Biomimetic Gradient Fibrous Aerogel Pressure Sensor Featuring Ultrawide Sensitive Range and Extraordinary Pressure Resolution for Machine Learning Enabled Posture Recognition

Gaoen Jia , Xiaoyan Yue , Lingmeihui Duan , Rui Yin , Caofeng Pan , Hu Liu , Chuntai Liu , Changyu Shen

Advanced Fiber Materials ›› 2025, Vol. 7 ›› Issue (5) : 1632 -1647.

PDF
Advanced Fiber Materials ›› 2025, Vol. 7 ›› Issue (5) : 1632 -1647. DOI: 10.1007/s42765-025-00576-z
Research Article
research-article

Biomimetic Gradient Fibrous Aerogel Pressure Sensor Featuring Ultrawide Sensitive Range and Extraordinary Pressure Resolution for Machine Learning Enabled Posture Recognition

Author information +
History +
PDF

Abstract

Achieving human skin-like sensitivity and wide-range pressure detection remains a significant challenge in the development of wearable pressure sensors. In this study, we engineered and fabricated a fibrous polyimide fiber (PIF)/carbon nanotube (CNT) composite aerogel with a gradient structure using a layer-by-layer freeze casting technique, aiming to overcome the limitations of traditional pressure sensors. Finite element analysis (FEA) reveals that this innovative gradient structure mimics the unique microstructure of human skin, enabling the sensor to detect a broad spectrum of pressure stimuli, ranging from subtle pressures as low as 10 Pa to intense pressures up to 1.58 MPa with exceptional sensitivity. Moreover, the sensor exhibits extraordinary pressure resolution across the entire pressure range, particularly at 1 MPa (0.001%). Additionally, the sensor demonstrates remarkable thermal stability, operating reliably across a wide temperature range from − 150 to 200 °C, making it suitable for extreme environments such as deep space exploration. When integrated with machine learning algorithms, the sensor shows great potential for real-time physiological monitoring, fitness tracking, and motion recognition. The proposed gradient fibrous pressure sensor, with its high sensitivity and resolution over a wide pressure range, paves the way for new opportunities in human–machine interaction.

Keywords

Fibrous aerogel / Gradient structure / Ultrawide sensitive range / Machine learning / Posture recognition

Cite this article

Download citation ▾
Gaoen Jia, Xiaoyan Yue, Lingmeihui Duan, Rui Yin, Caofeng Pan, Hu Liu, Chuntai Liu, Changyu Shen. Biomimetic Gradient Fibrous Aerogel Pressure Sensor Featuring Ultrawide Sensitive Range and Extraordinary Pressure Resolution for Machine Learning Enabled Posture Recognition. Advanced Fiber Materials, 2025, 7(5): 1632-1647 DOI:10.1007/s42765-025-00576-z

登录浏览全文

4963

注册一个新账户 忘记密码

References

[1]

YaoS, RenP, SongR, LiuY, HuangQ, DongJ, O'ConnorBT, ZhuY. Nanomaterial-enabled flexible and stretchable sensing systems: processing, integration, and applications. Adv Mater, 2020, 321902343

[2]

LiJ, LiN, ZhengY, LouD, JiangY, JiangJ, XuQ, YangJ, SunY, PanC, WangJ, PengZ, ZhengZ, LiuW. Interfacially locked metal aerogel inside porous polymer composite for sensitive and durable flexible piezoresistive sensors. Adv Sci, 2022, 92201912

[3]

WeiC, ChengR, NingC, WeiX, PengX, LvT, ShengF, DongK, WangZL. A self-powered body motion sensing network integrated with multiple triboelectric fabrics for biometric gait recognition and auxiliary rehabilitation training. Adv Funct Mater, 2023, 332303562

[4]

WangXM, TaoLQ, YuanM, WangZP, YuJ, XieD, LuoF, ChenX, WongC. Sea urchin-like microstructure pressure sensors with an ultra-broad range and high sensitivity. Nat Commun, 2021, 121776

[5]

GuH, HuoX, ChenJ, El-BahySME, El-BahyZME. An overview of cellulose aerogel: classification and applications. ES Food & Agrofor, 2022, 101

[6]

RusD, TolleyMT. Design, fabrication and control of soft robots. Nature, 2015, 521467

[7]

TuS, XiY, CuiX, XuZ, LiuZ, ZhuY. Skin-inspired interlocked microstructures with soft-hard synergistic effect for high-sensitivity and wide-linear-range pressure-sensing. Chem Eng J, 2024, 496154083

[8]

GaoY, YanC, HuangH, YangT, TianG, XiongD, ChenN, ChuX, ZhongS, DengW, FangY, YangW. Microchannel-confined MXene based flexible piezoresistive multifunctional micro-force sensor. Adv Funct Mater, 2020, 301909603

[9]

XiongZ, HuangJ, ChenJ, LiuZ, ZhuY, SuiG, LiuZ. Synergy of hierarchical structures and multiple conduction mechanisms for designing ultra-wide linear range pressure sensors. Chem Eng J, 2025, 503158359

[10]

WangJ, XiongZ, WuL, ChenJ, ZhuY. Highly sensitive and wide-range iontronic pressure sensors with a wheat awn-like hierarchical structure. J Colloid Interface Sci, 2024, 669190

[11]

GuoY, ZhongM, FangZ, WanP, YuG. A Wearable transient pressure sensor made with MXene nanosheets for sensitive broad-range human-machine interfacing. Nano Lett, 2019, 191143

[12]

LiL, ZhuG, WangJ, ChenJ, ZhaoG, ZhuY. A flexible and ultrasensitive interfacial iontronic multisensory sensor with an array of unique "cup-shaped" microcolumns for detecting pressure and temperature. Nano Energy, 2023, 105108012

[13]

GaoW, EmaminejadS, NyeinHYY, ChallaS, ChenK, PeckA, FahadHM, OtaH, ShirakiH, KiriyaD, LienD-H, BrooksGA, DavisRW, JaveyA. Fully integrated wearable sensor arrays for multiplexed in situ perspiration analysis. Nature, 2016, 529509

[14]

LouZ, ChenS, WangL, JiangK, ShenG. An ultra-sensitive and rapid response speed graphene pressure sensors for electronic skin and health monitoring. Nano Energy, 2016, 237

[15]

WangJ, CuiX, SongY, ChenJ, ZhuY. Flexible iontronic sensors with high-precision and high-sensitivity detection for pressure and temperature. Compos Commun, 2023, 39101544

[16]

PangC, LeeGY, KimTI, KimSM, KimHN, AhnSH, SuhKY. A flexible and highly sensitive strain-gauge sensor using reversible interlocking of nanofibres. Nat Mater, 2012, 11795

[17]

NieB, LiR, CaoJ, BrandtJD, PanT. Flexible transparent iontronic film for interfacial capacitive pressure sensing. Adv Mater, 2015, 276055

[18]

ZhangD, SunH, HuangM, SuM, MaY, ShiM, MiL, LiuC, LiuH. Construction of "island-bridge" microstructured conductive coating for enhanced impedance response of organohydrogel strain sensor. Chem Eng J, 2024, 496153752

[19]

WangQ, XuB, TanD, HuX, YangY, HuangJ, GaoY, LiuX. Nature-inspired scalable high-performance triboelectric nanogenerators for energy harvesting and sensing. Nano Energy, 2024, 121109217

[20]

SunH, FangX, FangZ, ZhaoL, TianB, VermaP, MaedaR, JiangZ. An ultrasensitive and stretchable strain sensor based on a microcrack structure for motion monitoring. Microsyst Nanoeng, 2022, 8111

[21]

WuY, LiuJ, LinS, HuangK, ChenE, HuangK, LeiM. New pressure matrix array sensor composed of flexible mechanical sensor elements. Eng Sci, 2022, 18105

[22]

LiuR, JiB, LeiM, HuF, ZhouB. Simultaneous optimization of sensitivity and linearity for flexible pressure sensor via coupling effect between microstructures and flat substrate component. ACS Appl Electron Mater, 2023, 56918

[23]

ShiJ, DaiY, ChengY, XieS, LiG, LiuY, WangJ, ZhangR, BaiN, CaiM, ZhangY, ZhanY, ZhangZ, YuC, GuoCF. Embedment of sensing elements for robust, highly sensitive, and cross-talk–free iontronic skins for robotics applications. Sci Adv, 2023, 9eadf8831

[24]

ParkK, YukH, YangM, ChoJ, LeeH, KimJ. A biomimetic elastomeric robot skin using electrical impedance and acoustic tomography for tactile sensing. Sci Robot, 2022, 7eabm7187

[25]

HuangZ, YuS, XuY, CaoZ, ZhangJ, GuoZ, WuT, LiaoQ, ZhengY, ChenZ, LiaoX. In-sensor tactile fusion and logic for accurate intention recognition. Adv Mater, 2024, 362407329

[26]

LiuL, YuS, XuY, ChenH, WangH, LinW, HuY, HuangZ, WeiC, LinY, GuoZ, WuT, ZhengJ, ChenZ, ZhengY, LiaoX. Dynamically Reversible Filament Networks Enabling Programmable In-Sensor Memory for High-Precision Neuromorphic Interactions. Adv Funct Mater, 2025.

[27]

ChortosA, LiuJ, BaoZ. Pursuing prosthetic electronic skin. Nat Mater, 2016, 15937

[28]

QiuZ, WanY, ZhouW, YangJ, YangJ, HuangJ, ZhangJ, LiuQ, HuangS, BaiN, WuZ, HongW, WangH, GuoCF. Ionic skin with biomimetic dielectric layer templated from Calathea zebrine leaf. Adv Funct Mater, 2018, 281802343

[29]

LiuW, LiuN, YueY, RaoJ, ChengF, SuJ, LiuZ, GaoY. Piezoresistive pressure sensor based on synergistical innerconnect polyvinyl alcohol nanowires/wrinkled graphene film. Small, 2018, 141704149

[30]

ShiL, LiZ, ChenM, QinY, JiangY, WuL. Quantum effect-based flexible and transparent pressure sensors with ultrahigh sensitivity and sensing density. Nat Commun, 2020, 113529

[31]

ZhangY, YangJ, HouX, LiG, WangL, BaiN, CaiM, ZhaoL, WangY, ZhangJ, ChenK, WuX, YangC, DaiY, ZhangZ, GuoCF. Highly stable flexible pressure sensors with a quasi-homogeneous composition and interlinked interfaces. Nat Commun, 2022, 131317

[32]

XuH, GaoL, WangY, CaoK, HuX, WangL, MuM, LiuM, ZhangH, WangW, LuY. Flexible waterproof piezoresistive pressure sensors with wide linear working range based on conductive fabrics. Nano-Micro Lett, 2020, 12159

[33]

MaC, XuD, HuangYC, WangP, HuangJ, ZhouJ, LiuW, LiST, HuangY, DuanX. Robust flexible pressure sensors made from conductive micropyramids for manipulation tasks. ACS Nano, 2020, 1412866

[34]

LuoN, HuangY, LiuJ, ChenSC, WongCP, ZhaoN. Hollow-structured graphene–silicone-composite-based piezoresistive sensors: decoupled property tuning and bending reliability. Adv Mater, 2017, 291702675

[35]

PyoS, LeeJ, BaeK, SimS, KimJ. Recent progress in flexible tactile sensors for human-interactive systems: from sensors to advanced applications. Adv Mater, 2021, 332005902

[36]

MannsfeldSCB, TeeBCK, StoltenbergRM, ChenCVHH, BarmanS, MuirBVO, SokolovAN, ReeseC, BaoZ. Highly sensitive flexible pressure sensors with microstructured rubber dielectric layers. Nat Mater, 2010, 9859

[37]

YuT, ZhangD, WuY, GuoS, LeiF, LiY, YangJ. Graphene foam pressure sensor based on fractal electrode with high sensitivity and wide linear range. Carbon, 2021, 182497

[38]

BoutryCM, NegreM, JordaM, VardoulisO, ChortosA, KhatibO, BaoZ. A hierarchically patterned, bioinspired e-skin able to detect the direction of applied pressure for robotics. Sci Robot, 2018, 3eaau6914

[39]

WangC, XiaK, WangH, LiangX, YinZ, ZhangY. Advanced carbon for flexible and wearable electronics. Adv Mater, 2019, 311801072

[40]

XuZ, WuD, ChenZ, WangZ, CaoC, ShaoX, ZhouG, ZhangS, WangL, SunD. A flexible pressure sensor with highly customizable sensitivity and linearity via positive design of microhierarchical structures with a hyperelastic model. Microsyst Nanoeng, 2023, 95

[41]

ZhangX, HuZ, SunQ, LiangX, GuP, HuangJ, ZuG. Bioinspired gradient stretchable aerogels for ultrabroad-range-response pressure-sensitive wearable electronics and high-efficient separators. Angew Chem Int Ed, 2023, 62e202213952

[42]

LinW, XuY, YuS, WangH, HuangZ, CaoZ, WeiC, ChenZ, ZhangZ, ZhaoZ, LiaoQ, ZhengY, LiaoX. Highly Programmable Haptic Decoding and Self-Adaptive Spatiotemporal Feedback Toward Embodied Intelligence. Adv Funct Mater, 2025.

[43]

MaZ, WeiA, MaJ, ShaoL, JiangH, DongD, JiZ, WangQ, KangS. Lightweight, compressible and electrically conductive polyurethane sponges coated with synergistic multiwalled carbon nanotubes and graphene for piezoresistive sensors. Nanoscale, 2018, 107116

[44]

BaiN, WangL, WangQ, DengJ, WangY, LuP, HuangJ, LiG, ZhangY, YangJ, XieK, ZhaoX, GuoCF. Graded intrafillable architecture-based iontronic pressure sensor with ultra-broad-range high sensitivity. Nat Commun, 2020, 11209

[45]

YangR, DuttaA, LiB, TiwariN, ZhangW, NiuZ, GaoY, ErdelyD, XinX, LiT, ChengH. Iontronic pressure sensor with high sensitivity over ultra-broad linear range enabled by laser-induced gradient micro-pyramids. Nat Commun, 2023, 142907

[46]

GaoC, DengW, PanF, FengX, LiY. Superhydrophobic electrospun PVDF membranes with silanization and fluorosilanization co-functionalized CNTs for improved direct contact membrane distillation. Eng Sci, 2020, 935

[47]

ZhengQ, LeeJH, ShenX, ChenX, KimJK. Graphene-based wearable piezoresistive physical sensors. Mater Today, 2020, 36158

[48]

SivasankarapillaiVS, SharmaTSK, HwaKY, WabaidurSM, AngaiahS, DhanusuramanR. MXene Based Sensing Materials: Current Status and Future Perspectives. ES Energy & Environment, 2022, 154

[49]

RenY, XieW, LiY, MaJ, LiJ, LiuY, ZouY, DengY. Noble metal nanoparticles decorated metal oxide semiconducting nanowire arrays interwoven into 3D mesoporous superstructures for low-temperature gas sensing. ACS Cent Sci, 2021, 71885

[50]

CaoK, WuM, BaiJ, WenZ, ZhangJ, WangT, PengM, LiuT, JiaZ, LiangZ, JiangL. Beyond skin pressure sensing: 3D printed laminated graphene pressure sensing material combines extremely low detection limits with wide detection range. Adv Funct Mater, 2022, 322202360

[51]

AbrairaVE, GintyDD. The sensory neurons of touch. Neuron, 2013, 79618

[52]

XiaoW, WuH, SuQ, YanJ, TangL, HuangX, LuL, GuW, SongP, GaoJ. MXene initiated in situ construction of superhydrophobic and electrically conductive nanofibrous composites for wearable multifunctional sensing. Chem Eng J, 2025, 508161074

[53]

LiJ, YinJ, WeeMGV, ChinnappanA, RamakrishnaS. A self-powered piezoelectric nanofibrous membrane as wearable tactile sensor for human body motion monitoring and recognition. Adv Fiber Mater, 2023, 51417

[54]

XiaoW, ChenY, PanG, YanJ, ZhangJ, GaoJ. Hydrophobic, hemostatic and durable nanofiber composites with a screw-like surface architecture for multifunctional sensing electronics. Adv Fiber Mater, 2023, 52040

[55]

YangW, LiuH, DuH, ZhangM, WangC, YinR, PanC, LiuC, ShenC. Robust and superelastic spider web-like polyimide fiber-based conductive composite aerogel for extreme temperature-tolerant linear pressure sensor. Sci China Mater, 2023, 662829

[56]

WangJ, ZhuY, WuZ, ZhangY, LinJ, ChenT, LiuH, WangF, SunL. Wearable multichannel pulse condition monitoring system based on flexible pressure sensor arrays. Microsyst Nanoeng, 2022, 816

[57]

SomeyaT, AmagaiM. Toward a new generation of smart skins. Nat Biotechnol, 2019, 37382

[58]

BushAW, GibsonRD, ThomasTR. The elastic contact of a rough surface. Wear, 1975, 3587

[59]

GaoHL, ZhuY-B, MaoLB, WangFC, LuoXS, LiuYY, LuY, PanZ, GeJ, ShenW, ZhengYR, XuL, WangLJ, XuWH, WuHA, YuSH. Super-elastic and fatigue resistant carbon material with lamellar multi-arch microstructure. Nat Commun, 2016, 712920

[60]

GuiX, WeiJ, WangK, CaoA, ZhuH, JiaY, ShuQ, WuD. Carbon nanotube sponges. Adv Mater, 2010, 22617

[61]

SuhrJ, VictorP, CiL, SreekalaS, ZhangX, NalamasuO, AjayanPM. Fatigue resistance of aligned carbon nanotube arrays under cyclic compression. Nat Nanotechnol, 2007, 2417

[62]

TeoN, JanaSC. Solvent effects on tuning pore structures in polyimide aerogels. Langmuir, 2018, 348581

[63]

MuC, SongY, HuangW, RanA, SunR, XieW, ZhangH. Flexible normal-tangential force sensor with opposite resistance responding for highly sensitive artificial skin. Adv Funct Mater, 2018, 281707503

[64]

XiaoF, JinS, ZhangW, ZhangY, ZhouH, HuangY. Wearable pressure sensor using porous natural polymer hydrogel elastomers with high sensitivity over a wide sensing range. Polymers, 2023, 152736

[65]

YueZ, YeX, LiuS, ZhuY, JiangH, WanZ, LinY, JiaC. Towards ultra-wide operation range and high sensitivity: graphene film based pressure sensors for fingertips. Biosens Bioelectron, 2019, 139111296

[66]

LiZ, ZhangB, LiK, ZhangT, YangX. A wide linearity range and high sensitivity flexible pressure sensor with hierarchical microstructures via laser marking. J Mater Chem C, 2020, 83088

[67]

GuanX, WangZ, ZhaoW, HuangH, WangS, ZhangQ, ZhongD, LinW, DingN, PengZ. Flexible piezoresistive sensors with wide-range pressure measurements based on a graded nest-like architecture. ACS Appl Mater Interfaces, 2020, 1226137

[68]

YangW, LiuS, WangZ, LiuH, PanC, LiuC, ShenC. Bioinspired composite fiber aerogel pressure sensor for machine-learning-assisted human activity and gesture recognition. Nano Energy, 2024, 127109799

[69]

GuanF, XieY, WuH, MengY, ShiY, GaoM, ZhangZ, ChenS, ChenY, WangH, PeiQ. Silver nanowire-bacterial cellulose composite fiber-based sensor for highly sensitive detection of pressure and proximity. ACS Nano, 2020, 1415428

[70]

ZhuoS, SongC, RongQ, ZhaoT, LiuM. Shape and stiffness memory ionogels with programmable pressure-resistance response. Nat Commun, 2022, 131743

[71]

ChenS, ZhuoB, GuoX. Large area one-step facile processing of microstructured elastomeric dielectric film for high sensitivity and durable sensing over wide pressure range. ACS Appl Mater Interfaces, 2016, 820364

[72]

HuangY, LiuB, ZhangW, QuG, JinS, LiX, NieZ, ZhouH. Highly sensitive active-powering pressure sensor enabled by integration of double-rough surface hydrogel and flexible batteries. NPJ Flex Electron, 2022, 692

Funding

National Natural Science Foundation of China(52373093)

Natural Science Foundation of Henan Province(242300421062)

Central Plains Youth Top notch Talent Program of Henan Province

111 project(D18023)

RIGHTS & PERMISSIONS

Donghua University, Shanghai, China

AI Summary AI Mindmap
PDF

387

Accesses

0

Citation

Detail

Sections
Recommended

AI思维导图

/