Recent Advances in Metal–Organic Frameworks Based on Electrospinning for Energy Storage

Shunyu Yao; Seeram Ramakrishna; Gang Chen

doi:10.1007/s42765-023-00287-3

Advanced Fiber Materials ›› 2023, Vol. 5 ›› Issue (5) : 1592 -1617. DOI: 10.1007/s42765-023-00287-3

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Recent Advances in Metal–Organic Frameworks Based on Electrospinning for Energy Storage

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¹MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, 150001, Harbin, People’s Republic of China

²Center for Nanotechnology and Sustainability, Department of Mechanical Engineering, National University of Singapore, 119260, Singapore, Singapore

^b seeram@nus.edu.sg

^c gchen@hit.edu.cn

Shunyu Yao

is a Ph.D. student at the Harbin Institute of Technology in Prof. Gang Chen’s group. She is also an exchange Ph.D. student at the National University of Singapore in 2021. Her research focuses on the targeted synthesis of transition metal and metal-organic framework compounds with surface interface regulation and their applications in energy conversion. Her research works have been reported in Nano-Energy, Applied Catalysis B: Environmental, Chemical Engineering Journal, ACS Sustainable Chemistry & Engineering, and Journal of Colloid and Interface Science, respectively. Cited time of the publications is over 1300 and H-factor is 17.

Seeram Ramakrishna

is a world-renowned poly-disciplinary scholar at the National University of Singapore. He is named among the World’s Most Influential Minds (Thomson Reuters) and Top 1% Highly Cited Researchers in material science as well as cross-field categories (Clarivate Analytics). His publications to date have an H-index of 177 and over 151,637 citations. He is an elected Fellow of the UK Royal Academy of Engineering (FREng), AAAS, ASM International, ASME, and AIMBE, USA.

Gang Chen

obtained his Ph.D. degree in Materials System from Toyohashi University of Technology in 1996. Then he was promoted to Professor in the Department of Materials Chemistry, Harbin Institute of Technology, in 1996. His main research interests are in the fields of energy conversion functional materials, including lithium-ion battery materials, nanomaterials, light-responding materials, mesoporous functional materials, and the corresponding theoretical simulations and calculations.

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Abstract

Metal–organic frameworks are linked by different central organic ligands and metal-ion coordination bonds to form periodic pore structures and rich pore volumes. Because of their structural advantages, metal–organic frameworks are considered to be one of the most promising candidates for new energy storage materials. To better utilize their advantages, metal–organic frameworks can be combined with electrospinning technology to effectively adjust the porosity and mechanical strength of composite materials. This paper summarizes the combination of the latest metal–organic frameworks and classical spinning technology, starting from the structural design of electrode materials, and applying them to supercapacitors, lithium-ion batteries, lithium–sulfur batteries, sodium-ion batteries, and potassium-ion batteries. Finally, the problems and challenges related to the preparation of metal–organic framework nanofibers are summarized, and future development trends are predicted.

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Shunyu Yao, Seeram Ramakrishna, Gang Chen. Recent Advances in Metal–Organic Frameworks Based on Electrospinning for Energy Storage. Advanced Fiber Materials, 2023, 5(5): 1592-1617 DOI:10.1007/s42765-023-00287-3