Towards the optimal design of optically clear adhesives for flexible display

Youngjoo Park , Junkyu Kim , Daewhan Kim , Seokju Lee , Daihyun Hwang , Min Sang Kwon

Soft Science ›› 2024, Vol. 4 ›› Issue (3) : 28

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Soft Science ›› 2024, Vol. 4 ›› Issue (3) :28 DOI: 10.20517/ss.2024.22
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Towards the optimal design of optically clear adhesives for flexible display

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Abstract

As device form factors evolve towards increased complexity and flexibility, the role of adhesives within the display module stack becomes increasingly crucial. These adhesives are essential for bonding functional layers with minimal thickness while mitigating stress during the dynamic behavior of flexible devices. This paper offers a comprehensive overview of the essential properties of adhesives - such as adhesion, viscoelasticity, optical characteristics, and environmental reliability - necessary for the stable operation of flexible display devices across diverse form factors and environments. In particular, it provides an in-depth look at ongoing research in simulation, material selection, polymer network control, and the integration of new functionalities to achieve optimal performance. Furthermore, this paper discusses extensive research outcomes addressing the growing demand for sustainable solutions. Building on this knowledge, we highlight the future direction of adhesives for flexible displays.

Keywords

Flexible display / flexible adhesives / low modulus / viscoelastic property

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Youngjoo Park, Junkyu Kim, Daewhan Kim, Seokju Lee, Daihyun Hwang, Min Sang Kwon. Towards the optimal design of optically clear adhesives for flexible display. Soft Science, 2024, 4(3): 28 DOI:10.20517/ss.2024.22

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References

[1]

Koo JH,Shim HJ,Kim D.Flexible and stretchable smart display: materials, fabrication, device design, and system integration.Adv Funct Mater2018;28:1801834

[2]

Park H,Lee G,Lee DW.Tailoring pressure sensitive adhesives with H6XDI-PEG diacrylate for strong adhesive strength and rapid strain recovery.Adv Funct Mater2023;33:2305750

[3]

Kim J,Yang J.Ultrathin quantum dot display integrated with wearable electronics.Adv Mater2017;29:1700217

[4]

Jeong YC.P-212: Late-News Poster: flexible cover window for foldable display.Symp Digest Tech Papers2018;49:1921-4

[5]

[SID 2021 Keynote speech] “The metaverse and the great future of display”. Available from: https://www.samsungdisplay.com/eng/media/movie/detail/movie210520.jsp. [Last accessed on 30 Jul 2024]

[6]

Kim DW,Lee G.Fabrication of practical deformable displays: advances and challenges.Light Sci Appl2023;12:61 PMCID:PMC9984414

[7]

Bi S,Han X.Recent progress in printing flexible electronics: a review.Sci China Technol Sci2023;67:2363-86

[8]

Benedek I.Applications of pressure-sensitive products. 1st ed. Boca Raton: CRC Press; 2008.

[9]

Satas D. Handbook of pressure sensitive adhesive technology. New York, NY: Springer; 1989. Available from: https://link.springer.com/book/9781475708684. [Last accessed on 26 Jul 2024]

[10]

Acrylic pressure sensitive adhesives (PSA) market size & share analysis - growth trends & forecasts (2024-2029). Available from: https://www.mordorintelligence.com/industry-reports/acrylic-pressure-sensitive-adhesives-market. [Last accessed on 26 Jul 2024]

[11]

Gengnagel C,Bäumer R.Natural-fibre-reinforced plastics in actively bent structures.Proc Inst Civ Eng Constr Mater2013;166:365-77

[12]

Kim TW,Kim YC,Kim BJ.Bending strain and bending fatigue lifetime of flexible metal electrodes on polymer substrates.Materials2019;12:2490 PMCID:PMC6696189

[13]

Ugural AC. Chapter 5: Bending beams. In: Advanced mechanics of materials and applied elasticity. 5th ed. Prentice; 2019. pp. 226-91. Available from: https://ptgmedia.pearsoncmg.com/images/9780137079209/samplepages/0137079206.pdf. [Last accessed on 30 Jul 2024]

[14]

Yeh M,Cheng H.Bending stress analysis of laminated foldable touch panel.Procedia Eng2014;79:189-93

[15]

Nishimura M,Yamaguchi H.56-3: quantitative evaluation of neutral-plane splitting in foldable displays using folding stiffness measurements and finite element method simulations.SID Int Symp Dig Tech2020;51:834-7

[16]

Chae Y,Youn YO,Shin SH.Optimal design of thickness and young’s modulus of multi-layered foldable structure considering bending stress, neutral plane and delamination under 2.5 mm radius of curvature.Int J Precis Eng Manuf2018;19:1143-54

[17]

Hwang B,Park M.Neutral plane control by using polymer/graphene flake composites for flexible displays.RSC Adv2017;7:8186-91

[18]

Park Y,Hwang B.69-2: Development of flexible cover window for large foldable display with a pen-touch function.Symp Digest Tech Papers2021;52:1033-5

[19]

Choi GM,Shin D.Flexible hard coating: glass-like wear resistant, yet plastic-like compliant, transparent protective coating for foldable displays.Adv Mater2017;29:1700205

[20]

Jeong YC,Kim H.66-1: invited paper: flexible yet robust cover window with enhanced bending stiffness.Symp Digest Tech Papers2023;54:932-5

[21]

Jeong SY,Na Y.Foldable and washable textile-based OLEDs with a multi-functional near-room-temperature encapsulation layer for smart e-textiles.npj Flex Elect2021;5:15

[22]

Jeong EG,Kang KS,Choi KC.A review of highly reliable flexible encapsulation technologies towards rollable and foldable OLEDs.J Inform Display2020;21:19-32

[23]

Ha M,Park B.Highly flexible cover window using ultra-thin glass for foldable displays.J Mech Sci Technol2021;35:661-8

[24]

Jo W,Park Y,Gap Im S.Thermally stable and soft pressure-sensitive adhesive for foldable electronics.Chem Eng J2023;452:139050

[25]

Salmon F,Campbell C,Erdogan-haug B.64-1: modeling the mechanical performance of a foldable display panel bonded by 3M optically clear adhesives.Symp Digest Tech Papers2017;48:938-41

[26]

Han SH,Choi SS.Analytical investigation of multi-layered rollable displays considering nonlinear elastic adhesive interfaces.Sci Rep2023;13:5697 PMCID:PMC10082164

[27]

Kwon Y,Kim J.Ultraviolet light blocking optically clear adhesives for foldable displays via highly efficient visible-light curing.Nat Commun2024;15:2829

[28]

Back JH,Cho H.Visible-light-curable acrylic resins toward UV-light-blocking adhesives for foldable displays.Adv Mater2023;35:e2204776

[29]

Choi JW.Selectively UV-blocking and visibly transparent adhesive films embedded with TiO2/PMMA hybrid nanoparticles for displays.Materials2020;13:5273 PMCID:PMC7700452

[30]

Wu C,Wang Z.Efficient mechanoluminescent elastomers for dual-responsive anticounterfeiting device and stretching/strain sensor with multimode sensibility.Adv Funct Mater2018;28:1803168

[31]

Wang J,Cui K.Contact electrification induced multicolor self-recoverable mechanoluminescent elastomer for wearable smart light-emitting devices.Adv Opt Mater2023;11:2203112

[32]

Wang C,Peng D,Zhu D.Soft devices empowered by mechanoluminescent materials.Soft Sci2023;3:39

[33]

Li L,Yang L.Multistimuli-responsive artificial skin with dual output of photoelectric signals.Macro Mater Eng2021;306:2100017

[34]

Abrahamson JT,Salmon F.Optically clear adhesives for OLED. In: Pyshkin S, editor. Luminescence - OLED technology and applications. IntechOpen; 2019.

[35]

Nishimura M,Hishinuma M,Murayama A.A 5.5-inch full HD foldable AMOLED display based on neutral-plane splitting concept.J Soc Info Display2019;27:480-6

[36]

Su Y,Li R.Splitting of neutral mechanical plane of conformal, multilayer piezoelectric mechanical energy harvester.Appl Phys Lett2015;107:041905

[37]

Hishinuma M,Yamaguchi H.[FLX3-1(Invited)] Analysis of neutral-plane splitting for foldable displays using digital image correlation method.Proc Int Display Workshops2020;27:898

[38]

Lecavelier des Etangs-levallois A,Lesecq M.A converging route towards very high frequency, mechanically flexible, and performance stable integrated electronics.J Appl Phys2013;113:153701

[39]

Shi Y,Gao C.Multiple neutral axes in bending of a multiple-layer beam with extremely different elastic properties.J Appl Mech2014;81:114501

[40]

Li S,Li R.Splitting of the neutral mechanical plane depends on the length of the multi-layer structure of flexible electronics.Proc Math Phys Eng Sci2016;472:20160087 PMCID:PMC4950202

[41]

Wald MJ, Salmon FT, Cosgrove DT, Everaerts AI, inventors; 3M Innovative Properties Co., assignee. Flexible displays having stiff layers for neutral plane adjustment. United States patent US10334723B2. 2016. Available from: https://patents.google.com/patent/US10334723B2/en?oq=US10334723B2. [Last accessed on 30 Jul 2024]

[42]

Jeong K,Ahn D.A hyperelastic adhesive forming multiple neutral planes even at extreme temperatures.Chem Eng J2024;480:148151

[43]

Nam J,Han M.Improved stack structure of rollable display to prevent delamination and permanent deformation.Int J Precis Eng Manuf2021;22:671-8

[44]

Okumura Y.The polyrotaxane gel: a topological gel by figure-of-eight cross-links.Adv Mater2001;13:485-7

[45]

Kato K.Dynamic transition between rubber and sliding states attributed to slidable cross-links.Soft Matter2011;7:8737-40

[46]

Fleury G,Brochon C.Topological polymer networks with sliding cross-link points:  the “sliding gels”. relationship between their molecular structure and the viscoelastic as well as the swelling properties.Macromolecules2007;40:535-43

[47]

Du R,Zhu C.A Highly stretchable and self-healing supramolecular elastomer based on sliding crosslinks and hydrogen bonds.Adv Funct Mater2020;30:1907139

[48]

Bin Imran A,Gotoh H.Extremely stretchable thermosensitive hydrogels by introducing slide-ring polyrotaxane cross-linkers and ionic groups into the polymer network.Nat Commun2014;5:5124 PMCID:PMC4214411

[49]

Yi M,Han G.Movable cross-linking in adhesives: superior stretching and adhesion properties via a supramolecular sliding effect.ACS Appl Polym Mater2021;3:2678-86

[50]

Watabe T.Enhancing the reactivity of mechanically responsive units via macromolecular design.Macromolecules2024;57:425-33

[51]

Wang S,Kouznetsova TB.Facile mechanochemical cycloreversion of polymer cross-linkers enhances tear resistance.Science2023;380:1248-52

[52]

Ghanem MA,Behrou R.The role of polymer mechanochemistry in responsive materials and additive manufacturing.Nat Rev Mater2021;6:84-98

[53]

Wang S,Bowser BH.Mechanism dictates mechanics: a molecular substituent effect in the macroscopic fracture of a covalent polymer network.J Am Chem Soc2021;143:3714-8

[54]

Beech HK,Sen D.Reactivity-guided depercolation processes determine fracture behavior in end-linked polymer networks.ACS Macro Lett2023;12:1685-91

[55]

Zhao C,Wang S,Xuan S.Shear stiffening gels for intelligent anti-impact applications.Cell Rep Phys Sci2020;1:100266

[56]

Zhong D,Jiang Y.Author correction: high-speed and large-scale intrinsically stretchable integrated circuits.Nature2024;630:E12

[57]

Chun S,Baik S.Conductive and stretchable adhesive electronics with miniaturized octopus-like suckers against dry/wet skin for biosignal monitoring.Adv Funct Mater2018;28:1805224

[58]

Ates HC,Gonzalez-Macia L.End-to-end design of wearable sensors.Nat Rev Mater2022;7:887-907 PMCID:PMC9306444

[59]

Choi S,Kim H.Highly flexible and efficient fabric-based organic light-emitting devices for clothing-shaped wearable displays.Sci Rep2017;7:6424 PMCID:PMC5526867

[60]

Lee S,Kwon S.A review of flexible OLEDs toward highly durable unusual displays.IEEE Trans Electron Devices2017;64:1922-31

[61]

Song YJ,Cho HE.Fibertronic organic light-emitting diodes toward fully addressable, environmentally robust, wearable displays.ACS Nano2020;14:1133-40

[62]

Rogers JA,Huang Y.Materials and mechanics for stretchable electronics.Science2010;327:1603-7

[63]

Sekitani T.Stretchable, large-area organic electronics.Adv Mater2010;22:2228-46

[64]

Kang SH,Lee JM.Full integration of highly stretchable inorganic transistors and circuits within molecular-tailored elastic substrates on a large scale.Nat Commun2024;15:2814 PMCID:PMC10985077

[65]

Shi Y,Zhang B.Freestanding serpentine silicon strips with ultrahigh stretchability over 300% for wearable electronics.Adv Mater2024;36:e2313603

[66]

Wang Y,Jin L.Excitation threshold reduction techniques for organic semiconductor lasers: a review.Coatings2023;13:1815

[67]

Chen J,Wang L.Recent research progress of organic small-molecule semiconductors with high electron mobilities.Adv Mater2023;35:2210772

[68]

Jung D,Cho S,Hong C.Multilayer stretchable electronics with designs enabling a compact lateral form.npj Flex Electron2024;8:13

[69]

Park J,Lim S.Conformal fixation strategies and bioadhesives for soft bioelectronics.Adv Funct Mater2024;34:2313728

[70]

Efstathiou S,Ross A,Haddleton DM.Moisture-cured solvent free silylated poly(ether-urea) pressure-sensitive adhesives (PSAs) for use as skin adhesives for application in transdermal drug delivery (TDD).Mater Adv2024;5:3396-410

[71]

Zheng Y,Duan M.Skin temperature-triggered switchable adhesive coatings for wearing comfortable epidermal electronics.Chem Eng J2024;488:150459

[72]

Fialho L,Pinho AS.Exploring innovative adhesive approaches to manage medical adhesive-related skin injuries (MARSI).Int J Adhes Adhes2024;130:103636

[73]

Guo H,Jia Z.A biodegradable supramolecular adhesive with robust instant wet adhesion for urgent hemostasis and wound repair.Adv Funct Mater2024;34:2401529

[74]

Yuan X,Xia P.Implantable wet-adhesive flexible electronics with ultrathin gelatin film.Adv Funct Mater2024;2404824

[75]

Zhou Y,Liu Y.Transparent, stretchable, self-healing, and self-adhesive ionogels for flexible multifunctional sensors and encryption systems.Chem Eng J2024;484:149632

[76]

Roslan MF,Khairusshima MKN.Finite element analysis on deformation of stretchable electronic interconnect substrate using polydimethylsiloxanes (PDMS).IOP Conf Ser Mater Sci Eng2018;290:012022

[77]

Shao Y,Novitski R.Uniaxial cell stretching device for live-cell imaging of mechanosensitive cellular functions.Rev Sci Instrum2013;84:114304 PMCID:PMC3862604

[78]

Hong JH,Lee J,Kim S.74-1: Invited paper: highly stretchable and shrinkable AMOLED for free deformation.Symp Digest Tech Papers2023;54:1041-4

[79]

Wang CL,Wang WT.41-3: Invited paper: high resolution stretchable micro-LED displays.Symp Digest Tech Papers2022;53:521-3

[80]

Sluka T.42-1: Invited paper: high-resolution light-field AR at comparable computing cost to stereo 3D.Symp Digest Tech Papers2022;53:526-7

[81]

Kang J,Tang W.71-2: Enabling processes and designs for tight-pitch micro-LED based stretchable display.Symp Digest Tech Papers2021;52:1056-9

[82]

Khang DY,Huang Y.A stretchable form of single-crystal silicon for high-performance electronics on rubber substrates.Science2006;311:208-12

[83]

Dana SF,Kochhar JS,Kang L.UV-curable pressure sensitive adhesive films: effects of biocompatible plasticizers on mechanical and adhesion properties.Soft Matter2013;9:6270-81

[84]

Roy A,Ray PG,Pal S.β-cyclodextrin-based ultrahigh stretchable, flexible, electro- and pressure-responsive, adhesive, transparent hydrogel as motion sensor.ACS Appl Mater Interfaces2022;14:17065-80

[85]

Mao J,Liu L.Adhesive, transparent, stretchable, and strain-sensitive hydrogel as flexible strain sensor.Compos Commun2021;25:100733

[86]

Han GY,Lee TH,Kim HJ.Highly resilient dual-crosslinked hydrogel adhesives based on a dopamine-modified crosslinker.ACS Appl Mater Interfaces2022;14:36304-14

[87]

Yi M,Lee S,Kim H.Topologically designed cross-linking network for stretchable and recoverable pressure-sensitive adhesives with exceptional softness.Mater Today Chem2022;26:101141

[88]

Campbell CJ,Behling RE.P-198: optically clear adhesives enabling foldable and flexible OLED displays.Symp Digest Tech Papers2017;48:2009-11

[89]

Lee TI,Kim W,Paik KW.Direct visualization of cross-sectional strain distribution in flexible devices.ACS Appl Mater Interfaces2019;11:13416-22

[90]

Kim W,Yoon Kim D.Controlled multiple neutral planes by low elastic modulus adhesive for flexible organic photovoltaics.Nanotechnology2017;28:194002

[91]

Park Y,Ahn D,Lee W.Biomass-derived optically clear adhesives for foldable displays.ChemSusChem2024;:e202301795

[92]

Lee MH,Hwang BH,Kim JJ.53-1: The foldable display architecture technique depending on the wide temperature range and the folding curvature.Symp Digest Tech Papers2022;53:692-5

[93]

Gower MD.Acrylic acid level and adhesive performance and peel master-curves of acrylic pressure-sensitive adhesives.J Polym Sci B Polym Phys2006;44:1237-52

[94]

Chang EP.Viscoelastic properties of pressure-sensitive adhesives.J Adhes1997;60:233-48

[95]

Tanaka F.Viscoelastic properties of physically crosslinked networks. 1. Transient network theory.Macromolecules1992;25:1516-23

[96]

Tanaka F.Viscoelastic properties of physically crosslinked networks: Part 2. Dynamic mechanical moduli.J Non-Newton Fluid Mech1992;43:273-88

[97]

Eckstein A,Friedrich C.Determination of plateau moduli and entanglement molecular weights of isotactic, syndiotactic, and atactic polypropylenes synthesized with metallocene catalysts.Macromolecules1998;31:1335-40

[98]

Dobrynin AV,Jacobs M.Forensics of polymer networks.Nat Mater2023;22:1394-400

[99]

Malvern Instrument. A basic introduction to rheology. Available from: https://cdn.technologynetworks.com/TN/Resources/PDF/WP160620BasicIntroRheology.pdf. [Last accessed on 26 Jul 2024]

[100]

Lee TH,Lee JH.Pressure-sensitive adhesives for flexible display applications. In: Vargas-Bernal R, He P, Zhang S, editors. Hybrid nanomaterials - flexible electronics materials. IntechOpen; 2019.

[101]

Mittal KL.The role of the interface in adhesion phenomena.Polym Eng Sci1977;17:467-73

[102]

Yuk H,Lin S,Zhao X.Tough bonding of hydrogels to diverse non-porous surfaces.Nat Mater2016;15:190-6 PMCID:PMC4762474

[103]

Krenceski MA,Temin SC.Chemical and physical factors affecting performance of pressure-sensitive adhesives.J Macromol Sci Part C Polym Rev1986;26:143-82

[104]

Kinloch AJ.Chapter 8 - The mechanics of peel tests.Adhes Sci Eng2002;1:273-301

[105]

Czech Z.Crosslinking of pressure sensitive adhesive based on water-borne acrylate.Polym Int2003;52:347-57

[106]

Lee J,Shim K.Effect of crosslinking density on adhesion performance and flexibility properties of acrylic pressure sensitive adhesives for flexible display applications.Int J Adhes Adhes2017;74:137-43

[107]

Kinloch AJ.Adhesion and adhesives: science and technology. Springer Science & Business Media; 1987.

[108]

Pocius AV.Adhesion and adhesives technology: an introduction. 3rd ed. Carl Hanser Verlag GmbH & Company KG; 2012.

[109]

Israelachvili J.Intermolecular and surface forces. 3rd ed. Academic Press; 2011.

[110]

Won Y,Jo M,Manda R.An electrically switchable dye-doped liquid crystal polarizer for organic light emitting-diode displays.J Mol Liquids2021;333:115922

[111]

Vaenkatesan V,Teunissen J,Bastiaansen C.Improving the brightness and daylight contrast of organic light-emitting diodes.Adv Funct Mater2005;15:138-42

[112]

Hack M, Ma R, inventors; Universal Display Corporation., assignee. Integrated circular polarizer and permeation barrier for flexible OLEDs. United States patent US20180047945A1. 2016. Available from: https://patents.google.com/patent/US20180047945A1/en?oq=US20180047945A1. [Last accessed on 30 Jul 2024]

[113]

Antosik AK,Czech Z.Aging of silicone pressure-sensitive adhesives.Polym Bull2018;75:1141-7

[114]

Schwotzer W,Roduit B. Simulating the aging of adhesives. Adhesives & Sealants Industry, 2008. Available from: https://www.adhesivesmag.com/articles/87025-simulating-the-aging-of-adhesives. [Last accessed on 26 Jul 2024]

[115]

Rudawska A,Müller M.Effect of ageing process on mechanical properties of adhesive tubular butt joints in aqueous environment.Int J Adhes Adhes2020;96:102466

[116]

ASTM D3632-98. Standard test method for accelerated aging of adhesive joints by the oxygen-pressure method. Available from: https://www.astm.org/d3632-98.html. [Last accessed on 30 Jul 2024]

[117]

ASTM D3611-06. Standard practice for accelerated aging of pressure-sensitive tapes. Available from: https://www.astm.org/d3611-06.html. [Last accessed on 30 Jul 2024]

[118]

Chiang C,Bull S.Mechanical modeling of flexible OLED devices.Org Electron2009;10:1268-74

[119]

Ma BS,Kim W.Mechanical modeling of rollable OLED display apparatus considering spring component.J Microelect Pack Soc2020;27:19-26

[120]

Li S,Li R.Shear deformation dominates in the soft adhesive layers of the laminated structure of flexible electronics.Int J Solids Struct2017;110-1:305-14

[121]

Jang SJ, Myung NJ, Hwang BH, Woo SW, Kwak TH, inventors; LG Display, assignee. Foldable display device. United States patent US10198038B2. 2019. Available from: https://patents.google.com/patent/US10198038B2/en?oq=US10198038B2. [Last accessed on 30 Jul 2024]

[122]

Jia Y,Wu D,Meng H.Mechanical simulation of foldable AMOLED panel with a module structure.Org Electron2019;65:185-92

[123]

Niu L,Liu W.Analysis on the mechanical behavior of flexible screens.Materials2022;15:2829 PMCID:PMC9032455

[124]

Chen ZP,Wang S,Yuan Z.P-119: modeling of mechanical effects in flexible display.Symp Digest Tech Papers2020;51:1818-21

[125]

Zhang Y,Dong F.Mechanical behavior and constitutive model characterization of optically clear adhesive in flexible devices.Micromachines2022;13:301 PMCID:PMC8879156

[126]

Lee JH,Baek MJ,Lee DW.Effects of monomer functionality on physical properties of 2-ethylhexyl acrylate based stretchable pressure sensitive adhesives.Polym Test2019;76:305-11

[127]

Lee JH,Myung MH,Kim H.Stretchable and recoverable acrylate-based pressure sensitive adhesives with high adhesion performance, optical clarity, and metal corrosion resistance.Chem Eng J2021;406:126800

[128]

Lim D,Kim H,Lee DW.Carboxyethyl acrylate incorporated optically clear adhesives with outstanding adhesion strength and immediate strain recoverability for stretchable electronics.Chem Eng J2022;437:135390

[129]

Lee K,Martchenko V.A modular strategy for functional pressure sensitive adhesives.ACS Appl Mater Interfaces2021;13:3161-5

[130]

Seok WC,Song HJ.Acrylic pressure-sensitive adhesives based on ethylene glycol acrylate for flexible display application: Highly elastic and recoverable properties.Polym Test2022;108:107491

[131]

Seok WC,Song HJ.Effect of silane acrylate on the surface properties, adhesive performance, and rheological behavior of acrylic pressure sensitive adhesives for flexible displays.J Ind Eng Chem2022;111:98-110

[132]

Seok WC,Song HJ.The effect of silane acrylate containing ethylene glycol chains on the adhesive performance and viscoelastic behavior of acrylic pressure-sensitive adhesives for flexible displays.Polymers2023;15:3601 PMCID:PMC10489647

[133]

Moussa K.Light-induced polymerization of new highly reactive acrylic monomers.J Polym Sci A Polym Chem1993;31:2197-203

[134]

Lee TY,Jönsson ES,Hoyle CE.Influence of hydrogen bonding on photopolymerization rate of hydroxyalkyl acrylates.Macromolecules2004;37:3659-65

[135]

Vleeschouwer F, Van Speybroeck V, Waroquier M, Geerlings P, De Proft F. Electrophilicity and nucleophilicity index for radicals.Org Lett2007;9:2721-4

[136]

Taghizadeh SM.Rheological and adhesion properties of acrylic pressure-sensitive adhesives.J Appl Polymer Sci2011;120:411-8

[137]

Sanai Y,Kubota K.Cross-linking photopolymerization of monoacrylate initiated by benzophenone.J Polym Sci Part A Polym Chem2018;56:1545-53

[138]

Novikov V.Correlation between glass transition temperature and molecular mass in non-polymeric and polymer glass formers.Polymer2013;54:6987-91

[139]

Hintermeyer J,Kahlau R,Rössler EA.Molecular weight dependence of glassy dynamics in linear polymers revisited.Macromolecules2008;41:9335-44

[140]

Zhang P,He Y.Stretchable heterogeneous polymer networks of high adhesion and low hysteresis.ACS Appl Mater Interfaces2022;14:49264-73

[141]

Moon H,Kwak MJ,Im SG.Solvent-free deposition of ultrathin copolymer films with tunable viscoelasticity for application to pressure-sensitive adhesives.ACS Appl Mater Interfaces2018;10:32668-77

[142]

Kim J,Baek D,Kim Y.Characterization and flexibility properties of UV LED cured acrylic pressure-sensitive adhesives for flexible displays.J Mater Res Technol2021;10:1176-83

[143]

Kim J,Kim Y.Flexibility properties of pressure-sensitive adhesive with different pattern of crosslinking density for electronic displays.J Mater Res Technol2021;15:1408-15

[144]

Lee J,Kim H.Ultraviolet-patterned acrylic pressure-sensitive adhesives for flexible displays.Polymer2021;237:124324

[145]

Back JH,Kim Y.Heterogeneous acrylic resins with bicontinuous nanodomains as low-modulus flexible adhesives.Small2024;e2403497

[146]

Bonnotte T,Araque M,Dumeignil F.Dehydration of lactic acid: the state of the art.ChemBioEng Rev2018;5:34-56

[147]

Haque FM,Lidston CAL.Defining the macromolecules of tomorrow through synergistic sustainable polymer research.Chem Rev2022;122:6322-73

[148]

Gabriel VA.Toward a fully biobased pressure-sensitive adhesive.Ind Eng Chem Res2023;62:478-88

[149]

Droesbeke MA,Simula A,Du Prez FE.Biobased acrylic pressure-sensitive adhesives.Prog Polym Sci2021;117:101396

[150]

Chen TTD,Sulley GS,Williams CK.Bio-based and degradable block polyester pressure-sensitive adhesives.Angew Chem Int Ed Engl2020;132:23656-61 PMCID:PMC7756385

[151]

Albanese KR,Morris PT.Building tunable degradation into high-performance poly(acrylate) pressure-sensitive adhesives.ACS Macro Lett2023;12:787-93

[152]

Machado TO,Chiaradia V.A renewably sourced, circular photopolymer resin for additive manufacturing.Nature2024;629:1069-74 PMCID:PMC11136657

[153]

Castagnet T,Asua JM.Bioinspired enzymatic synthesis of terpenoid-based (meth)acrylic monomers: a solvent-, metal-, amino-, and halogen-free approach.ACS Sustainable Chem Eng2020;8:7503-12

[154]

Hermens JGH,Feringa BL.Highly efficient biobased synthesis of acrylic acid.Angew Chem Int Ed Engl2022;61:e202112618 PMCID:PMC9299676

[155]

Droesbeke MA.Sustainable synthesis of renewable terpenoid-based (meth)acrylates using the CHEM21 green metrics toolkit.ACS Sustainable Chem Eng2019;7:11633-9

[156]

Obermeier F,Stockmann PN.Syntheses and polymerization of monoterpene-based (meth)acrylates: IBO(M)A as a relevant monomer for industrial applications.Green Chem2024;26:4387-416

[157]

Jarach N.Debondable, recyclable and/or biodegradable naturally-based adhesives. In: Dunky M, Mittal K, editors. Biobased adhesives. Wiley; 2023. pp. 427-61.

[158]

Veith C,Miller SA.Synthesis and polymerization of bio-based acrylates: a review.Polym Chem2020;11:7452-70

[159]

Nasiri M,Reineke TM.Enhanced mechanical and adhesion properties in sustainable triblock copolymers via non-covalent interactions.Macromolecules2018;51:2456-65

[160]

Badía A,Barandiaran MJ.Removable biobased waterborne pressure-sensitive adhesives containing mixtures of isosorbide methacrylate monomers.Biomacromolecules2020;21:4522-31

[161]

Gallagher JJ,Reineke TM.Acrylic triblock copolymers incorporating isosorbide for pressure sensitive adhesives.ACS Sustainable Chem Eng2016;4:3379-87

[162]

Heo J,Jang SG.Improved performance of protected catecholic polysiloxanes for bioinspired wet adhesion to surface oxides.J Am Chem Soc2012;134:20139-45 PMCID:PMC3521601

[163]

Li Y.Synthesis and characterization of acrylic polyols and polymers from soybean oils for pressure-sensitive adhesives.RSC Adv2015;5:44009-17

[164]

Fouilloux H,Robert C,Thomas CM.Multicatalytic transformation of (meth)acrylic acids: a one-pot approach to biobased poly(meth)acrylates.Angew Chem Int Ed Engl2021;60:19374-82

[165]

Abraham TW, Allen E, Hahn JJ, Tsobanakis P, Bohnert EC, Frank CL, inventors; Cargill Inc., assignee. Recovery of 3-hydroxypropionic acid. United States patent US10442748B2. 2019. Available from: https://patents.google.com/patent/US10442748B2/en?oq=US10442748B2. [Last accessed on 30 Jul 2024]

[166]

Abubakar UC,Forster L,D’agostino C.Conversion of glycerol to acrylic acid: a review of strategies, recent developments and prospects.React Chem Eng2023;8:1819-38

[167]

Bio-acrylic acid market by type (methyl acrylate, ethyl acrylate, butyl acrylate, elastomers, 2-ethylhexyl acrylate, superabsorbent polymers), application and tegion (north america, europe, the asia pacific, and the rest of the world.) - global forecast to 2027. Available from: https://www.marketsandmarkets.com/Market-Reports/bio-acrylic-acid-market-144896040.html. [Last accessed on 26 Jul 2024]

[168]

Atkinson RL,Elsmore MT.RAFT polymerisation of renewable terpene (meth)acrylates and the convergent synthesis of methacrylate-acrylate-methacrylate triblock copolymers.Polym Chem2021;12:3177-89

[169]

Zhang L,Wang L,Bai Y.Polyacrylate emulsion containing IBOMA for removable pressure sensitive adhesives.J Appl Polym Sci2016;133:42886

[170]

Droesbeke MA,Asua JM.Biosourced terpenoids for the development of sustainable acrylic pressure-sensitive adhesives via emulsion polymerisation.Green Chem2020;22:4561-9

[171]

Baek SS.Preparation of biomass-based transparent pressure sensitive adhesives for optically clear adhesive and their adhesion performance.Eur Polym J2017;92:97-104

[172]

Baek SS,Hwang SH.Construction and adhesion performance of biomass tetrahydro-geraniol-based sustainable/transparent pressure sensitive adhesives.J Ind Eng Chem2017;53:429-34

[173]

Badía A,Agirre A,Leiza JR.UV-tunable biobased pressure-sensitive adhesives containing piperonyl methacrylate.ACS Sustainable Chem Eng2019;7:19122-30

[174]

Agirre A,Degrandi E,Asua JM.Improving adhesion of acrylic waterborne PSAs to low surface energy materials: introduction of stearyl acrylate.J Polym Sci A Polym Chem2010;48:5030-9

[175]

Iso T,Kagami S,Sanai Y.Environmentally-friendly UV-curable coatings utilizing bio-based polyester acrylates.Prog Org Coat2023;175:107356

[176]

Hub L,Held M,Abetz V.Amphiphilic block copolymers via blue-light-induced iniferter RAFT ab initio emulsion polymerization in water–alcoholic media.Macromolecules2024;57:2273-86

[177]

Lovell PA.Fundamentals of emulsion polymerization.Biomacromolecules2020;21:4396-441

[178]

Noppalit S,Billon L.On the nitroxide mediated polymerization of methacrylates derived from bio-sourced terpenes in miniemulsion, a step towards sustainable products.Polym Chem2020;11:1151-60

[179]

Yan Y,Wang Y.Strong and UV-responsive plant oil-based ethanol aqueous adhesives fabricated via surfactant-free RAFT-mediated emulsion polymerization.ACS Sustainable Chem Eng2021;9:13695-702

[180]

Lee Y,Kim Y.A water-soluble organic photocatalyst discovered for highly efficient additive-free visible-light-driven grafting of polymers from proteins at ambient and aqueous environments.Adv Mater2022;34:e2108446

[181]

Niu J,Dolinski ND.Rapid visible light-mediated controlled aqueous polymerization with in situ monitoring.ACS Macro Lett2017;6:1109-13

[182]

Chung KY.Boron-methylated dipyrromethene as a green light activated type i photoinitiator for rapid radical polymerizations.J Am Chem Soc2023;145:17912-8

[183]

Tucker BS,Figg CA.Grafting-from proteins using metal-free PET-RAFT polymerizations under mild visible-light irradiation.ACS Macro Lett2017;6:452-7

[184]

Borjigin T,Giacoletto N.The blue-LED-sensitive naphthoquinone-imidazolyl derivatives as type II photoinitiators of free radical photopolymerization.Adv Mater Interfaces2023;10:2202352

[185]

Lee Y,Kwon MS.Photocontrolled RAFT polymerization: past, present, and future.Chem Soc Rev2023;52:3035-97

[186]

Jeon W,Kwon MS.Highly efficient dual photoredox/copper catalyzed atom transfer radical polymerization achieved through mechanism-driven photocatalyst design.Nat Commun2024;15:5160 PMCID:PMC11183263

[187]

Corrigan N,Judzewitsch P,Boyer C.Seeing the light: advancing materials chemistry through photopolymerization.Angew Chem Int Ed Engl2019;58:5170-89

[188]

Fors BP.Control of a living radical polymerization of methacrylates by light.Angew Chem Int Ed Engl2012;51:8850-3

[189]

Singh VK,Badgujar S.Highly efficient organic photocatalysts discovered via a computer-aided-design strategy for visible-light-driven atom transfer radical polymerization.Nat Catal2018;1:794-804

[190]

Kim D,Jeon W.Ultraviolet light debondable optically clear adhesives for flexible displays through efficient visible-light curing.Adv Mater2024;36:e2309891

[191]

Song Y,Zhang Y,Chen EYX.Recyclable cyclic bio-based acrylic polymer via pairwise monomer enchainment by a trifunctional Lewis pair.Nat Chem2023;15:366-76

[192]

Jehanno C,Roosen M.Critical advances and future opportunities in upcycling commodity polymers.Nature2022;603:803-14

[193]

Deacy AC,Sulley GS,Williams CK.Sequence control from mixtures: switchable polymerization catalysis and future materials applications.J Am Chem Soc2021;143:10021-40 PMCID:PMC8297863

[194]

Liu Z.Switchable adhesion: on-demand bonding and debonding.Adv Sci2022;9:e2200264 PMCID:PMC9036041

[195]

Wang ZH,Zeng FR.Fully recyclable multifunctional adhesive with high durability, transparency, flame retardancy, and harsh-environment resistance.Sci Adv2022;8:eadd8527 PMCID:PMC9750157

[196]

Hwang J,Lee G.Ambient air-operated thermo-switchable adhesion of N-isopropylacrylamide-incorporated pressure sensitive adhesives.Mater Horiz2023;10:2013-23

[197]

Mulcahy KR,Harper GDJ,Abbott AP.Debondable adhesives and their use in recycling.Green Chem2022;24:36-61

[198]

Beharaj A,Grinstaff MW.Poly(alkyl glycidate carbonate)s as degradable pressure-sensitive adhesives.Angew Chem2019;131:1421-5

[199]

Beharaj A,Blessing WA.Sustainable polycarbonate adhesives for dry and aqueous conditions with thermoresponsive properties.Nat Commun2019;10:5478 PMCID:PMC6889139

[200]

Shieh P,Husted KEL.Cleavable comonomers enable degradable, recyclable thermoset plastics.Nature2020;583:542-7 PMCID:PMC7384294

[201]

Pesenti T.100th Anniversary of Macromolecular Science Viewpoint: degradable polymers from radical ring-opening polymerization: latest advances, new directions, and ongoing challenges.ACS Macro Lett2020;9:1812-35

[202]

Kim HJ,Shim J,Hillmyer MA.Sustainable triblock copolymers as tunable and degradable pressure sensitive adhesives.ACS Sustainable Chem Eng2020;8:12036-44

[203]

Bakar R, Hepburn KS, Keddie JL, Roth PJ. Degradable, ultraviolet-crosslinked pressure-sensitive adhesives made from thioester-functional acrylate copolymers.Angew Chem Int Ed Engl2023;62:e202307009

[204]

Bakar RA,Roth PJ.New chemistries for degradable pressure-sensitive adhesive networks.Chempluschem2024;89:e202400034

[205]

Albanese KR,Read de Alaniz J,Hawker CJ.Controlled-radical polymerization of α-lipoic acid: a general route to degradable vinyl copolymers.J Am Chem Soc2023;145:22728-34 PMCID:PMC10591472

[206]

Korpusik AB,Bhatt K,Seidel D.Degradation of polyacrylates by one-pot sequential dehydrodecarboxylation and ozonolysis.J Am Chem Soc2023;145:10480-5

[207]

Abel BA,Coates GW.Chemically recyclable thermoplastics from reversible-deactivation polymerization of cyclic acetals.Science2021;373:783-9

[208]

Bandl C,Schlögl S.Adhesives for “debonding-on-demand”: triggered release mechanisms and typical applications.Int J Adhes Adhes2020;99:102585

[209]

Lundberg DJ,Kilgallon LJ.Defining reactivity-deconstructability relationships for copolymerizations involving cleavable comonomer additives.ACS Macro Lett2024;13:521-7

[210]

McCluskey P,Beysser O.Low temperature delamination of plastic encapsulated microcircuits.Microelectro Reliab1998;38:1829-34

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