Microstructure Manipulation of Covalent Organic Frameworks (COFs)-based Membrane for Efficient Separations

Hanze Ma; Shaoyu Wang; Yanxiong Ren; Xu Liang; Yuhan Wang; Ziting Zhu; Guangwei He; Zhongyi Jiang

doi:10.1007/s40242-022-1474-6

Chemical Research in Chinese Universities ›› 2022, Vol. 38 ›› Issue (2) : 325 -338. DOI: 10.1007/s40242-022-1474-6

Review

Microstructure Manipulation of Covalent Organic Frameworks (COFs)-based Membrane for Efficient Separations

Hanze Ma ¹^,²
, Shaoyu Wang ¹^,²
, Yanxiong Ren ¹^,²^,³
, Xu Liang ¹^,²
, Yuhan Wang ¹^,²
, Ziting Zhu ¹^,²
, Guangwei He ¹^,²^,^g
, Zhongyi Jiang ¹^,²^,³^,^h

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Abstract

Covalent organic framework(COF) membranes have exhibited great potential to become the next-generation membranes for efficient separations due to the diverse structures, ordered framework pores, tunable functionality and excellent stability. This review presents the microstructure manipulation strategies for separation performance enhancement of COF membranes in recent years. Based on the three mechanisms of molecular sieving, surface diffusion, and facilitated transport, the structural modulation methods to enhance the selectivity of COF membranes are analyzed in detail. Next, strategies of realizing ultrashort mass transfer pathways and ultralow mass transfer resistance for the permeability enhancement are elaborated. Furthermore, the framework stability in COFs, interlayer stability between COF nanosheets and interfacial stability between COF layer and substrate are discussed. Finally, we discuss the existing challenges and perspectives on the future development of COF membranes, targeting at identifying the most promising strategies and directions for the engineering of COF membranes.

Keywords

Covalent organic framework / Organic molecular sieve membrane / Membrane separation / Microporous material

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Hanze Ma, Shaoyu Wang, Yanxiong Ren, Xu Liang, Yuhan Wang, Ziting Zhu, Guangwei He, Zhongyi Jiang. Microstructure Manipulation of Covalent Organic Frameworks (COFs)-based Membrane for Efficient Separations. Chemical Research in Chinese Universities, 2022, 38(2): 325-338 DOI:10.1007/s40242-022-1474-6

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