Pore structure characteristics of low-rank coal reservoirs with different ash yields and their implications for recoverability of coalbed methane—a case study from the Erlian Basin, northeastern China

Dawei DONG, Jiaosheng YANG, Qiujia HU, Shitao CUI, Fenjin SUN, Jidong ZHANG, Xinrui CUI

PDF(4232 KB)
PDF(4232 KB)
Front. Earth Sci. ›› 2023, Vol. 17 ›› Issue (1) : 18-29. DOI: 10.1007/s11707-022-1015-0
RESEARCH ARTICLE
RESEARCH ARTICLE

Pore structure characteristics of low-rank coal reservoirs with different ash yields and their implications for recoverability of coalbed methane—a case study from the Erlian Basin, northeastern China

Author information +
History +

Abstract

Pores are the main accumulation sites and migration pathways for coalbed methane (also referred to as CBM). Pore structure restricts the content and recoverability of CBM from coal reservoirs. In this study, 12 representative coal samples with different ash yields that have similar tectonic characteristics and burial depths were collected from different mining areas in the Jiergalangtu and Huolinhe depressions in the Erlian Basin. These samples were used to study the restrictions of ash yield on the characteristics of coal pore structures and the recoverability of CBM through macroscopic and microscopic structure observation, scanning electron microscope observations, vitrinite reflectance tests, low-temperature N2 adsorption, nuclear magnetic resonance (NMR), and micro-computed tomography. The results show that coal reservoirs in the study area vary greatly in ash yield, based on which they can be divided into three types, i.e., low-ash-content, ash-bearing, and high-ash-content coal reservoirs. In addition, the ash yield has a certain impact on the development of coal pores; coal samples with lower ash yields indicate the presence of well-developed medium-large pores and better connectivity. Ash yield also has a certain impact on the brittleness of coal wherein a lower ash yield implies the development of brittle coal that is more liable to fracture as compared to less brittle samples at the same pressure. Absorbed gas content also varies significantly with ash yield; a low ash yield impacts the gas saturation of coal. Overall, for coal reservoirs in the study area, their porosity, pore diameter, movable fluid porosity, adsorbed gas amount, and recoverability decrease as the ash yield increases.

Graphical abstract

Keywords

coal reservoir / ash / pore structure / recoverability / Erlian Basin

Cite this article

Download citation ▾
Dawei DONG, Jiaosheng YANG, Qiujia HU, Shitao CUI, Fenjin SUN, Jidong ZHANG, Xinrui CUI. Pore structure characteristics of low-rank coal reservoirs with different ash yields and their implications for recoverability of coalbed methane—a case study from the Erlian Basin, northeastern China. Front. Earth Sci., 2023, 17(1): 18‒29 https://doi.org/10.1007/s11707-022-1015-0

References

[1]
Cai Y D, Liu D M, Pan Z J, Che Y, Liu Z H (2016). Investigating the effects of seepage-pores and fractures on coal permeability by fractal analysis.Transp Porous Media, 111(2): 479–497
CrossRef Google scholar
[2]
Cai Y D, Liu D M, Pan Z J, Yao Y B, Li J Q, Qiu Y K (2014). Pore structure of selected Chinese coals with heating and pressurization treatments.Sci China Earth Sci, 57(7): 1567–1582
CrossRef Google scholar
[3]
Clarkson C R, Bustin R M (1999). The effect of pore structure and gas pressure upon the transport properties of coal: a laboratory and modeling study. 2. Adsorption rate modeling.Fuel, 78(11): 1345–1362
CrossRef Google scholar
[4]
Clarkson C R, Solano N, Bustin R M, Bustin A M M, Chalmers G R L, He L, Melnichenko Y B, Radlinski A P, Blach T P (2013). Pore structure characterization of North American shale gas reservoirs using USANS/SANS, gas adsorption, and mercury intrusion.Fuel, 103: 606–616
CrossRef Google scholar
[5]
Fu H J, Tang D Z, Xu T, Xu H, Tao S, Li S, Yin Z Y, Chen B L, Zhang C, Wang L L (2017). Characteristics of pore structure and fractural dimension of low-rank coal: a case study of Lower Jurassic Xishayao coal in the southern Junggar Basin, NW China.Fuel, 193: 254–264
CrossRef Google scholar
[6]
FuX H, QinY, WeiC T (2007). Coalbed Methane Geology. Xuzhou: China University of Mining and Technology Press (in Chinese)
[7]
Golab A, Ward C R, Permana A, Lennox P, Botha P (2013). High-resolution three-dimensional imaging of coal using microfocus X-ray computed tomography, with special reference to modes of mineral occurrence.Int J Coal Geol, 113: 97–108
CrossRef Google scholar
[8]
Harris L A, Yust C S (1976). Transmisssion electron microscope observations of porosity in coal.Fuel, 55(3): 233–236
CrossRef Google scholar
[9]
Hou S H, Wang X M, Wang X J, Yuan Y D, Pan S, Wang X (2017). Pore structure characterization of low volatile bituminous coals with different particle size and tectonic deformation using low pressure gas adsorption.Int J Coal Geol, 183: 1–13
CrossRef Google scholar
[10]
Huang T, Liu Z (2019). Analysis on pore structure characteristics and influencing factors of coal reservoir in Yushe-Wuxiang Block.Coal Sci Technol, 47(7): 227–233
[11]
Jia T F, Wang M, Gao X Y, Zhao J G, Zhu J Q (2021). Pore structure characteristics of low-rank coal reservoirs and evaluation of fractal models.Nat Gas Geosci, 32(3): 423–436
[12]
JiangW P, SongX Z, ZhongL W (2011). Research on the pore properties of different coal body structure coals and the effects on gas outburst based on the low-temperature nitrogen adsorption method. China Coal Soc, 36(4): 609–614 (in Chinese)
[13]
Jing Y, Armstrong R T, Mostaghimi P (2017). Digital coal: generation of fractured cores with microscale features.Fuel, 207: 93–101
CrossRef Google scholar
[14]
Jing Y, Armstrong R T, Ramandi H L, Mostaghimi P (2016). Coal cleat reconstruction using micro-computed tomography imaging.Fuel, 181: 286–299
CrossRef Google scholar
[15]
Jiu B, Huang W H, Shi J, Hao R L (2021). A method to extract the content, radius and specific surface area of maceral compositions in coal reservoirs based on image modeling.J Petrol Sci Eng, 201: 108419
CrossRef Google scholar
[16]
Kang J Q, Fu X H, Li X, Liang S (2019). Nitrogen injection to enhance methane and water production: an experimental study using the LF-NMR relaxation method.Int J Coal Geol, 211: 103228
CrossRef Google scholar
[17]
Li S, Tang D Z, Xu H, Yang Z (2012). The pore-fracture system properties of coalbed methane reservoirs in the Panguan Syncline, Guizhou, China.Geosci Front, 3(6): 853–862
CrossRef Google scholar
[18]
LiZ T (2018). Evolution of Pore-fractures of Coal Reservoir and Its Impact on CBM Microcosmic Flow. Dissertation for Doctor Degree. Beijing: China University of Geosciences (Beijing) (in Chinese)
[19]
Li Z T, Liu D M, Cai Y D, Ranjith P G, Yao Y B (2017). Multi-scale quantitative characterization of 3-D pore-fracture networks in bituminous and anthracite coals using FIB-SEM tomography and X-ray μ-CT.Fuel, 209: 43–53
CrossRef Google scholar
[20]
Li Z T, Liu D M, Cai Y D, Shi T L (2016). Investigation of methane diffusion in low-rank coals by a multiparous diffusion model.J Nat Gas Sci Eng, 33: 97–107
CrossRef Google scholar
[21]
Liu D M, Liu Z H, Cai Y D (2020a). Research progress on accumulation mechanism and formation geological conditions of coalbed methane.Coal Sci Technol, 48(10): 1–16
[22]
Liu D M, Wang Y J, Cai Y D (2018). Analysis of main geological controls on coalbed methane enrichment and accumulation patterns in low rank coals.Coal Sci Technol, 46(6): 1–8
[23]
Liu H H, Farid I I, Sang S X, Shang J H, Wu H Y, Xu H J, Zhang P S, Liu Q M (2020b). Synthetical study on the difference and reason for the pore structure of the No.3 coal reservoir from the southern Qinshui Basin, China, using mercury intrusion porosimetry, low-temperature N2 adsorption, low field nuclear magnetic resonance, and nuclear magnetic resonance cryoporometry.Energy Rep, 6: 1876–1887
CrossRef Google scholar
[24]
Liu H H, Sang S X, Wang G G, Li M, Xu H, Liu S, Li J, Ren B, Zhao Z, Xie Y (2014). Block scale investigation on gas content of coalbed methane reservoirs in southern Qinshui Basin with statistical model and visual map.J Petrol Sci Eng, 114: 1–14
CrossRef Google scholar
[25]
LiuJ H, WangS W, SuD M (2021). Study on pore development characteristics of low rank coal reservoirs in Erlian Basin group. Safety Coal Mines, 52(2): 7–12 (in Chinese)
[26]
Liu S Q, Sang S X, Wang G, Ma J S, Wang X, Wang W F, Du Y, Wang T (2017). FIB-SEM and X-ray CT characterization of interconnected pores in high-rank coal formed from regional metamorphism.J Nat Gas Sci Eng, 148: 21–31
[27]
MengY J, TangD Z, XuH, GanQ, YanT T (2020). Identifying the key factor of medium-rank coalbed methane productivity with gray relational analysis: a case study in Liulin area, Ordos Basin, China. Energy Sources A Recovery Util Environ Effects: 1–14
CrossRef Google scholar
[28]
Meng Y J, Tang D Z, Xu H, Li C, Li L, Meng S Z (2014). Geological controls and coalbed methane production potential evaluation: a case study in Liulin area, eastern Ordos Basin, China.J Nat Gas Sci Eng, 21: 95–111
CrossRef Google scholar
[29]
Meyers R A (1982). Coal Structure. New York: Academic Press
[30]
Nie B S, Liu X F, Yang L, Meng J, Li X (2015). Pore structure characterization of different rank coals using gas adsorption and scanning electron microscopy.Fuel, 158: 908–917
CrossRef Google scholar
[31]
Okolo G N, Everson R C, Neomagus H W J P, Roberts M J, Sakurovs R (2015). Comparing the porosity and surface areas of coal as measured by gas adsorption, mercury intrusion and SAXS techniques.Fuel, 141: 293–304
CrossRef Google scholar
[32]
Sakurovs R, He L L, Melnichenko Y B, Radlinski A P, Blach T, Lemmel H, Mildner D F R (2012). Pore size distribution and accessible pore size distribution in bituminous coals.Int J Coal Geol, 100: 51–64
CrossRef Google scholar
[33]
SongX X, TangL W, LiW, ZengF G, XiangJ H (2014). Pore structure in tectonically deformed coals by small angle X-ray scattering. J China Coal Soc, 39(4): 719–724 (in Chinese)
[34]
Sun F J, Li W Z, Sun Q P, Sun B, Tian W G, Chen Y J, Chen Z H (2017). Low-rank coalbed methane exploration in Jiergalangtu Sag, Erlian basin.Acta Petrol Sin, 38(2): 485–492
[35]
Wang A M, Wei Y C, Yuan Y, Li C F, Li Y, Cao D Y (2017). Coalbed methane reservoir’s pore-structure characterization of different macrolithotypes in the southern Junggar Basin of northwest China.Mar Pet Geol, 86: 675–688
CrossRef Google scholar
[36]
WangT, DengZ, HuH Y, Cao M L, ZhangB X, JiaoP F, YuZ (2019). Study on characteristics comparison of low rank coal coalbed methane reservoirs at home and abroad. Coal Sci Technol, 47(9): 41–50 (in Chinese)
[37]
WangY Z(2020). Fractal characteristics of coal rock pores in the Baliancheng Mining Area, Hunchun Basin. J Southwest Petrol U (Sci & Tech Edi), 42(1): 57–68 (in Chinese)
[38]
Wang Y, Mao C (2021). Nano/micro pore structure and fractal characteristics of Baliancheng Coalfield in Hunchun Basin.J Nanosci Nanotechnol, 21(1): 682–692
CrossRef Pubmed Google scholar
[39]
Watanabe N, Ishibashi T, Hirano N, Tsuchiya N, Ohsaki Y, Tamagawa T, Tsuchiya Y, Okabe H (2011). Precise 3D numerical modeling of fracture flow coupled with X-ray computed tomography for reservoir core samples.SPE J, 16(3): 683–691
CrossRef Google scholar
[40]
YangF, HeD, MaD M, Duan Z H, TianT, FuD L (2020). Multi-scale joint characterization of micro-pore structure of low-rank coal reservoir. Lithologic Reservoirs, 32(3): 14–23 (in Chinese)
[41]
YaoH P, LvW B, WangK F, Li L, LiW H, LinH T, LiF C, LiZ (2020). Key geological factors and evaluation methods for huge low-rank coalbed methane reservoirs: taking Bayanhua depression in Erlian basin as an example. Coal Geo Explor, 48(1): 85–95 (in Chinese)
[42]
Yao Y B, Liu D M (2012). Comparison of low-field NMR and mercury intrusion porosimetry in characterizing pore size distributions of coals.Fuel, 95: 152–158
CrossRef Google scholar
[43]
Yao Y B, Liu D M, Che Y, Tang D Z, Tang S H, Huang W H (2010). Petrophysical characterization of coals by low-field nuclear magnetic resonance (NMR).Fuel, 89(7): 1371–1380
CrossRef Google scholar
[44]
Yao Y B, Liu D M, Tang D Z, Tang S H, Huang W H (2008). Fractal characterization of adsorption-pores of coals from north China: an investigation on CH4 adsorption capacity of coals.Int J Coal Geol, 73(1): 27–42
CrossRef Google scholar
[45]
Yao Y B, Liu D M, Tang D Z, Tang S H, Huang W H, Liu Z H, Che Y (2009). Fractal characterization of seepage-pores of coals from China: an investigation on permeability of coals.Comput Geosci, 35(6): 1159–1166
CrossRef Google scholar
[46]
Zhang J J, Wei C T, Ju W, Yan G Y, Lu G W, Hou X W, Kai Z (2019a). Stress sensitivity characterization and heterogeneous variation of the pore-fracture system in middle-high rank coals reservoir based on NMR experiments.Fuel, 238: 331–344
CrossRef Google scholar
[47]
Zhang J J, Wei C, Vandeginste V, Ju W, Qin Z, Quan F, Soh Tamehe L (2019b). Experimental simulation study on water migration and methane depressurizing desorption based on nuclear magnetic resonance technology: a case study of middle-rank coals from the Panguan syncline in the western Guizhou region.Energy Fuels, 33(9): 7993–8006
CrossRef Google scholar
[48]
ZhaoD F, GuoY H, MaoX X, Lu C G, LiM, QianF C (2017a). Characteristics of macro-nanopores in anthracite coal based on mercury injection, nitrogen adsorption and FE-SEM. J China Coal Soc, 42(6): 1517–1526 (in Chinese)
[49]
Zhao J L, Xu H, Tang D Z, Mathews J P, Li S, Tao S (2016). A comparative evaluation of coal specific surface area by CO2 and N2 adsorption and its influence on CH4 adsorption capacity at different pore sizes.Fuel, 183: 420–431
CrossRef Google scholar
[50]
Zhao X Z, Liu G D, Jin F M, Huang Z L, Lu X J, Sun M L, Ding X J, Chen Z L (2015). Distribution features and pattern of effective source rock in small faulted lacustrine basin: a case study of the Lower Cretaceous in Erlian Basin.Acta Petrol Sin, 36(6): 641–652
[51]
Zhao Y X, Liu S M, Elsworth D, Jiang Y D, Zhu J (2014). Pore structure characterization of coal by synchrotron small-angle X ray scattering and transmission electron microscopy.Energy Fuels, 28(6): 3704–3711
CrossRef Google scholar
[52]
Zhao Y X, Sun Y F, Liu S M, Wang K, Jiang Y D (2017b). Pore structure characterization of coal by NMR cryoporometry.Fuel, 190: 359–369
CrossRef Google scholar
[53]
Zheng S J, Yao Y B, Liu D M, Cai Y D, Liu Y (2018). Characterizations of full-scale pore size distribution, porosity and permeability of coals: a novel methodology by nuclear magnetic resonance and fractal analysis theory.Int J Coal Geol, 196: 148–158
CrossRef Google scholar
[54]
Zhou S D, Liu D M, Cai Y D, Yao Y B, Li Z T (2017). 3D characterization and quantitative evaluation of pore-fracture networks of two Chinese coals using FIB-SEM tomography.Int J Coal Geol, 174: 41–54
CrossRef Google scholar
[55]
ZhouY L, LiuN, LiuQ R (2011). Plant Biology. Beijing: Higher Education Press (in Chinese)
[56]
Zhu J F, Liu J Z, Yang Y M, Cheng J, Zhou J H, Cen K F (2016). Fractal characteristics of pore structures in 13 coal specimens: relationship among fractal dimension, pore structure parameter, and slurry ability of coal.Fuel Process Technol, 149: 256–267
CrossRef Google scholar

Acknowledgments

This study was financially supported by the National Natural Science Foundation of China (Grant No. 42072162), the Natural Science Foundation of Shandong Province (No. ZR2020MD036), and a forward-looking and basic technology research project of PetroChina (No. 2021DJ2301).

RIGHTS & PERMISSIONS

2023 Higher Education Press
AI Summary AI Mindmap
PDF(4232 KB)

Accesses

Citations

Detail

Sections
Recommended

/