Laser-induced graphene-coated wearable smart textile electrodes for biopotentials signal monitoring
C. M. Vidhya, Yogita Maithani, Sakshi Kapoor, J. P. Singh
Laser-induced graphene-coated wearable smart textile electrodes for biopotentials signal monitoring
This paper describes how to produce a wearable dry electrode at a reasonable cost and how to use it for the monitoring of biopotentials in electrocardiography. Smart textiles in wearable technologies have made a great advancement in the health care management and living standards of humans. Graphene was manufactured using the low-cost single-step process, laser ablation of polyimide, a commercial polymer. Graphene dispersions were made using solvent isopropyl alcohol which has low boiling point, nontoxicity, and environmental friendliness. After successive coating of the graphene dispersion on the cotton fabric to make it conductive, the sheet resistance of the resulting fabric dropped to 3% of its initial value. The laser-induced graphene (LIG) cotton dry electrodes thus manufactured are comparable to Ag/AgCl wet electrodes in terms of the skin-to-electrode impedance, measuring between 78.0 and 7.2 kΩ for the frequency between 40 Hz and 1 kHz. The LIG cotton electrode displayed a signal-to-noise ratio of 20.17 dB. Due to its comfort, simplicity, and good performance over a longer period of time, the textile electrode appears suited for medical applications.
biopotential / electrocardiogram / electromyogram / flexible electrode / textile / porous graphene
[1] |
World Health Organization. The top 10 causes of death. 9 December 2020 (accessed 2023-08-07 from the official website of WHO)
|
[2] |
Debon R, Coleone J D, Bellei E A,
CrossRef
Google scholar
|
[3] |
Webster J G, ed
|
[4] |
Sörnmo L, Laguna P. Bioelectrical Signal Processing in Cardiac and Neurological Applications. Burlington MA, USA: Elsevier Academic Press, 2005
|
[5] |
Wang M H, Chen K C, Hung M H,
CrossRef
Google scholar
|
[6] |
Button V L D S N. Electrodes for biopotential recording and tissue stimulation. In: Principles of Measurement and Transduction of Biomedical Variables. Elsevier, 2015, 25–76
|
[7] |
Tam H W, Webster J G . Minimizing electrode motion artifact by skin abrasion.IEEE Transactions on Biomedical Engineering, 1977, 24(2): 134–139
CrossRef
Google scholar
|
[8] |
Liu C M, Chang S L, Yeh Y H,
CrossRef
Google scholar
|
[9] |
Zheng S, Li W, Ren Y,
CrossRef
Google scholar
|
[10] |
Liang X, Zhu M, Li H,
CrossRef
Google scholar
|
[11] |
Wang Y, Wang J, Cao S,
CrossRef
Google scholar
|
[12] |
Li Q, Chen G, Cui Y,
CrossRef
Google scholar
|
[13] |
Yapici M K, Alkhidir T, Samad Y A,
CrossRef
Google scholar
|
[14] |
Zhou Y, Ding X, Zhang J,
CrossRef
Google scholar
|
[15] |
Li M, Xiong W, Li Y . Wearable measurement of ECG signals based on smart clothing.International Journal of Telemedicine and Applications, 2020, 2020: 6329360
CrossRef
Google scholar
|
[16] |
Pani D, Achilli A, Spanu A,
CrossRef
Google scholar
|
[17] |
Karim N, Afroj S, Malandraki A,
CrossRef
Google scholar
|
[18] |
Arquilla K, Webb A K, Anderson A P . Textile electrocardiogram (ECG) electrodes for wearable health monitoring.Sensors, 2020, 20(4): 1013
CrossRef
Google scholar
|
[19] |
Rattfält L, Lindén M, Hult P,
CrossRef
Google scholar
|
[20] |
Maithani Y, Singh A, Mehta B R,
CrossRef
Google scholar
|
[21] |
Gao D, Zhu J, Ye M,
CrossRef
Google scholar
|
[22] |
Arvidsson R, Boholm M, Johansson M,
CrossRef
Google scholar
|
[23] |
Shathi M A, Chen M, Khoso N A,
CrossRef
Google scholar
|
[24] |
Xu X, Luo M, He P,
CrossRef
Google scholar
|
[25] |
Maithani Y, Mehta B R, Singh J P . Implementation of hybrid Ag nanorods embedded RGO–PDMS conductive material for flexible and dry electrocardiography sensor.Materials Letters-X, 2022, 15: 100152
CrossRef
Google scholar
|
[26] |
Lin J, Peng Z, Liu Y,
CrossRef
Google scholar
|
[27] |
Vlassiouk I, Fulvio P, Meyer H,
CrossRef
Google scholar
|
[28] |
Camara N, Rius G, Huntzinger J R,
CrossRef
Google scholar
|
[29] |
Allen M J, Tung V C, Kaner R B . Honeycomb carbon: a review of graphene.Chemical Reviews, 2010, 110(1): 132–145
CrossRef
Google scholar
|
[30] |
Novoselov K S, Geim A K, Morozov S V,
CrossRef
Google scholar
|
[31] |
Yapici M K, Alkhidir T E . Intelligent medical garments with graphene-functionalized smart-cloth ECG sensors.Sensors, 2017, 17(4): 875
CrossRef
Google scholar
|
[32] |
Shathi M A, Chen M, Khoso N A,
CrossRef
Google scholar
|
[33] |
Ozturk O, Golparvar A, Acar G,
CrossRef
Google scholar
|
[34] |
Celik N, Manivannan N, Strudwick A,
CrossRef
Google scholar
|
[35] |
Lou C, Li R, Li Z,
CrossRef
Google scholar
|
[36] |
Lam C L, Saleh S M, Yudin M B M, ,
|
[37] |
Li G . Direct laser writing of graphene electrodes.Journal of Applied Physics, 2020, 127(1): 010901
CrossRef
Google scholar
|
[38] |
Tehrani F, Beltrán-Gastélum M, Sheth K,
CrossRef
Google scholar
|
[39] |
Nilghaz A, Wicaksono D H B, Gustiono D,
CrossRef
Google scholar
|
[40] |
Rousselle M A, Price J B, Thomasson J A,
CrossRef
Google scholar
|
[41] |
Nguyen V T, Le H D, Nguyen V C,
CrossRef
Google scholar
|
[42] |
Kapoor S, Jha A, Ahmad H,
CrossRef
Google scholar
|
[43] |
Wu J B, Lin M L, Cong X,
CrossRef
Google scholar
|
[44] |
Santra S, Hu G, Howe R C T,
CrossRef
Google scholar
|
[45] |
Tran T S, Dutta N K, Choudhury N R . Graphene inks for printed flexible electronics: graphene dispersions, ink formulations, printing techniques and applications.Advances in Colloid and Interface Science, 2018, 261: 41–61
CrossRef
Google scholar
|
[46] |
O’Neill A, Khan U, Nirmalraj P N,
CrossRef
Google scholar
|
[47] |
Polyakova E Y, Rim K T, Eom D,
CrossRef
Google scholar
|
[48] |
Skaltsas T, Ke X, Bittencourt C,
CrossRef
Google scholar
|
[49] |
Perumal S, Atchudan R, Cheong I W . Recent studies on dispersion of graphene–polymer composites.Polymers, 2021, 13(14): 2375
CrossRef
Google scholar
|
[50] |
Torrisi F, Hasan T, Wu W,
CrossRef
Google scholar
|
[51] |
Wajid A S, Das S, Irin F,
CrossRef
Google scholar
|
[52] |
Htwe Y Z N, Mariatti M . Surfactant-assisted water-based graphene conductive inks for flexible electronic applications.Journal of the Taiwan Institute of Chemical Engineers, 2021, 125: 402–412
CrossRef
Google scholar
|
[53] |
Konios D, Stylianakis M M, Stratakis E,
CrossRef
Google scholar
|
[54] |
Soltani-kordshuli F, Zabihi F, Eslamian M . Graphene-doped PEDOT:PSS nanocomposite thin films fabricated by conventional and substrate vibration-assisted spray coating (SVASC).Engineering Science and Technology: An International Journal, 2016, 19(3): 1216–1223
CrossRef
Google scholar
|
[55] |
Saini P, Sharma B, Singh M,
CrossRef
Google scholar
|
[56] |
Zahid M, Papadopoulou E L, Athanassiou A,
CrossRef
Google scholar
|
[57] |
Park C, Yoo D, Im S,
CrossRef
Google scholar
|
[58] |
Lin Y J, Ni W S, Lee J Y . Effect of incorporation of ethylene glycol into PEDOT:PSS on electron phonon coupling and conductivity.Journal of Applied Physics, 2015, 117(21): 215501
CrossRef
Google scholar
|
[59] |
Wei Q, Mukaida M, Naitoh Y,
CrossRef
Google scholar
|
[60] |
Barani H, Miri A, Sheibani H . Comparative study of electrically conductive cotton fabric prepared through the in situ synthesis of different conductive materials.Cellulose, 2021, 28(10): 6629–6649
CrossRef
Google scholar
|
[61] |
Ali B, Bidsorkhi H C, D’Aloia A G,
CrossRef
Google scholar
|
[62] |
Ali B, Bidsorkhi H C, D’Aloia A G, ,
|
[63] |
Arunkumar K, Raghu R, LetaTesfaye J,
CrossRef
Google scholar
|
[64] |
Ghosh S, Ganguly S, Das P,
CrossRef
Google scholar
|
[65] |
Alimohammadi F, Gashti M P, Mozaffari A . Polyvinylpyrrolidone/carbon nanotube/cotton functional nanocomposite: preparation and characterization of properties.Fibers and Polymers, 2018, 19(9): 1940–1947
CrossRef
Google scholar
|
[66] |
Xie R, Li Q, Teng L,
CrossRef
Google scholar
|
[67] |
Beckmann L, Neuhaus C, Medrano G,
CrossRef
Google scholar
|
[68] |
Bora D J, Dasgupta R . Estimation of skin impedance models with experimental data and a proposed model for human skin impedance.IET Systems Biology, 2020, 14(5): 230–240
CrossRef
Google scholar
|
[69] |
Murphy B B, Scheid B H, Hendricks Q,
CrossRef
Google scholar
|
[70] |
Takeshita T, Yoshida M, Takei Y,
CrossRef
Google scholar
|
[71] |
Mason J W, Ramseth D J, Chanter D O,
CrossRef
Google scholar
|
[72] |
Krummen D E, Feld G K, Narayan S M . Diagnostic accuracy of irregularly irregular RR intervals in separating atrial fibrillation from atrial flutter.The American Journal of Cardiology, 2006, 98(2): 209–214
CrossRef
Google scholar
|
[73] |
Myers A C, Huang H, Zhu Y . Wearable silver nanowire dry electrodes for electrophysiological sensing.RSC Advances, 2015, 5(15): 11627–11632
CrossRef
Google scholar
|
[74] |
Welch P . The use of fast Fourier transform for the estimation of power spectra: a method based on time averaging over short, modified periodograms.IEEE Transactions on Audio and Electroacoustics, 1967, 15(2): 70–73
CrossRef
Google scholar
|
/
〈 | 〉 |