sz = 1/2 to 22P1/2(F = 3/2, m = 3/2) and then observe fluorescence. As long as the spin accumulations are separated to, e.g., larger than 5−10 microns, the two separated images can be resolved in the experiment.

Finally, we can numerically check the adiabatic condition in the present system. The typical values of the parameters can be set ∆~107s−1, l < 104, f = 107−8(s·m)−1, x0≈0.2 mm. The velocity then satisfies v¯ < 1.0 m/s and τ±/|Eψ+ − Eψ−| < 10−3 ≪ 1, which guarantees the validity of the adiabatic condition. Furthermore, if we employ an atomic system with the atomic density na≈1.0 × 1010cm−3, one can find the spin current Jszy ≈1.322 × 10−5eV/cm2. On the other hand, practically the light fields have a finite cross section Sxy, whose effect is ignored in the calculation of spin currents. For our purpose, this effect can be neglected when lf2Sxy/Δ2≫1, which means the effective magnetic flux induced by the light fields can support an enough large number of quantum states for each Landau level. Since the decoherence rate of atomic spin currents is generally much smaller than that of the counterparts in semiconductors, the created atomic spin currents could be applicable in quantum information devices.

6 Discussion and conclusions

Generation of adiabatic gauge field in the cold atomic system is a rapidly developing research field in recent years. The adiabatic gauge field in atomic systems, which leads to effective spin-orbit couplings in atomic motion, can result in very rich physical features. Compared with the solid system, where the spin-orbit coupling is originated from Dirac equation, the effective spin-orbit coupling in atomic systems is created via atom-light coupling, and has more freedom in controllability, and thus attracts wide attention. Besides the results discussed in this work, several interesting applications of the adiabatic gauge field in cold atoms have been investigated. For example, By extending the atomic SHE from fermi systems to bosonic systems, the fractional spin Hall effect (FSHE) can be studied [79]. Generalized Stern-Gerlach effect is studied by extending the result in three-level Λ-type atomic systems to ∆-type systems [80]. In the four-level tripod atomic system, the effective Rashba and linear Dresselhaus model is obtained by properly adjusting the atom-light interactions [81]. Combining the approach of creating non-Abelian gauge field with optical lattice, many interesting results can be obtained, e.g. realization of the non-Abelian Aharonov-Bohm effect, non-Abelian interferometry and simulating lattice gauge dynamics [82].

In summary, we have reviewed the general theory of generating adiabatic gauge field in quantum systems and in particular, we have discussed how to generate effective spin-orbit couplings in atomic systems by coupling atoms to external optical fields with OAM. Two novel applications of the adiabatic gauge field in atoms have been studied. First, we introduced the scheme for the creation of macroscopic superposition of vortex-antivortex states from a five-level M-type atomic system, and then we showed the realization of the spin Hall effect in fermi atomic system. Further investigations on the applications of the adiabatic gauge field in atoms and experimental demonstration of the theoretically predicted results will be the next focus in this intriguing topic.

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