Continuous aramid fiber/unsaturated polyester resin composites with excellent interfacial and mechanical properties

Yan Zhang , Yinchun Hu , Kexin Chen , Zhibin Jin , Qi Lei , Yongcun Li , Chuanbo Cong , Qiong Zhou , Yingying Wang

Front. Mater. Sci. ›› 2025, Vol. 19 ›› Issue (2) : 250728

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Front. Mater. Sci. ›› 2025, Vol. 19 ›› Issue (2) : 250728 DOI: 10.1007/s11706-025-0728-x
RESEARCH ARTICLE

Continuous aramid fiber/unsaturated polyester resin composites with excellent interfacial and mechanical properties

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Abstract

The surface microstructure of continuous aramid fibers (AFs) is significant for AF/unsaturated polyester (UP) resin composites. The chemical modification of the AF surface is the key point to enhance mechanical properties of AF/UP composites. In this study, the polyethyleneimine (PEI)‒polydopamine (PDA) coating was formed on the continuous AF surface via a one-step process. Morphologies and functional groups of PEI‒PDA-coated AFs were studied. It was revealed that the interfacial bonding strength between PEI–PDA-AFs and the UP matrix was increased by 82.47% due to formation of the chemical bonding between amino groups on PEI and hydroxyl groups on UP. The tensile strength of the PEI–PDA-AF/UP composite reached 959.07 MPa, increased by 34.19% compared with that before modification. This study presents a simple and efficient method to prepare high-strength continuous AF/UP composites which could be used in engineering fields of deep-sea pipeline, aerospace, construction, military, safety, sports equipment, etc.

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continuous aramid fiber / unsaturated polyester resin / polymer composite / interfacial shear strength / interlaminar shear strength

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Yan Zhang,Yinchun Hu,Kexin Chen,Zhibin Jin,Qi Lei,Yongcun Li,Chuanbo Cong,Qiong Zhou,Yingying Wang. Continuous aramid fiber/unsaturated polyester resin composites with excellent interfacial and mechanical properties. Front. Mater. Sci., 2025, 19(2): 250728 DOI:10.1007/s11706-025-0728-x

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