Ivy-Inspired Double-Spiral Gel Fibers with Multifunctional Sensing and Electromagnetic Interference Shielding Properties Toward Wearable Health Care and Monitoring

Li Chen , Guifen Sun , Jingle Duan , Peng Wang , Chuizhou Meng

Advanced Fiber Materials ›› : 1 -18.

PDF
Advanced Fiber Materials ›› :1 -18. DOI: 10.1007/s42765-026-00711-4
Research Article
research-article
Ivy-Inspired Double-Spiral Gel Fibers with Multifunctional Sensing and Electromagnetic Interference Shielding Properties Toward Wearable Health Care and Monitoring
Author information +
History +
PDF

Abstract

Flexible sensors with multi-mode sensing capability are highly desired for wearable health monitoring; meanwhile, electromagnetic interference (EMI) shielding is also needed for the special health care of pregnant women and children. Herein, inspired by the helical structure of natural ivy, multifunctional double-spiral gel fibers are developed through a facial wet spinning-intertwining method. The conducting polymer-incorporated sodium polyacrylate polymer matrix serves as the adhesive and conductive hydrogel substrate, while different conductive fillers of carbon nanotubes (CNTs) and silver nanowires (AgNWs) are composited in each fiber for mutual synergistic effect. Due to the combined electrical conducting behaviors of CNTs and AgNWs, remarkable strain-sensing performance (sensitivity approximately 70.12) for single double-spiral fibers and effective EMI shielding property (total shielding effectiveness approximately 21.9 dB) for woven textiles are achieved. Because of differentiated triboelectric polarities of CNTs and AgNWs, the double-spiral fibers can also be used as a noncontact triboelectric nanogenerator sensor (sensitivity approximately -4.6 mV mm−1). The practicality of the developed multifunctional double-spiral gel fibers is comprehensively demonstrated to detect various body joint and limb motions, monitor chest and wrist electrocardiogram signal, recognize nearby object material type with the help of artificial intelligence, and shield EMI from Bluetooth headset.

Graphical Abstract

Keywords

Double-spiral fibers / Hydrogels / Strain sensor / Noncontact triboelectric sensor / Electromagnetic interference (EMI) shielding

Cite this article

Download citation ▾
Li Chen, Guifen Sun, Jingle Duan, Peng Wang, Chuizhou Meng. Ivy-Inspired Double-Spiral Gel Fibers with Multifunctional Sensing and Electromagnetic Interference Shielding Properties Toward Wearable Health Care and Monitoring. Advanced Fiber Materials 1-18 DOI:10.1007/s42765-026-00711-4

登录浏览全文

4963

注册一个新账户 忘记密码

References

[1]

Zhang P, Wang W, Ma Y, Zhang H, Zhou D, Ji X, Liu W, Liu Y, Zhang D. MXene-based self-adhesive, ultrasensitive, highly tough flexible hydrogel pressure sensors for motion monitoring and robotic tactile sensing. Chem Eng J, 2024, 499 156173

[2]

Wang Y, Qin W, Yang M, Tian Z, Guo W, Sun J, Zhou X, Fei B, An B, Sun R, Yin S, Liu Z. High linearity, low hysteresis Ti3C2Tx MXene/AgNW/liquid metal self-healing strain sensor modulated by dynamic disulfide and hydrogen bonds. Adv Funct Mater, 2023, 33 2301587

[3]

Zhao C, Fang Y, Chen H, Zhang S, Wan Y, Riaz MS, Zhang Z, Dong W, Diao L, Ren D, Huang F. Ultrathin Mo2S3 nanowire network for high-sensitivity breathable piezoresistive electronic skins. ACS Nano, 2023, 17: 4862-4870

[4]

Cui Y, He X, Liu W, Zhu S, Zhou M, Wang Q. Highly stretchable, sensitive, and multifunctional thermoelectric fabric for synergistic-sensing systems of human signal monitoring. Adv Fiber Mater, 2024, 6: 170-180

[5]

Su T, Liu N, Gao Y, Lei D, Wang L, Ren Z, Zhang Q, Su J, Zhang Z. MXene/cellulose nanofiber-foam based high performance degradable piezoresistive sensor with greatly expanded interlayer distances. Nano Energy, 2021, 87 106151

[6]

Wang Y-Q, Cao M, Liu B-W, Zeng F-R, Fu Q, Zhao H-B, Wang Y-Z. Controllable proton-reservoir ordered gel towards reversible switching and reliable electromagnetic interference shielding. Mater Horiz, 2024, 11: 978-987

[7]

Zeng Z, Wang G, Wolan BF, Wu N, Wang C, Zhao S, Yue S, Li B, He W, Liu J, Lydng JW. Printable aligned single-walled carbon nanotube film with outstanding thermal conductivity and electromagnetic interference shielding performance. Nano-Micro Lett, 2022, 14 179

[8]

Chen T, Cai J, Cheng X, Cui S, Zhang D, Gong D. Bio-inspired flexible versatile textiles for excellent absorption-dominated electromagnetic interference shielding, thermal management, and strain sensing. Chem Eng J, 2023, 477 147116

[9]

Zhang Z, Liu G, Wu J, Jiang X, Liu H, Li Z. High-strength dual-network hydrogels with chain-growth enhancement for multifunctional flexible sensors, triboelectric nanogenerators, and EMI shielding. Chem Eng J, 2025, 519 165710

[10]

Wang W, Liu J, Li H, Zhao Y, Wan R, Wang Q, Xu J, Lu B. Photopatternable PEDOT:PSS hydrogels for high-resolution photolithography. Adv Sci, 2025, 12 2414834

[11]

Wu R, Zhu T, Ni Y, Wu C, Wang W, Zhao K, Huang J, Lai Y. UV-Cured dense double network hydrogel via multiple dynamic crosslinking for stable amphibious motion sensing. Adv Funct Mater, 2025, 36 e15120

[12]

Wang H, Zhuang T, Wang J, Sun X, Wang Y, Li K, Dai X, Guo Q, Li X, Chong D, Chen B, Yan J. Multifunctional filler-free PEDOT:PSS hydrogels with ultrahigh electrical conductivity induced by Lewis-Acid-promoted ion exchange. Adv Mater, 2023, 35 2302919

[13]

He X, Zhang B, Liu Q, Chen H, Cheng J, Jian B, Yin H, Li H, Duan K, Zhang J, Ge Q. Highly conductive and stretchable nanostructured ionogels for 3D printing capacitive sensors with superior performance. Nat Commun, 2024, 15 6431

[14]

Liu Y, Tian G, Du Y, Shi P, Li N, Li Y, Qin Z, Jiao T, He X. Highly stretchable, low-hysteresis, and adhesive TA@MXene-composited organohydrogels for durable wearable sensors. Adv Funct Mater, 2024, 34 2315813

[15]

Yao X, Zhang S, Wei N, Qian L, Coseri S. Cellulose-based conductive hydrogels for emerging intelligent sensors. Adv Fiber Mater, 2024, 6: 1256-1305

[16]

Zhao Y, Zhang X, Hao Y, Zhao Y, Ding P, Zhai W, Dai K, Zheng G, Liu C, Shen C. Multifunctional PVA/PNIPAM conductive hydrogel sensors enabled human-machine interaction intelligent rehabilitation training. Adv Compos Hybrid Mater, 2024, 7 245

[17]

Li L, Wang X, You X, Rao P, Liu X, Zhang D, Zhang W, Wang W, Xing L, Li J, Zhang H. Super stretchable gelatin/poly (ionic liquid) hydrogel enabled by weak hydrogen bonds and microphase separation towards multifunctional and self-powered sensors. Nano Energy, 2025, 138 110875

[18]

Wang X-Q, Chan KH, Lu W, Ding T, Ng SWL, Cheng Y, Li T, Hong M, Tee BC, Ho GW. Macromolecule conformational shaping for extreme mechanical programming of polymorphic hydrogel fibers. Nat Commun, 2022, 13 3369

[19]

Wang Y, Zeng S, Shi S, Jiang Y, Du Z, Wang B, Li X. Hybrid assembly of conducting nanofiber network for ultra-stretchable and highly sensitive conductive hydrogels. J Mater Sci Technol, 2024, 169: 1-10

[20]

Li H, Luo R, Hu J, Yang K, Du B, Zhou S, Zhou X. Self-assembled gel-assisted preparation of high-performance hydrophobic PDMS@MWCNTs/PEDOT:PSS composite aerogels for wearable piezoresistive sensors. J Mater Sci Technol, 2024, 182: 22-32

[21]

Zhao K, Zhao Y, Xu J, Qian R, Yu Z, Ye C. Stretchable, adhesive and self-healing conductive hydrogels based on PEDOT:PSS-stabilized liquid metals for human motion detection. Chem Eng J, 2024, 494 152971

[22]

Lu P, Liao X, Guo X, Cai C, Liu Y, Chi M, Du G, Wei Z, Meng X, Nie S. Gel-based triboelectric nanogenerators for flexible sensing: principles, properties, and applications. Nano-Micro Lett, 2024, 16: 206

[23]

Liu J, Zhao W, Ma Z, Zhao H, Ren L. Self-powered flexible electronic skin tactile sensor with 3D force detection. Mater Today, 2024, 81: 84-94

[24]

Serairi L, Santillo C, Basset P, Lavorgna M, Pace G. Boosting contact electrification by amorphous polyvinyl alcohol endowing improved contact adhesion and electrochemical capacitance. Adv Mater, 2024, 36: 2403366

[25]

Ding Y, Guo H, Ouyang M, Meng G, Chen F, Kuang T. Humidity-resistant wearable triboelectric nanogenerator utilizing a bound-water-rich zwitterionic hydrogel with microphase-separated domains. Adv Funct Mater, 2025, 35: 2421164

[26]

Duan J, Yue G, Li H, Liu T, Wang P, Yu W, Shang P, Meng C, Guo S. Self-powered noncontact triboelectric nanogenerators with microstructured square-loop surface and dielectric electron-blocking layer for far-distance motion perception and trajectory tracking. Nano Energy, 2024, 128 109860

[27]

Yan D, Ye J, Zhou Y, Lei X, Deng B, Xu W. Research progress of fabrics with different geometric structures for triboelectric nanogenerators in flexible and wearable electronics. Adv Fiber Mater, 2023, 5: 1852-1878

[28]

Zhang Y, Ruan K, Gu J. Flexible sandwich-structured electromagnetic interference shielding nanocomposite films with excellent thermal conductivities. Small, 2021, 17: 2101951

[29]

Peng F, Zhu W, Fang Y, Fu B, Chen H, Ji H, Ma X, Hang C, Li M. Ultralight and highly conductive silver nanowire aerogels for high-performance electromagnetic interference shielding. ACS Appl Mater Interfaces, 2023, 15: 4284-4293

[30]

Wang P, Wang G, Sun G, Bao C, Li Y, Meng C, Yao Z. A flexible-integrated multimodal hydrogel-based sensing patch. Nano-Micro Lett, 2025, 17: 156

[31]

Zhang C, Wu B, Zhou Y, Zhou F, Liu W, Wang Z. Mussel-inspired hydrogels: from design principles to promising applications. Chem Soc Rev, 2020, 49: 3605-3637

[32]

Li X, Yuan L, Liu R, He H, Hao J, Lu Y, Wang Y, Liang G, Yuan G, Guo Z. Engineering textile electrode and bacterial cellulose nanofiber reinforced hydrogel electrolyte to enable high-performance flexible all-solid-state supercapacitors. Adv Energy Mater, 2021, 11: 2003010

[33]

Guo J, Zhang T, Hao X, Liu S, Zou Y, Li J, Wu W, Chen L, Liu X. Aramid nanofiber/MXene-reinforced polyelectrolyte hydrogels for absorption-dominated electromagnetic interference shielding and wearable sensing. Nano-Micro Lett, 2025, 17: 271

[34]

Hu L, Chee PL, Sugiarto S, Yu Y, Shi C, Yan R, Yao Z, Shi X, Zhi J, Kai D, Yu H-D, Huang W. Hydrogel-based flexible electronics. Adv Mater, 2023, 35: 2205326

[35]

Wang Y, Liu H, Xie H, Zhou S. An autofluorescent hydrogel with water-dependent emission for dehydration-visualizable smart wearable electronics. Adv Funct Mater, 2023, 33: 2213545

[36]

Wang Y, Cheng Y, Cai L, Chen H, Zhao Y. Phase separation derived anisotropic adhesive structural color hydrogel films for flexible electronics. Adv Funct Mater, 2024, 34: 2407848

[37]

Wang W, Zhou H, Xu Z, Li Z, Zhang L, Wan P. Flexible conformally bioadhesive MXene hydrogel electronics for machine learning-facilitated human-interactive sensing. Adv Mater, 2024, 36: 2401035

[38]

Cheng M, Ying M, Zhao R, Ji L, Li H, Liu X, Zhang J, Li Y, Dong X, Zhang X. Transparent and flexible electromagnetic interference shielding materials by constructing sandwich AgNW@MXene/wood composites. ACS Nano, 2022, 16: 16996-17007

[39]

Chen W, Liu L-X, Zhang H-B, Yu Z-Z. Kirigami-inspired highly stretchable, conductive, and hierarchical Ti3C2Tx MXene films for efficient electromagnetic interference shielding and pressure sensing. ACS Nano, 2021, 15: 7668-7681

[40]

Liu K, Liu W, Li W, Duan Y, Zhou K, Zhang S, Ni S, Xu T, Du H, Si C. Strong and highly conductive cellulose nanofibril/silver nanowires nanopaper for high performance electromagnetic interference shielding. Adv Compos Hybrid Mater, 2022, 5: 1078-1089

[41]

Zhang N, Wang Z, Song R, Wang Q, Chen H, Zhang B, Lv H, Wu Z, He D. Flexible and transparent graphene/silver-nanowires composite film for high electromagnetic interference shielding effectiveness. Sci Bull, 2019, 64: 540-546

[42]

Yang R, Gui X, Yao L, Hu Q, Yang L, Zhang H, Yao Y, Mei H, Tang Z. Ultrathin, lightweight, and flexible CNT buckypaper enhanced using MXenes for electromagnetic interference shielding. Nano-Micro Lett, 2021, 13 66

[43]

Shi Y-Y, Liao S-Y, Wang Q-F, Xu X-Y, Wang X-Y, Gu X-Y, Hu Y-G, Zhu P-L, Sun R, Wan Y-J. Enhancing the interaction of carbon nanotubes by Metal–organic decomposition with improved mechanical strength and ultra-broadband EMI shielding performance. Nano-Micro Lett, 2024, 16 134

[44]

Shin B, Mondal S, Lee M, Kim S, Huh Y-I, Nah C. Flexible thermoplastic polyurethane-carbon nanotube composites for electromagnetic interference shielding and thermal management. Chem Eng J, 2021, 418 129282

[45]

Wang X, Hu X, Liu Z, Zhu C, Shen R, Quan B, Yan X, Wang W, Lu X, Qu J. Interpenetrating double-network ANF/MXene-K+ aerogels enable integrated electromagnetic interference shielding, infrared camouflage, and Joule heating in adaptive multifunctional systems. Nano Res, 2025, 18 94907702

[46]

Hu X, Ai B, Quan B, Shi Z, Liu Z, Sheng M, Ding Y, Yan H, Xiao Y, Lu G, Liu S, Wu H, Huang X, Yan X, Lu X, Qu J. Synergistically networked 1D/2D/3D phase change composites with ultra-fast contactless thermal energy conversion and enhanced electromagnetic interference shielding performance. Chemical engineering for nanomaterials. Chem Eng J, 2025, 504 158915

[47]

Ji Q, Sheng X, Li X, Liu S, Chen Q, Guo P, Yang Y, Huang Y, Zhang G, Lu X, Qu J. Camel skin-fat structure inspired MXene@PVA/PCC aerogel composite for efficient medium and low temperature infrared stealth. Chem Eng J, 2023, 476 146671

[48]

Zhang HY, Li JY, Pan Y, Liu YF, Mahmood N, Jian X. Flexible carbon fiber-based composites for electromagnetic interference shielding. Rare Met, 2022, 41: 3612-3629

[49]

Nan Z, Wei W, Lin Z, Chang J, Hao Y. Flexible nanocomposite conductors for electromagnetic interference shielding. Nano-Micro Lett, 2023, 15 172

[50]

Kausar A, Ahmad I, Zhao T, Aldaghri O, Ibnaouf KH, Eisa MH, Lam TD. Graphene nanocomposites for electromagnetic interference shielding—trends and advancements. J Compos Sci, 2023, 7 384

[51]

Liu L-X, Chen W, Zhang H-B, Ye L, Wang Z, Zhang Y, Min P, Yu Z-Z. Super-tough and environmentally stable aramid. Nanofiber@MXene coaxial fibers with outstanding electromagnetic interference shielding efficiency. Nano-Micro Lett, 2022, 14 111

[52]

Zhang Y, Ruan K, Gu J. Flexible sandwich-structured electromagnetic interference shielding nanocomposite films with excellent thermal conductivities. Small, 2021, 17 2101951

[53]

Li Y, Wang Y, Huang Y. A review on MXene/nanocellulose composites: toward wearable multifunctional electromagnetic interference shielding application. Small, 2024, 21 2410283

[54]

Miao Z, Chen X, Zhou H, Liu P, Fu S, Yang J, Gao Y, Ren Y, Rong D. Interfacing MXene flakes on a magnetic fiber network as a stretchable, flexible, electromagnetic shielding fabric. Nanomaterials, 2021, 12 20

[55]

Zhu L, Zhang W, Luan S, Wei J, Yang Y, Miao J. Nanomaterials for smart wearable fibers and textiles: a critical review. iScience, 2025, 28 113126

[56]

Zhu S, Peng S, Qiang Z, Ye C, Zhu M. Cryogenic-environment resistant, highly elastic hybrid carbon foams for pressure sensing and electromagnetic interference shielding. Carbon, 2022, 193: 258-271

[57]

Wang X, Smith P, Qiang Z, Guan Q, You Z, Ye C, Zhu M. Fire-retardant, self-extinguishing multiblock poly(esterimide)s/graphene composites with segregated structure for electromagnetic interference shielding. Compos Part A Appl Sci Manuf, 2022, 163 107262

Funding

Higher Education Institution Science and Technology Research Project of Hebei Province(JZX2024024)

RIGHTS & PERMISSIONS

Donghua University, Shanghai, China

PDF

2

Accesses

0

Citation

Detail

Sections
Recommended

/