A Supported Palladium on Gallium-based Liquid Metal Catalyst for Enhanced Oxygen Reduction Reaction

Chunrong Ma; Bingyi Song; Zhentao Ma; Xiaoqian Wang; Lin Tian; Haoran Zhang; Cai Chen; Xusheng Zheng; Li-ming Yang; Yuen Wu

doi:10.1007/s40242-022-2092-z

Chemical Research in Chinese Universities ›› 2022, Vol. 38 ›› Issue (5) : 1219 -1225. DOI: 10.1007/s40242-022-2092-z

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A Supported Palladium on Gallium-based Liquid Metal Catalyst for Enhanced Oxygen Reduction Reaction

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Abstract

Developing high-performance catalysts for oxygen reduction reaction to replace costly platinum-based materials is of great importance but still confronted with challenges. Herein, a kind of supported palladium liquid metal catalyst, which is prepared by galvanic replacement, surpasses commercial Pt/C and Pd/C in oxygen reduction catalysis with a higher half-wave potential of 0.92 V, mass activity of 1.85 A/mg_Pd at 0.90 V, and superior durability. The liquid metal support can both optimize the electronic structures of Pd sites and guarantee the dispersion of Pd atoms, which explains the enhanced activity and durability, respectively. This work opens an avenue for rational design of catalysts.

Keywords

Liquid metal / Supported catalyst / Oxygen reduction / Electrocatalysis

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Chunrong Ma, Bingyi Song, Zhentao Ma, Xiaoqian Wang, Lin Tian, Haoran Zhang, Cai Chen, Xusheng Zheng, Li-ming Yang, Yuen Wu. A Supported Palladium on Gallium-based Liquid Metal Catalyst for Enhanced Oxygen Reduction Reaction. Chemical Research in Chinese Universities, 2022, 38(5): 1219-1225 DOI:10.1007/s40242-022-2092-z

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