Influence of precursor concentration on printable mesoscopic perovskite solar cells

Shuangquan JIANG , Yusong SHENG , Yue HU , Yaoguang RONG , Anyi MEI , Hongwei HAN

Front. Optoelectron. ›› 2020, Vol. 13 ›› Issue (3) : 256 -264.

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Front. Optoelectron. ›› 2020, Vol. 13 ›› Issue (3) : 256 -264. DOI: 10.1007/s12200-020-1013-3
RESEARCH ARTICLE
RESEARCH ARTICLE

Influence of precursor concentration on printable mesoscopic perovskite solar cells

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Abstract

Over the last decade, the power conversion efficiency of hybrid organic–inorganic perovskite solar cells (PSCs) has increased dramatically from 3.8% to 25.2%. This rapid progress has been possible due to the accurate control of the morphology and crystallinity of solution-processed perovskites, which are significantly affected by the concentration of the precursor used. This study explores the influence of precursor concentrations on the performance of printable hole-conductor-free mesoscopic PSCs via a simple one-step drop-coating method. The results reveal that lower concentrations lead to larger grains with inferior pore filling, while higher concentrations result in smaller grains with improved pore filling. Among concentrations ranging from 0.24–1.20 M, devices based on a moderate strength of 0.70 M were confirmed to exhibit the best efficiency at 16.32%.

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printable perovskite solar cell (PSC) / precursor concentration / crystallization / morphology

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Shuangquan JIANG, Yusong SHENG, Yue HU, Yaoguang RONG, Anyi MEI, Hongwei HAN. Influence of precursor concentration on printable mesoscopic perovskite solar cells. Front. Optoelectron., 2020, 13(3): 256-264 DOI:10.1007/s12200-020-1013-3

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