Perpendicular compensated ferrimagnetic tunnel junctions

Qi Liu , Pengfei Liu , Xiaowen Li , Shanquan Chen , Sixia Hu , Yao Wang , Zedong Xu , Songbai Hu , Mao Ye , Kaiyou Wang , Lang Chen

Microstructures ›› 2026, Vol. 6 ›› Issue (4) : 2026094

PDF
Microstructures ›› 2026, Vol. 6 ›› Issue (4) :2026094 DOI: 10.20517/microstructures.2026.88
Research Article
Perpendicular compensated ferrimagnetic tunnel junctions
Author information +
History +
PDF

Abstract

Combining the advantages of ferromagnetic and antiferromagnetic tunnel junctions, ferrimagnetic tunnel junctions are highly desirable for spintronic applications. Here, we design and experimentally demonstrate a novel type of perpendicular compensated ferrimagnetic tunnel junction composed of the ferrimagnetic oxide NiCo2O4 and the compensated ferrimagnetic alloy Co100-xGdx separated by an MgAl2O4 insulating barrier. The tunneling magnetoresistance undergoes a sign transition from positive to negative (from +72% to -22%) as the temperature increases across the magnetization compensation point of Co100-xGdx, which is attributed to the reversible magnetic dominance between the Co and Gd sublattices. Furthermore, we employ this ferrimagnetic tunnel junction to realize temperature-dependent non-volatile multilevel states. Our findings on the perpendicular compensated ferrimagnetic tunnel junctions can provide an attractive avenue for developing ferrimagnet-based devices.

Keywords

Ferrimagnetic tunnel junctions / perpendicular magnetic anisotropy / non-volatile

Cite this article

Download citation ▾
Qi Liu, Pengfei Liu, Xiaowen Li, Shanquan Chen, Sixia Hu, Yao Wang, Zedong Xu, Songbai Hu, Mao Ye, Kaiyou Wang, Lang Chen. Perpendicular compensated ferrimagnetic tunnel junctions. Microstructures, 2026, 6 (4) : 2026094 DOI:10.20517/microstructures.2026.88

登录浏览全文

4963

注册一个新账户 忘记密码

References

[1]

Yuasa S,Fukushima A,Ando K.Giant room-temperature magnetoresistance in single-crystal Fe/MgO/Fe magnetic tunnel junctions.Nat Mater2004;3:868-71

[2]

Yang H,Chshiev M.Two-dimensional materials prospects for non-volatile spintronic memories.Nature2022;606:663-73

[3]

Cai K,Ju H.Electric field control of deterministic current-induced magnetization switching in a hybrid ferromagnetic/ferroelectric structure.Nat Mater2017;16:712-6

[4]

Cao Y,Edmonds KW,Zheng H.Deterministic magnetization switching using lateral spin-orbit torque.Adv Mater2020;32:e1907929

[5]

Cao Y,Sheng Y,Wang K.Tuning a binary ferromagnet into a multistate synapse with spin-orbit-torque-induced plasticity.Adv Funct Mater2019;29:1808104

[6]

Xue F,Ma Y.Integrated memory devices based on 2D materials.Adv Mater2022;34:e2201880

[7]

Gurung G,Luo QQ,Tsymbal EY.Nearly perfect spin polarization of noncollinear antiferromagnets.Nat Commun2024;15:10242 PMCID:PMC11599937

[8]

Shao D.Antiferromagnetic tunnel junctions for spintronics.npj Spintronics2024;2:14

[9]

Echtenkamp W,Yang Y.Prospects of electric field control in perpendicular magnetic tunnel junctions and emerging 2D spintronics for ultralow energy memory and logic devices.Adv Funct Mater2026;36:2505426

[10]

Freeman MR.Advances in magnetic microscopy.Science2001;294:1484-8

[11]

Zhou S,Liu Y.Modelling of magnetic stray fields in multilayer magnetic films with in-plane or perpendicular anisotropy.Magnetochemistry2022;8:159

[12]

De Ranieri E,Fang D.Piezoelectric control of the mobility of a domain wall driven by adiabatic and non-adiabatic torques.Nat Mater2013;12:808-14

[13]

Kimel AV,Pisarev RV,Kirilyuk A.Inertia-driven spin switching in antiferromagnets.Nat Phys2009;5:727-31

[14]

Han J,Liu L,Fukami S.Coherent antiferromagnetic spintronics.Nat Mater2023;22:684-95

[15]

Kim KJ,Hirata Y.Fast domain wall motion in the vicinity of the angular momentum compensation temperature of ferrimagnets.Nat Mater2017;16:1187-92

[16]

Kim C,Kim HG.Distinct handedness of spin wave across the compensation temperatures of ferrimagnets.Nat Mater2020;19:980-5

[17]

Din A,Wadley P.Antiferromagnetic spintronics and beyond.npj Spintronics2024;2:29

[18]

Kim SK,Lee KJ,Rasing T.Ferrimagnetic spintronics.Nat Mater2022;21:24-34

[19]

Ishibashi M,Kawaguchi M,Nakatsuji S.Ferrimagnetic compensation and its thickness dependence in TbFeCo alloy thin films.Appl Phys Lett2022;120:022405

[20]

Finley J.Spintronics with compensated ferrimagnets.Appl Phys Lett2020;116:110501

[21]

Kiphart D,Stobiecki F,Matczak M.Tailoring ferrimagnetic properties using proximity effects in Co/Tb-Co bilayers.Adv Mater Interfaces2025;12:e00330

[22]

Ueda K,de Brouwer PWP,Beach GSD.Temperature dependence of spin-orbit torques across the magnetic compensation point in a ferrimagnetic TbCo alloy film.Phys Rev B2017;96:064410

[23]

Wang J,An Y,Zhang S.Interplay between magnetization compensation temperature and thickness in ferrimagnetic CoGd alloy films.Appl Phys Lett2025;126:072401

[24]

Xu T,Dong Y.Evolution of compensated magnetism and spin-torque switching in ferrimagnetic Fe1-xTbx.Phys Rev Appl2023;19

[25]

Mishra R,Qiu X,Venkatesan T.Anomalous current-induced spin torques in ferrimagnets near compensation.Phys Rev Lett2017;118:167201

[26]

Li Y,Zhu W.Spin-canting mediated anomalous nernst effect in ferrimagnetic CoTb films.Chinese Phys Lett2026;43:020708

[27]

Kaiser C,Parkin SS.Finite tunneling spin polarization at the compensation point of rare-earth-metal-transition-metal alloys.Phys Rev Lett2005;95:047202

[28]

Zhu W,Pan C.Sign-tunable magnetic tunnel junctions engineered via ferrimagnets for efficient all-electrical and thermal switching.Adv Funct Mater2026;36:2505415

[29]

Jiang X,Sun JZ.Temperature dependence of current-induced magnetization switching in spin valves with a ferrimagnetic CoGd free layer.Phys Rev Lett2006;97:217202

[30]

Shen Y,Lin I,Suzuki I.Perpendicular magnetic tunnel junctions based on half-metallic NiCo2O4.Appl Phys Lett2020;117:042408

[31]

Brinkman WF,Rowell JM.Tunneling conductance of asymmetrical barriers.J Appl Phys1970;41:1915-21

[32]

Miller CW,Schuller IK,Slaughter JM.Dynamic spin-polarized resonant tunneling in magnetic tunnel junctions.Phys Rev Lett2007;99:047206

[33]

Santos TS,Migdal P,Satpati B.Room-temperature tunnel magnetoresistance and spin-polarized tunneling through an organic semiconductor barrier.Phys Rev Lett2007;98:016601

[34]

Kaiser B,Norum M,Dewey J.Optimizing nonlocal spin valves via wide-range interfacial-resistance tuning: Toward spin-accumulation sensors.Phys Rev Appl2024;22

[35]

Oliver B.Temperature and bias dependence of dynamic conductance-low resistive magnetic tunnel junctions.J Appl Phys2004;95:546-50

[36]

Kresse G.Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set.Phys Rev B1996;54:11169-86

[37]

Sun J,Perdew JP.Strongly constrained and appropriately normed semilocal density functional.Phys Rev Lett2015;115:036402

[38]

Vasiukov DM,Wen F.Epitaxial stabilization of thin films of the frustrated Ge-based spinels.Phys Rev Mater2021;5:064419

[39]

Liu Q,Zhu Y.Oxygen controlled perpendicular magnetic anisotropy in LaCoO3-δ/La0.7Sr0.3MnO3/LaCoO3-δ heterostructures.Appl Phys Lett2022;120:242902

[40]

Liu Q,Li X.Perpendicular manganite magnetic tunnel junctions induced by interfacial coupling.ACS Appl Mater Interfaces2022;14:13883-90

[41]

Chen X,Han MG.Magnetotransport anomaly in room-temperature ferrimagnetic NiCo2O4 thin films.Adv Mater2019;31:e1805260

[42]

Kan D,Kitamura M.Spin and orbital magnetic moments in perpendicularly magnetized Ni1-xCo2+yO4-z epitaxial thin films: effects of site-dependent cation valence states.Phys Rev B2020;101:224434

[43]

Bitla Y,Lin JC.Origin of metallic behavior in NiCo2O4 ferrimagnet.Sci Rep2015;5:15201 PMCID:PMC4606736

[44]

Siddiqui SA,Finley JT,Liu L.Current-induced domain wall motion in a compensated ferrimagnet.Phys Rev Lett2018;121:057701

[45]

Meo A,Darwin E.Spin-wave eigenmodes in nanoscale magnetic tunnel junctions with perpendicular magnetic anisotropy.Phys Rev Appl2025;23:034086

[46]

Chen D,Tong S.Noncollinear spin state and unusual magnetoresistance in ferrimagnet Co-Gd.Phys Rev Materials2022;6:014402

[47]

Park J,Kang J.Unconventional magnetoresistance induced by sperimagnetism in GdFeCo.Phys Rev B2021;103:014421

[48]

Shen Y,Tan Z,Shimakawa Y.Tuning of ferrimagnetism and perpendicular magnetic anisotropy in NiCo2O4 epitaxial films by the cation distribution.Phys Rev B2020;101:094412

[49]

Rivas-Murias B,Jiménez-Cavero P,Morellón L.Independent control of the magnetization in ferromagnetic La2/3Sr1/3MnO3/SrTiO3/LaCoO3 heterostructures achieved by epitaxial lattice mismatch.Nano Lett2016;16:1736-40

[50]

Wu H,Zhang P.Magnetic memory driven by topological insulators.Nat Commun2021;12:6251 PMCID:PMC8556271

[51]

Currivan-Incorvia JA,Dutta S.Logic circuit prototypes for three-terminal magnetic tunnel junctions with mobile domain walls.Nat Commun2016;7:10275 PMCID:PMC4729928

[52]

Bartolomé J,Kazak NV.Uniaxial magnetic anisotropy in Co2.25Fe0.75O2BO3 compared to Co3O2BO3 and Fe3O2BO ludwigites.Phys Rev B2011;83:144426

[53]

Kou X,Wang J.Metal-to-insulator switching in quantum anomalous Hall states.Nat Commun2015;6:8474 PMCID:PMC4633736

[54]

Liu L,Lin W.Current-induced magnetization switching in all-oxide heterostructures.Nat Nanotechnol2019;14:939-44

[55]

Hurd CM.The hall effect in metals and alloys. Springer Science & Business Media, 2012.

[56]

Chang TC,Lee CH.The effect of degrees of inversion on the electronic structure of spinel NiCo2O4: a density functional theory study.ACS Omega2021;6:9692-9

PDF

2

Accesses

0

Citation

Detail

Sections
Recommended

/

〈 〉