Adaptive Printing of Conductive Microfibers for Seamless Functional Enhancement Across Diverse Surfaces and Shapes

Stanley Gong Sheng Ka , Wenyu Wang , Henry Giddens , Zhuo Chen , Ahsan Noor Khan , Yuan Shui , Andre Sarker Andy , Shuyu Lyu , Tawfique Hasan , Yang Hao , Yan Yan Shery Huang

Advanced Fiber Materials ›› 2025, Vol. 7 ›› Issue (4) : 1274 -1289.

PDF
Advanced Fiber Materials ›› 2025, Vol. 7 ›› Issue (4) : 1274 -1289. DOI: 10.1007/s42765-025-00561-6
Research Article
research-article

Adaptive Printing of Conductive Microfibers for Seamless Functional Enhancement Across Diverse Surfaces and Shapes

Author information +
History +
PDF

Abstract

Developing methods to non-destructively deposit conductive materials onto existing objects can enhance their functionalities on-demand. However, designing and creating such structures to accommodate diverse shapes and surface textures of pre-fabricated objects remains challenging. We report an on-demand printing strategy for creating substrate-less, conducting microfiber patterns that can be adaptively deposited onto a wide range of objects, including daily-use stationery, tools, smartwatches, and unconventional materials like porous graphene aerogels. Solution-drawn microfibers are directly deposited onto the object in a semi-wet state upon synthesis, enabling seamless fiber-object integration in a single step. The design and format of the microfiber patterns can be tuned on-demand to adapt to the shapes and surface textures of target objects, ensuring compatibility with user-specific applications. These air-permissive, highly transparent layers minimally obstruct the original appearance and functions of the objects while equipping them with additional sensing, energy conversion, and electronic connectivity capabilities.

Keywords

Fiber / Sensor / Functionalization / Transient electronics / Customization / Fiber-of-things (FoT)

Cite this article

Download citation ▾
Stanley Gong Sheng Ka, Wenyu Wang, Henry Giddens, Zhuo Chen, Ahsan Noor Khan, Yuan Shui, Andre Sarker Andy, Shuyu Lyu, Tawfique Hasan, Yang Hao, Yan Yan Shery Huang. Adaptive Printing of Conductive Microfibers for Seamless Functional Enhancement Across Diverse Surfaces and Shapes. Advanced Fiber Materials, 2025, 7(4): 1274-1289 DOI:10.1007/s42765-025-00561-6

登录浏览全文

4963

注册一个新账户 忘记密码

References

[1]

TianG, ShiY, DengJ, YuW, YangL, LuY, ZhaoY, JinX, KeQ, HuangC. Low-cost, scalable fabrication of all-fabric piezoresistive sensors via binder-free, in-situ welding of carbon nanotubes on bicomponent nonwovens. Adv Fiber Mater, 2024, 6: 120-132

[2]

WuG, DuH, ChaYL, LeeD, KimW, Feyzbar-Khalkhali-NejadF, OhT-S, ZhangX, KimD-J. A wearable mask sensor based on polyaniline/CNT nanocomposites for monitoring ammonia gas and human breathing. Sens Actuators B Chem, 2023, 375132858

[3]

LiuF, DeswalS, ChristouA, SandamirskayaY, KaboliM, DahiyaR. Neuro-inspired electronic skin for robots. Sci Robot, 2022, 7eab17344

[4]

ZhangW, XiY, WangE, QuX, YangY, FanY, ShiB, LiZ. Self-powered force sensors for multidimensional tactile sensing. ACS Appl Mater Interfaces, 2022, 14: 20122-20131

[5]

CunhaI, MartinsJ, GasparD, BahubalindruniPG, FortunatoE, MartinsR, PereiraL. Healable cellulose iontronic hydrogel stickers for sustainable electronics on paper. Adv Elect Mater, 2021, 72001166

[6]

MekidS, ChenaouaK. IoT-enabled smart mask for monitoring body parameters and location through cloud. Internet Things, 2023, 22100794

[7]

YogeswaranN, DangW, NavarajWT, ShakthivelD, KhanS, PolatEO, GuptaS, HeidariH, KaboliM, LorenzelliL, ChengG, DahiyaR. New materials and advances in making electronic skin for interactive robots. Adv Robot, 2015, 29: 1359-1373

[8]

GohGL, ZhangH, ChongTH, YeongWY. 3D printing of multilayered and multimaterial electronics: a review. Adv Electron Mater, 2021, 72100445

[9]

XuY, WuX, GuoX, KongB, ZhangM, QianX, MiS, SunW. The boom in 3D-printed sensor technology. Sensors, 2017, 171166

[10]

YangX, ShangW, LuH, LiuY, YangL, TanR, WuX, ShenY. An agglutinate magnetic spray transforms inanimate objects into millirobots for biomedical applications. Sci Robot, 2020, 5eabc8191

[11]

PanY, WangW, ShuiY, MurphyJF, HuangYYS. Fabrication, sustainability, and key performance indicators of bioelectronics via fiber building blocks. Cell Rep Phys Sci, 2024, 5101930

[12]

WuG, WuX, ZhuX, XuJ, BaoN. Two-dimensional hybrid nanosheet-based supercapacitors: from building block architecture, fiber assembly, and fabric construction to wearable applications. ACS Nano, 2022, 16: 10130-10155

[13]

SunF, JiangH, WangH, ZhongY, XuY, XingY, YuM, FengL-W, TangZ, LiuJ, SunH, WangH, WangG, ZhuM. Soft fiber electronics based on semiconducting polymer. Chem Rev, 2023, 123: 4693-4763

[14]

XueE, LiuL, WuW, WangB. Soft fiber/textile actuators: from design strategies to diverse applications. ACS Nano, 2024, 18: 89-118

[15]

ChenC, FengJ, LiJ, GuoY, ShiX, PengH. Functional fiber materials to smart fiber devices. Chem Rev, 2023, 123: 613-662

[16]

ZhangX, LuW, ZhouG, LiQ. Understanding the mechanical and conductive properties of carbon nanotube fibers for smart electronics. Adv Mater, 2020, 321902028

[17]

DuY, ZhangX, WangJ, LiuZ, ZhangK, JiX, YouY, ZhangX. Reaction-spun transparent silica aerogel fibers. ACS Nano, 2020, 14: 11919-11928

[18]

KaragiorgisX, ShakthivelD, KhandelwalG, GinesiR, SkabaraPJ, DahiyaR. Highly conductive PEDOT:PSS: Ag nanowire-based nanofibers for transparent flexible electronics. ACS Appl Mater Interfaces, 2024, 16: 19551-19562

[19]

MiyamotoA, LeeS, CoorayNF, LeeS, MoriM, MatsuhisaN, JinH, YodaL, YokotaT, ItohA, SekinoM, KawasakiH, EbiharaT, AmagaiM, SomeyaT. Inflammation-free, gas-permeable, lightweight, stretchable on-skin electronics with nanomeshes. Nat Nanotech, 2017, 12: 907-913

[20]

LeeS, FranklinS, HassaniFA, YokotaT, NayeemMOG, WangY, LeibR, ChengG, FranklinDW, SomeyaT. Nanomesh pressure sensor for monitoring finger manipulation without sensory interference. Science, 2020, 370: 966-970

[21]

KimKK, KimM, PyunK, KimJ, MinJ, KohS, RootSE, KimJ, NguyenB-NT, NishioY, HanS, ChoiJ, KimC-Y, TokJB-H, JoS, KoSH, BaoZ. A substrate-less nanomesh receptor with meta-learning for rapid hand task recognition. Nat Electron., 2022, 6: 64-75

[22]

WangP, LiG, LiuJ, HouZ, MengC, GuoS. Flexible, freestanding, ultrasensitive, and iontronic tactile sensing textile. ACS Appl Electron Mater, 2021, 3: 2195-2202

[23]

WangW, PanY, ShuiY, HasanT, LeiIM, KaSGS, SavinT, Velasco-BosomS, CaoY, McLarenSBP, CaoY, XiongF, MalliarasGG, HuangYYS. Imperceptible augmentation of living systems with organic bioelectronic fibres. Nat Electron, 2024, 7: 586-597

[24]

WalkerSB, LewisJA. Reactive silver inks for patterning high-conductivity features at mild temperatures. J Am Chem Soc, 2012, 134: 1419-1421

[25]

WangW, OuarasK, RutzAL, LiX, GerigkM, NaegeleTE, MalliarasGG, HuangYYS. Inflight fiber printing toward array and 3D optoelectronic and sensing architectures. Sci Adv, 2020, 6eaba0931

[26]

ChenZ, ZhouB, XiaoM, BhowmickT, Karthick KannanP, OcchipintiLG, GardnerJW, HasanT. Real-time, noise and drift resilient formaldehyde sensing at room temperature with aerogel filaments. Sci Adv, 2024, 10eadk6856

[27]

GonzalezG, RoppoloI, PirriCF, ChiapponeA. Current and emerging trends in polymeric 3D printed microfluidic devices. Addit Manuf, 2022, 55102867

[28]

KircherK, ShiX, PatilS, ZhangKM. Cleanroom energy efficiency strategies: modeling and simulation. Energy Build, 2010, 42: 282-289

[29]

ShuaibM, HaleemA, KumarS, JavaidM. Impact of 3D printing on the environment: a literature-based study. Sustain Oper Comput, 2021, 2: 57-63

[30]

DingY, XuW, WangW, FongH, ZhuZ. Scalable and facile preparation of highly stretchable electrospun PEDOT:PSS@PU fibrous nonwovens toward wearable conductive textile applications. ACS Appl Mater Interfaces, 2017, 9: 30014-30023

[31]

HuangY, BaiX, ZhouM, LiaoS, YuZ, WangY, WuH. Large-scale spinning of silver nanofibers as flexible and reliable conductors. Nano Lett, 2016, 16: 5846-5851

[32]

NiittynenJ, AbbelR, MäntysaloM, PerelaerJ, SchubertUS, LupoD. Alternative sintering methods compared to conventional thermal sintering for inkjet printed silver nanoparticle ink. Thin Solid Films, 2014, 556: 452-459

[33]

KimT, KimG, KimH, YoonH-J, KimT, JunY, ShinT-H, KangS, CheonJ, HwangD, MinB, ShimW. Megahertz-wave-transmitting conducting polymer electrode for device-to-device integration. Nat Commun, 2019, 10653

[34]

VolmanV, ZhuY, RajiA-RO, GenorioB, LuW, XiangC, KittrellC, TourJM. Radio-frequency-transparent, electrically conductive graphene nanoribbon thin films as deicing heating layers. ACS Appl Mater Interfaces, 2014, 6: 298-304

[35]

KhanAN, ErmakovA, SukhorukovG, HaoY. Radio frequency controlled wireless drug delivery devices. Appl Phys Rev, 2019, 6041301

[36]

BelloO, ZeadallyS. Intelligent device-to-device communication in the internet of things. IEEE Syst J, 2016, 10: 1172-1182

[37]

Hao Y, Alomainy A, Hall PS, Nechayev YI, Parini CG, Constantinou CC. Antennas and propagation for body centric wireless communications. In: IEEE/ACES international conference on wireless communications and applied computational electromagnetics, 2005. Honolulu, HI: IEEE; 2005. p. 586–9.

[38]

LivingstonJDElectronic properties of engineering materials, 1999, New York. Wiley.

[39]

DongJ, TangX, PengY, FanC, LiL, ZhangC, LaiF, HeG, MaP, WangZ, WeiQ, YanX-P, QianH-L, HuangY, LiuT. Highly permeable and ultrastretchable E-textiles with EGaIn-superlyophilicity for on-skin health monitoring, joule heating, and electromagnetic shielding. Nano Energy, 2023, 108108194

[40]

WangJ, HuQ, HuangJ, LiJ, LuY, LiangT, ShenB, ZhengW, SongW. Multifunctional textiles enabled by simultaneous interaction with infrared and microwave electromagnetic waves. Adv Mat Int, 2022, 92102322

[41]

ChuH, ZhangH, ZhangY, PengR, WangM, HaoY, LaiY. Invisible surfaces enabled by the coalescence of anti-reflection and wavefront controllability in ultrathin metasurfaces. Nat Commun, 2021, 124523

[42]

GillEL, WangW, LiuR, HuangYYS. Additive batch electrospinning patterning of tethered gelatin hydrogel fibres with swelling-induced fibre curling. Addit Manuf, 2020, 36101456

[43]

GillEL, WillisS, GerigkM, CohenP, ZhangD, LiX, HuangYYS. Fabrication of designable and suspended microfibers via low-voltage 3D micropatterning. ACS Appl Mater Interfaces, 2019, 11: 19679-19690

[44]

RobinsonAJ, Pérez-NavaA, AliSC, González-CamposJB, HollowayJL, Cosgriff-HernandezEM. Comparative analysis of fiber alignment methods in electrospinning. Matter, 2021, 4: 821-844

[45]

Davoodi P, Gill EL, Wang W, Shery Huang YY. Advances and innovations in electrospinning technology. In: Biomedical applications of electrospinning and electrospraying. Elsevier; 2021. p. 45–81.

[46]

WangW, StippPN, OuarasK, FathiS, HuangYYS. Broad bandwidth, self-powered acoustic sensor created by dynamic near-field electrospinning of suspended, transparent piezoelectric nanofiber mesh. Small, 2020, 162000581

[47]

PalumboA, VizzaP, CalabreseB, IelpoN. Biopotential signal monitoring systems in rehabilitation: a review. Sensors, 2021, 217172

[48]

PortelliA, NasutoS. Design and development of non-contact bio-potential electrodes for pervasive health monitoring applications. Biosensors, 2017, 72

[49]

YangJC, MunJ, KwonSY, ParkS, BaoZ, ParkS. Electronic skin: recent progress and future prospects for skin-attachable devices for health monitoring, robotics, and prosthetics. Adv Mater, 2019, 311904765

[50]

LiangY, OffenhäusserA, IngebrandtS, MayerD. PEDOT:PSS-based bioelectronic devices for recording and modulation of electrophysiological and biochemical cell signals. Adv Healthc Mater, 2021, 102100061

[51]

RichSI, JiangZ, FukudaK, SomeyaT. Well-rounded devices: the fabrication of electronics on curved surfaces—a review. Mater Horiz, 2021, 8: 1926-1958

[52]

HuangY, WuH, XiaoL, DuanY, ZhuH, BianJ, YeD, YinZ. Assembly and applications of 3D conformal electronics on curvilinear surfaces. Mater Horiz, 2019, 6: 642-683

[53]

RajiA-RO, SaltersS, SamuelELG, ZhuY, VolmanV, TourJM. Functionalized graphene nanoribbon films as a radiofrequency and optically transparent material. ACS Appl Mater Interfaces, 2014, 6: 16661-16668

[54]

HongJ, JungJH, YongS, KimY, ParkJ, LeeSJ, ChoiJ. Radio-frequency transparent carbon nanotube electrothermal film for radome de-icing application. J Mater Res Technol, 2020, 9: 10854-10862

[55]

DuY, XuJ, PaulB, EklundP. Flexible thermoelectric materials and devices. Appl Mater Today, 2018, 12: 366-388

[56]

WanK, LiuY, SantagiulianaG, BarandunG, Taroni JuniorP, GüderF, BastiaansenCW, BaxendaleM, FenwickO, PapageorgiouDG, KrauseS, ZhangH, BilottiE. Self-powered ultrasensitive and highly stretchable temperature–strain sensing composite yarns. Mater Horiz, 2021, 8: 2513-2519

[57]

WangY, YangL, ShiX, ShiX, ChenL, DarguschMS, ZouJ, ChenZ. Flexible thermoelectric materials and generators: challenges and innovations. Adv Mater, 2019, 311807916

[58]

GorgolisG, GaliotisC. Graphene aerogels: a review. 2D Mater., 2017, 4032001

[59]

ZhouB, ChenZ, ChengQ, XiaoM, BaeG, LiangD, HasanT. Controlling surface porosity of graphene-based printed aerogels. npj 2D Mater Appl., 2022, 634

[60]

XuX, LiH, ZhangQ, HuH, ZhaoZ, LiJ, LiJ, QiaoY, GogotsiY. Self-sensing, ultralight, and conductive 3D graphene/iron oxide aerogel elastomer deformable in a magnetic field. ACS Nano, 2015, 9: 3969-3977

[61]

AydemirC, AltayBN, AkyolM. Surface analysis of polymer films for wettability and ink adhesion. Color Res Appl, 2021, 46: 489-499

Funding

European Research Council(ERC-StG)

Engineering and Physical Sciences Research Council(EP/R035393/1)

IET AF Harvey Research Prize

the Royal Academy of Engineering

RIGHTS & PERMISSIONS

The Author(s)

AI Summary AI Mindmap
PDF

154

Accesses

0

Citation

Detail

Sections
Recommended

AI思维导图

/