Dynamically Self-adaptive Metafabrics with Phase-Change Material-Enhanced Radiative Cooling for Thermo-hygrometric Regulation

Shengnan Ouyang , Qingtao Liu , Qiaoling Xue , Sheng Li , Jiale Zhang , Jinfeng Wang , Jinming Zhang , Jun Zhang , Xungai Wang

Advanced Fiber Materials ›› : 1 -17.

PDF
Advanced Fiber Materials ›› :1 -17. DOI: 10.1007/s42765-026-00702-5
Research Article
research-article
Dynamically Self-adaptive Metafabrics with Phase-Change Material-Enhanced Radiative Cooling for Thermo-hygrometric Regulation
Author information +
History +
PDF

Abstract

Reducing energy consumption plays a crucial role in promoting global sustainable development. However, achieving multifunctional collaborative thermal management for both efficient cooling and adaptive temperature regulation remains challenging. Herein, we report a phase-change material-enhanced passive radiative cooling (PCM–PRC) metafabric that integrates radiative cooling, evaporative cooling, and phase-change thermoregulation in a single system. The PCM–PRC exhibits excellent spectral selectivity (97% sunlight reflectivity, 94% selective infrared emissivity), along with high air and moisture permeability. Cooling experiments revealed that under mid-day sunlight (72.5 mW·cm−2 solar intensity) on a sunny day, the PCM–PRC metafabric achieved a 14.4 °C average temperature reduction, significantly outperforming conventional radiative fabrics. Its hierarchical wettability gradient enabled a high water–vapor transmission rate of 0.35 g·cm−2·day−1, thus triggering rapid sweat evaporation and efficient evaporation cooling. Furthermore, the incorporation of phase-change materials enables PCM–PRC with excellent adaptive thermoregulation performance under extreme temperature conditions (60 °C and 7 °C), combined with superior wearing comfort, air permeability, and long-term stability. These results provide a novel strategy for designing smart thermal management textiles with potential applications in adaptive thermal regulation, thermal and humidity comfort management and sustainable energy conservation.

Graphical abstract

Keywords

Passive radiative cooling / Phase-change material / Adaptive thermal management / Evaporative cooling / Metafabric

Cite this article

Download citation ▾
Shengnan Ouyang, Qingtao Liu, Qiaoling Xue, Sheng Li, Jiale Zhang, Jinfeng Wang, Jinming Zhang, Jun Zhang, Xungai Wang. Dynamically Self-adaptive Metafabrics with Phase-Change Material-Enhanced Radiative Cooling for Thermo-hygrometric Regulation. Advanced Fiber Materials 1-17 DOI:10.1007/s42765-026-00702-5

登录浏览全文

4963

注册一个新账户 忘记密码

References

[1]

Sherwood SC. Adapting to the challenges of warming. Science. 2020, 370: 782-783.

[2]

Wang ZC, Kim SK, Hu R. Self-switchable radiative cooling. Matter. 2022, 5: 780-782.

[3]

Lin M, Suter C, Diethelm S, Jan VH, Haussener S. Integrated solar-driven high-temperature electrolysis operating with concentrated irradiation. Joule. 2022, 6: 2102-2121.

[4]

Zhu B, Li W, Zhang Q, Li D, Liu X, Wang Y, Xu N, Wu Z, Li J, Li X, Catrysse PB, Xu W, Fan S, Zhu J. Subambient daytime radiative cooling textile based on nanoprocessed silk. Nat Nanotechnol. 2021, 16: 1342-1348.

[5]

Mazzone A, Fulkaxò Cruz DK, Tumwebaze S, Ushigua M, Trotter PA, Carvajal AE, Schaeffer R, Khosla R. Indigenous cosmologies of energy for a sustainable energy future. Nat Energy. 2023, 8: 19-29.

[6]

Li D, Liu X, Li W, Lin ZH, Zhu B, Li ZZ, Li JL, Li B, Fan SH, Xie JW, Zhu J. Scalable and hierarchically designed polymer film as a selective thermal emitter for high-performance all-day radiative cooling. Nat Nanotechnol. 2021, 16: 153-158.

[7]

Liu R, Wang SC, Zhou ZG, Zhang KY, Wang GY, Chen CY, Long Y. Materials in radiative cooling technologies. Adv Mater. 2025, 37. 2401577

[8]

Zhang XS, Yang WF, Shao ZW, Li YG, Su Y, Zhang QH, Hou CY, Wang HZ. A moisture-wicking passive radiative cooling hierarchical metafabric. ACS Nano. 2022, 16: 2188-2197.

[9]

Li JL, Wang XY, Liang D, Xu N, Zhu B, Li W, Yao PC, Jiang Y, Min XZ, Huang ZZ, Zhu SN, Fan SH, Zhu J. A tandem radiative/evaporative cooler for weather-insensitive and high-performance daytime passive cooling. Sci Adv. 2022, 8. eabq0411

[10]

Wu XE, Wang YD, Liang XP, Zhang Y, Bi P, Zhang MC, Li S, Liang HR, Wang S, Wang HM, Lu HJ, Zhang YY. Durable radiative cooling multilayer silk textile with excellent comprehensive performance. Adv Funct Mater. 2024, 34. 2313539

[11]

Ge Q, Chu JW, Cao WQ, Yi FL, Ran Z, Jin Z, Mao BY, Li ZL, Novoselov KS. Graphene-based textiles for thermal management and flame retardancy. Adv Funct Mater. 2022, 32. 2205934

[12]

He CY, Zhao P, Zhang H, Chen K, Liu BH, Lu ZW, Li Y, La PQ, Liu G, Gao XH. Efficient warming textile enhanced by a high-entropy spectrally selective nanofilm with high solar absorption. Adv Sci. 2023, 10. 2204817

[13]

Zeng SN, Pian SJ, Su MY, Wang ZN, Wu MQ, Liu XH, Chen MY, Xiang YZ, Wu JW, Zhang MN, Cen QQ, Tang YW, Zhou XH, Huang ZH, Wang R, Tunuhe A, Sun XY, Xia ZG, Tian MW, Chen M. Hierarchical-morphology metafabric for scalable passive daytime radiative cooling. Science. 2021, 373: 692-696.

[14]

An YA, Fu Y, Dai JG, Yin XB, Lei DY. Switchable radiative cooling technologies for smart thermal management. Cell Rep Phys Sci. 2022, 3. 101098

[15]

Cai CY, Wei ZC, Ding CX, Sun BJ, Chen WB, Gerhard C, Nimerovsky E, Fu Y, Zhang K. Dynamically tunable all-weather daytime cellulose aerogel radiative supercooler for energy-saving building. Nano Lett. 2022, 22: 4106-4114.

[16]

Dong JC, Peng YD, Nie XL, Li L, Zhang C, Lai FL, He GJ, Ma PM, Wei QF, Huang YP, Liu TX. Hierarchically designed super-elastic metafabric for thermal-wet comfortable and antibacterial epidermal electrode. Adv Funct Mater. 2022, 32. 2209762

[17]

Miao DY, Cheng NB, Wang XF, Yu JY, Ding B. Integration of Janus wettability and heat conduction in hierarchically designed textiles for all-day personal radiative cooling. Nano Lett. 2022, 22: 680-687.

[18]

Peng YC, Cui Y. Advanced textiles for personal thermal management and energy. Joule. 2020, 4: 724-742.

[19]

Miao DY, Wang XF, Yu JY, Ding B. Nanoengineered textiles for outdoor personal cooling and drying. Adv Funct Mater. 2022, 32. 2209029

[20]

Wang XF, Huang Z, Miao DY, Zhao J, Yu JY, Ding B. Biomimetic fibrous murray membranes with ultrafast water transport and evaporation for smart moisture-wicking fabrics. ACS Nano. 2018, 13: 1060-1070.

[21]

Hou LL, Wang N, Man XK, Cui ZM, Wu J, Liu JC, Li S, Li DM, Jiang L, Zhao Y. Interpenetrating Janus membrane for high rectification ratio liquid unidirectional penetration. ACS Nano. 2019, 13: 4124-4132.

[22]

Tang KPM, Chau KH, Kan CW, Fan JT. Assessing the accumulated stickiness magnitude from fabric-skin friction: effect of wetness level of various fabrics. R Soc Open Sci. 2018, 5. 180860

[23]

Fan CH, Zhang YX, Long ZW, Mensah A, Wang QQ, Lv PF, Wei QF. Dynamically tunable subambient daytime radiative cooling metafabric with Janus wettability. Adv Funct Mater. 2023, 33. 2300794

[24]

Shan XM, Liu L, Wu YS, Yuan DS, Wang J, Zhang CJ, Wang J. Aerogel-functionalized thermoplastic polyurethane as waterproof, breathable freestanding films and coatings for passive daytime radiative cooling. Adv Sci. 2022, 9. e2201190

[25]

Hu RJ, Wang N, Hou LL, Liu JC, Cui ZM, Zhang CH, Zhao Y. Bilayer nanoporous polyethylene membrane with anisotropic wettability for rapid water transportation/evaporation and radiative cooling. ACS Appl Mater Interfaces. 2022, 14: 9833-9843.

[26]

Feng MX, Cai HR, Feng SJ, Liu YM, Li ZH, He X, Liang S, Bu XH, Huang J, Zhou YM. Asymmetric gradient porous fabric with dynamically tunable thermal management and electromagnetic interference shielding via delayed phase separation. Adv Funct Mater. 2025, 35. 2422487

[27]

Wei YF, Zhang LN, Bernasconi F, Wu TT, Li YG, Zhang QH, Li KR, Malfait WJ, Hou CY, Zhao SY, Wang HZ. Temperature‐responsive resonator metafabrics for self‐adaptive thermoregulation. Adv Funct Mater. 2025, 35. 2422485

[28]

Pian SJ, Wang ZN, Lu CT, Wu PX, Chen QK, Liu X, Ma YG. Scalable colored Janus fabric scheme for dynamic thermal management. iScience. 2024, 27. 110948

[29]

Li XZ, Liao GD, Cai WW, Yang J, Jiang RW, Wan JL, Zhao HX, Cui JX. Polyurethane based smart composite fabric for personal thermal management in multi-mode. Small. 2024, 20. 2403334

[30]

Chen W, Wei XX, Liu W, Xu FJ. Dual-functional thermal management textiles for dynamic temperature regulation based on ultra-stretchable spiral conductive composite yarn with 500%-strain thermal stability and durability. Mater Horiz. 2024, 11: 792-802.

[31]

Jing YG, Zhao ZC, Cao XL, Sun QR, Yuan YP, Li TX. Ultraflexible, cost-effective and scalable polymer-based phase change composites via chemical cross-linking for wearable thermal management. Nat Commun. 2023, 14. 8060

[32]

Liu HQ, Zhou F, Shi XY, Sun KY, Kou Y, Das P, Li YG, Zhang XY, Mateti S, Chen Y, Wu ZS, Shi Q. A thermoregulatory flexible phase change nonwoven for all-season high-efficiency wearable thermal management. Nano-Micro Lett. 2023, 15. 29

[33]

Liu HQ, Zhang XY, Zhang SH, Kou Y, Fu HC, Zhou F, Wu ZS, Shi Q. Intrinsically flexible phase change fibers for intelligent thermal regulation. Angew Chem Int Ed. 2024, 136. e202408857

[34]

Wu YH, Chen MS, Zhao GZ, Qi DB, Zhang XH, Li YR, Huang YB, Yang WT. Recyclable solid-solid phase change materials with superior latent heat via reversible anhydride‐alcohol crosslinking for efficient thermal storage. Adv Mater. 2024, 36. 2311717

[35]

Yang M, Zhong HM, Li T, Wu BY, Wang ZK, Sun DZ. Phase change material enhanced radiative cooler for temperature-adaptive thermal regulation. ACS Nano. 2023, 17: 1693-1700.

[36]

Tang K, Dong K, Li JC, Gordon MP, Reichertz FG, Kim H, Rho Y, Wang QJ, Lin CY, Grigoropoulos CP, Javey A, Urban JJ, Yao J, Levinson R, Wu JQ. Temperature-adaptive radiative coating for all-season household thermal regulation. Science. 2021, 374: 1504-1509.

[37]

Zhou X, Chen WX, Zhao ZX, Peng SQ, Wu LX, Weng ZX. Broad-spectrum bionic polydisperse radiative cooling fiber membrane integrating high phase change and evaporation efficiency. Adv Funct Mater. 2025, 35e10443

[38]

Wang T, Wu Y, Shi L, Hu XH, Chen M, Wu LM. A structural polymer for highly efficient all-day passive radiative cooling. Nat Commun. 2021, 12. 365

[39]

Rockwood DN, Preda RC, Yücel T, Wang XQ, Lovett ML, Kaplan DL. Materials fabrication from Bombyx mori silk fibroin. Nat Protoc. 2011, 6: 1612-1631.

[40]

Zhou SJ, Zhang CH, Fu Z, Zhu QM, Zhou ZZX, Gong JY, Zhu N, Wang XF, Wei XJ, Xia LJ, Xu WL. Color construction of multi-colored carbon fibers using glucose. Nat Commun. 2024, 15. 1979

Funding

Innovative Research Group Project of the National Natural Science Foundation of China(52203124)

RIGHTS & PERMISSIONS

Donghua University, Shanghai, China

PDF

0

Accesses

0

Citation

Detail

Sections
Recommended

/