Electroactuated liquid crystal polymers

Ruitong Song , Jiu-an Lv

Responsive Materials ›› 2025, Vol. 3 ›› Issue (4) : e70022

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Responsive Materials ›› 2025, Vol. 3 ›› Issue (4) :e70022 DOI: 10.1002/rpm2.70022
REVIEW ARTICLE
Electroactuated liquid crystal polymers
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Abstract

As a typical smart soft material, liquid crystal polymers (LCPs) exhibit significant reversible deformation under external stimuli, possessing excellent mechanical and processable properties, which make LCPs highly promising for applications in artificial muscles, soft robotics, smart fabrics, smart wearable devices, and microfluidics. LCPs can respond to various stimuli, including heat, light, electricity, magnetism, and humidity. Among these, electroactuated LCPs stand out because they can integrate with circuits to achieve programmable control, multichannel parallel control, and effective control in dense and/or sheltered environments. This review introduces recent research progress on electroactuated LCPs. First, electroactuated LCPs are classified based on actuation principles, and working mechanisms, advantages, and shortcomings are discussed. Then, the related applications capable of demonstrating the characteristics of electroactuated LCPs are introduced. Finally, we summarize each class of electroactuated LCPs and discuss their potential for future developments.

Keywords

artificial muscles / bionic actuators / electro-response / liquid crystal polymers / soft robotics

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Ruitong Song, Jiu-an Lv. Electroactuated liquid crystal polymers. Responsive Materials, 2025, 3(4): e70022 DOI:10.1002/rpm2.70022

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References

[1]

P. G. d. Gennes, Science 1992, 256, 495.

[2]

J. Su, K. He, Y. Li, J. Tu, X. Chen, Chem. Rev. 2025, 125, 5848.

[3]

M. Ilami, H. Bagheri, R. Ahmed, E. O. Skowronek, H. Marvi, Adv. Mater. 2020, 33, 2003139.

[4]

Y. Zhang, Z. G. Zheng, Q. Li, Responsive Mater. 2024, 2, 2, e20230029.

[5]

H. K. Bisoyi, Q. Li, Chem. Rev. 2021, 122, 4887.

[6]

J. Gao, Y. Tang, D. Martella, J. Guo, D. S. Wiersma, Q. Li, Responsive Mater. 2023, 1, e20230008.

[7]

K. M. Herbert, H. E. Fowler, J. M. McCracken, K. R. Schlafmann, J. A. Koch, T. J. White, Nat. Rev. Mater. 2021, 7, 23.

[8]

S. V. Ahir, A. R. Tajbakhsh, E. M. Terentjev, Adv. Funct. Mater. 2006, 16, 556.

[9]

H. Yang, A. Buguin, J.-M. Taulemesse, K. Kaneko, S. Méry, A. Bergeret, P. Keller, J. Am. Chem. Soc. 2009, 131, 15000.

[10]

T. J. White, D. J. Broer, Nat. Mater. 2015, 14, 1087.

[11]

M. H. Li, P. Keller, B. Li, X. Wang, M. Brunet, Adv. Mater. 2003, 15, 569.

[12]

Y. Xu, M. Jin, J. Wang, S. Huang, Q. Li, Responsive Mater. 2024, 2, e20240020.

[13]

W. Zhang, Y. Nan, Z. Wu, Y. Shen, D. Luo, Molecules 2022, 27, 4330.

[14]

Z. Zhang, J. Li, R. Zhang, R. Chen, Y. Zhang, T. Wang, K. L. Yang, J. Zhu, Responsive Mater. 2024, 2, e20240021.

[15]

J. Wang, Y. Wen, D. Pan, S. Lin, A. Chinnappan, Q. He, C. Liu, Z. Huang, S. Cai, S. Ramakrishna, S. Shin, Nano Lett. 2024, 24, 9990.

[16]

Y. Takezawa, N. Furukawa, S. Nachimuthu, R. Zhou, A. Torbati, ACS Omega 2024, 9, 20839.

[17]

J. Ma, Z. Yang, Matter 2025, 8, 101950.

[18]

W. Hou, J. Wang, J.-a. Lv, Adv. Mater. 2023, 35, e2211800.

[19]

Z. Hu, Y. Li, J. A. Lv, Nat. Commun. 2021, 12, 3211.

[20]

Q. He, Z. Wang, Y. Wang, Z. Wang, C. Li, R. Annapooranan, J. Zeng, R. Chen, S. Cai, Sci. Robot. 2021, 6, eabi9704.

[21]

H. Yang, D. Wu, S. Zheng, Y. Yu, L. Ren, J. Li, H. Ke, P. Lv, Q. Wei, ACS Appl. Mater. Interfaces 2024, 16, 9313.

[22]

P. Zhang, G. Wang, H. Yu, Responsive Mater. 2024, 2, e20240016.

[23]

Y. Wu, S. Zhang, Y. Yang, Z. Li, Y. Wei, Y. Ji, Sci. Adv. 2022, 8, eabo6021.

[24]

Y. Nemati, Q. Yang, F. Sohrabi, J. V. I. Timonen, C. Sánchez-Somolinos, M. Honkanen, H. Zeng, A. Priimagi, ACS Appl. Mater. Interfaces 2025, 17, 5316.

[25]

V. Maurin, Y. Chang, Q. Ze, S. Leanza, J. Wang, R. R. Zhao, Adv. Mater. 2023, 36, 2302765.

[26]

X. Yang, S. Leanza, Q. Ze, R. R. Zhao, Mater. Today 2025, 87, 11.

[27]

R. Lan, W. Shen, W. Yao, J. Chen, X. Chen, H. Yang, Mater. Horiz. 2023, 10, 2824.

[28]

A. Agrawal, H. Chen, H. Kim, B. Zhu, O. Adetiba, A. Miranda, A. Cristian Chipara, P. M. Ajayan, J. G. Jacot, R. Verduzco, ACS Macro Lett. 2016, 5, 1386.

[29]

C. P. Ambulo, M. J. Ford, K. Searles, C. Majidi, T. H. Ware, ACS Appl. Mater. Interfaces 2020, 13, 12805.

[30]

M. J. Ford, C. P. Ambulo, T. A. Kent, E. J. Markvicka, C. Pan, J. Malen, T. H. Ware, C. Majidi, Proc. Natl. Acad. Sci. 2019, 116, 21438.

[31]

S. Schuhladen, F. Preller, R. Rix, S. Petsch, R. Zentel, H. Zappe, Adv. Mater. 2014, 26, 7247.

[32]

Q. He, Z. Wang, Y. Wang, A. Minori, M. T. Tolley, S. Cai, Sci. Adv. 2019, 5, eaax5746.

[33]

C. Wang, K. Sim, J. Chen, H. Kim, Z. Rao, Y. Li, W. Chen, J. Song, R. Verduzco, C. Yu, Adv. Mater. 2018, 30, 1706695.

[34]

Y. Y. Xiao, Z. C. Jiang, X. Tong, Y. Zhao, Adv. Mater. 2019, 31, 1903452.

[35]

Y. Wang, Z. Wang, Q. He, P. Iyer, S. Cai, Adv. Intell. Syst. 2020, 2, 1900177.

[36]

J. H. Lee, J. Bae, J. H. Hwang, M. Y. Choi, Y. S. Kim, S. Park, J. H. Na, D. G. Kim, S. k. Ahn, Adv. Funct. Mater. 2021, 32, 2110360.

[37]

K. Liu, F. Hacker, C. Daraio, Sci. Robot. 2021, 6, eabf5116.

[38]

H. Yang, X. Yin, C. Zhang, B. Chen, P. Sun, Y. Xu, Sci. Adv. 2025, 11, eads3058.

[39]

A. Kotikian, J. M. Morales, A. Lu, J. Mueller, Z. S. Davidson, J. W. Boley, J. A. Lewis, Adv. Mater. 2021, 33, 2101814.

[40]

J. Sun, Y. Wang, W. Liao, Z. Yang, Small 2021, 17, 2103700.

[41]

X. Zhang, W. Liao, C. Zhu, Z. Yang, ACS Appl. Polym. Mater. 2024, 6, 11050.

[42]

M. Wang, Z.-W. Cheng, B. Zuo, X.-M. Chen, S. Huang, H. Yang, ACS Macro Lett. 2020, 9, 860.

[43]

P. Lv, X. Yang, H. K. Bisoyi, H. Zeng, X. Zhang, Y. Chen, P. Xue, S. Shi, A. Priimagi, L. Wang, W. Feng, Q. Li, Mater. Horiz. 2021, 8, 2475.

[44]

Y. Wang, Q. He, Z. Wang, S. Zhang, C. Li, Z. Wang, Y.-L. Park, S. Cai, Adv. Mater. 2023, 35, e2211283.

[45]

H. Kim, J. Gibson, J. Maeng, M. O. Saed, K. Pimentel, R. T. Rihani, J. J. Pancrazio, S. V. Georgakopoulos, T. H. Ware, ACS Appl. Mater. Interfaces 2019, 11, 19506.

[46]

J. C. Ince, A. R. Duffy, N. V. Salim, Macromol. Rapid Commun. 2024, 45, 2400370.

[47]

C. Zhu, Y. Zhang, G. He, Y. Shi, Y. Wu, Y. Yu, X. Liu, Adv. Funct. Mater. 2024, 35, 2413845.

[48]

D. Wu, Y. Zhang, H. Yang, A. Wei, Y. Zhang, A. Mensah, R. Yin, P. Lv, Q. Feng, Q. Wei, Mater. Horiz. 2023, 10, 2587.

[49]

S. Wu, Y. Hong, Y. Zhao, J. Yin, Y. Zhu, Sci. Adv. 2023, 9, eadf8014.

[50]

C. Yuan, D. J. Roach, C. K. Dunn, Q. Mu, X. Kuang, C. M. Yakacki, T. J. Wang, K. Yu, H. J. Qi, Soft Matter 2017, 13, 5558.

[51]

T. A. Kent, M. J. Ford, E. J. Markvicka, C. Majidi, Multifunct. Mater. 2020, 3, 025003.

[52]

B. Ma, C. Xu, L. Cui, C. Zhao, H. Liu, ACS Appl. Mater. Interfaces 2021, 13, 5574.

[53]

P. Lyu, D. J. Broer, D. Liu, Nat. Commun. 2024, 15, 4191.

[54]

L. S. van Hazendonk, Z. J. Khalil, W. van Grondelle, L. E. A. Wijkhuijs, I. Schreur-Piet, M. G. Debije, H. Friedrich, ACS Appl. Mater. Interfaces 2024, 16, 32739.

[55]

H. Liu, H. Tian, J. Shao, Z. Wang, X. Li, C. Wang, X. Chen, ACS Appl. Mater. Interfaces 2020, 12, 56338.

[56]

J. Wang, H. Zhou, Y. Fan, W. Hou, T. Zhao, Z. Hu, E. Shi, J.-a. Lv, Mater. Horiz. 2024, 11, 1877.

[57]

Z. Wang, J. Zhang, G. J. Weng, Polymer 2025, 324, 128262.

[58]

X. Li, J. Lin, J. Wu, M. Liu, P. Du, L. Xu, D. Yan, L. Jia, Z. Li, Adv. Funct. Mater. 2025, 35, 2420839.

[59]

K. Zheng, B. Tian, P. Guo, H. Zhan, J. Liang, Y. Wu, W. Wu, Chem. Eng. J. 2024, 492, 152172.

[60]

Y. Liu, Y. Wu, H. Liang, H. Xu, Y. Wei, Y. Ji, Adv. Funct. Mater. 2023, 33, 2302110.

[61]

Z. S. Davidson, H. Shahsavan, A. Aghakhani, Y. Guo, L. Hines, Y. Xia, S. Yang, M. Sitti, Sci. Adv. 2019, 5, eaay0855.

[62]

H. E. Fowler, P. Rothemund, C. Keplinger, T. J. White, Adv. Mater. 2021, 33, 2103806.

[63]

C. Zhang, G. Chen, K. Zhang, B. Jin, Q. Zhao, T. Xie, Adv. Mater. 2024, 36, 2313078.

[64]

M.-Y. Choi, K. Kim, K. Kim, S.-k. Ahn, J.-H. Na, Chem. Eng. J. 2023, 475, 146237.

[65]

R. Annapooranan, Y. Wang, S. Cai, Adv. Mater. Technol. 2023, 8, 2201969.

[66]

D. Liu, D. J. Broer, Nat. Commun. 2015, 6, 8334.

[67]

D. Liu, N. B. Tito, D. J. Broer, Nat. Commun. 2017, 8, 1526.

[68]

G. Babakhanova, T. Turiv, Y. Guo, M. Hendrikx, Q.-H. Wei, A. P. H. J. Schenning, D. J. Broer, O. D. Lavrentovich, Nat. Commun. 2018, 9, 456.

[69]

W. Feng, D. J. Broer, D. Liu, Adv. Mater. 2018, 30, 1704970.

[70]

W. Feng, D. J. Broer, L. Grebikova, C. Padberg, J. G. Vancso, D. Liu, ACS Appl. Mater. Interfaces 2019, 12, 5265.

[71]

C. Feng, C. P. H. Rajapaksha, J. M. Cedillo, C. Piedrahita, J. Cao, V. Kaphle, B. Lussem, T. Kyu, A. Jakli, Macromol. Rapid Commun. 2019, 40, e1900299.

[72]

G. Liu, Y. Deng, B. Ni, G. T. M. Nguyen, C. Vancaeyzeele, A. Brûlet, F. Vidal, C. Plesse, M. H. Li, Small 2023, 20, 2307565.

[73]

C. M. Spillmann, B. R. Ratna, J. Naciri, Appl. Phys. Lett. 2007, 90, 021911.

[74]

K. Hiraoka, M. Kobayasi, R. Kazama, H. Finkelmann, Macromolecules 2009, 42, 5600.

[75]

Y. Deng, G. Liu, A. Brûlet, G. T. M. Nguyen, D. Dudzinski, F. Vidal, C. Plesse, C. Vancaeyzeele, M. H. Li, Adv. Funct. Mater. 2024, 34, 2403892.

[76]

C.-H. Wu, M. Yoshio, J. Mater. Chem. C 2023, 11, 10154.

[77]

C.-H. Wu, W. Meng, M. Yoshio, ACS Mater. Lett. 2021, 4, 153.

[78]

C.-H. Wu, W. Meng, K. Iakoubovskii, M. Yoshio, ACS Appl. Mater. Interfaces 2023, 15, 4495.

[79]

M. Yoshio, C. H. Wu, C. Liu, Adv. Funct. Mater. 2024, 34, 2314087.

[80]

J. Liu, Z. P. Song, L. Y. Sun, B. X. Li, Y. Q. Lu, Q. Li, Responsive Mater. 2023, 1, 1, e20230005.

[81]

R. Köhler, R. Stannarius, C. Tolksdorf, R. Zentel, Appl. Phys. A. 2005, 80, 381.

[82]

W. Lehmann, H. Skupin, C. Tolksdorf, E. Gebhard, R. Zentel, P. KruÈger, M. LoÈsche, F. Kremer, Nature 2001, 410, 447.

[83]

S. M. Mirvakili, I. W. Hunter, Adv. Mater. 2017, 30, 1704407.

[84]

R. Lan, X. G. Hu, J. Chen, X. Zeng, X. Chen, T. Du, X. Song, H. Yang, Responsive Mater. 2024, 2, e20230030.

[85]

C. Ohm, M. Brehmer, R. Zentel, Adv. Mater. 2010, 22, 3366.

[86]

H. Jiang, C. Li, X. Huang, Nanoscale 2013, 5, 5225.

[87]

J. D. W. Madden, N. A. Vandesteeg, P. A. Anquetil, P. G. A. Madden, A. Takshi, R. Z. Pytel, S. R. Lafontaine, P. A. Wieringa, I. W. Hunter, Ieee. J. Oceanic. Eng. 2004, 29, 706.

[88]

D. Rus, M. T. Tolley, Nature 2015, 521, 467.

[89]

S. I. Rich, R. J. Wood, C. Majidi, Nat. Electron. 2018, 1, 102.

[90]

D. R. Yao, I. Kim, S. Yin, W. Gao, Adv. Mater. 2024, 36, 2308829.

[91]

L. Hines, K. Petersen, G. Z. Lum, M. Sitti, Adv. Mater. 2016, 29, 1603483.

[92]

C. Chen, S. Ding, J. Wang, Nat. Rev. Mater. 2024, 9, 159.

[93]

S. Huang, Y. Shen, H. K. Bisoyi, Y. Tao, Z. Liu, M. Wang, H. Yang, Q. Li, J. Am. Chem. Soc. 2021, 143, 12543.

[94]

Y.-Y. Xiao, Z.-C. Jiang, J.-B. Hou, X.-S. Chen, Y. Zhao, Soft Matter 2022, 18, 4850.

[95]

S. A. M. Weima, R. Norouzikudiani, J. Baek, J. A. Peixoto, T. K. Slot, D. J. Broer, A. DeSimone, D. Liu, Sci. Adv. 2024, 10, eadp0421.

[96]

Y. Fan, H. Geng, H. Wu, J. a. Lv, Adv. Mater. Technol. 2024, 10, 2401590.

[97]

Y. Fan, H. Wu, J. Wang, J. a. Lv, Adv. Mater. 2024, 37, 2410604.

[98]

M. Chen, X. Xing, Z. Liu, Y. Zhu, H. Liu, Y. Yu, F. Cheng, Appl. Phys. A. 2010, 100, 39.

[99]

K. Dradrach, M. Zmyslony, Z. Deng, A. Priimagi, J. Biggins, P. Wasylczyk, Nat. Commun. 2023, 14, 1877.

[100]

C. Schmidleithner, Y. You, F. Staniszewski, S. Schrittwieser, D. J. Broer, J. R. Peham, Sensor Actuat. B-chem. 2024, 412, 135820.

[101]

A. Sánchez-Ferrer, T. Fischl, M. Stubenrauch, A. Albrecht, H. Wurmus, M. Hoffmann, H. Finkelmann, Adv. Mater. 2011, 23, 4526.

[102]

Q. Liu, G. Yu, C. Zhu, B. Peng, R. Li, T. Yi, Y. Yu, Small Methods 2021, 5, 2100969.

[103]

J. A. Lv, Y. Liu, J. Wei, E. Chen, L. Qin, Y. Yu, Nature 2016, 537, 179.

[104]

J. E. Park, H. S. Kang, M. Koo, C. Park, Adv. Mater. 2020, 32, 2002178.

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