We report the numerical and experimental studies of the two-dimensional Brillouin gain spectrum (BGS) distribution deformation induced by the self-phase modulation in the Brillouin optical time domain reflectometry (BOTDR) with a 20.6 km sensing distance. The BGS distribution deformation is investigated by analyzing the evolution of the point spread function along the fiber in the two-dimensional model of the BOTDR. In the simulation and experimental results, the specific deformation degree of the BGS distribution induced by the self-phase modulation is related to the pump pulse profile, pump pulse peak power, BGS demodulation method, and detected scattered light component. By comprehensively analyzing the evolution of the point spread function induced by the self-phase modulation and using the image deconvolution, a typical BOTDR sensor with a 25 ns pump pulse reaches the 20 cm spatial resolution over the 20.6 km sensing fiber.
In the paper, an optical fiber sensor based on a seven-core fiber composite structure is presented, which enables dual-parameter sensing of bending and temperature. The proposed structure is fabricated by combining the strongly-coupled seven-core fibers (SC-SCFs) and a weakly-coupled seven-core fiber (WC-SCF). The SC-SCF acts as a beam coupler and enhances the Mach-Zehnder interference, while the WC-SCF serves as the enhanced section of another Mach-Zehnder interference. Therefore, the spectrum response of the fiber structure mentioned above exhibits a superposition effect of two Mach-Zehnder interferometers (MZIs). Among them, two dips corresponding to different MZIs are used to measure bending and temperature. The experimental results show the bending sensitivity and temperature sensitivity of the two MZIs are −4.238 nm/m−1, −2.263 nm/m−1, 0.047 nm/°C, and 0.064 nm/°C, respectively. It proves that our sensor is very sensitive to bending. Through the dual-wavelength matrix method, the bending and temperature can be measured simultaneously. With the benefit of the composite structure, low cost, and ease of fabrication, the proposed sensor can be used in harsh environments.
This study presented a surface-functionalized sensor probe using 3-aminopropyltriethoxysilane (APTES) self-assembled monolayers on a Kretschmann-configured plasmonic platform. The probe featured stacked nanocomposites of gold (via sputtering) and graphene quantum dots (GQD, via spin-coating) for highly sensitive and accurate uric acid (UA) detection within the physiological ranges. Characterization encompassed the field emission scanning electron microscopy for detailed imaging, energy-dispersive X-ray spectroscopy for elemental analysis, and Fourier transform infrared spectroscopy for molecular identification. Surface functionalization increased sensor sensitivity by 60.64%, achieving 0.0221 °/(mg/dL) for the gold-GQD probe and 0.035 5 °/(mg/dL) for the gold-APTES-GQD probe, with linear correlation coefficients of 0.8249 and 0.8509, respectively. The highest sensitivity was 0.070 6 °/(mg/dL), with a linear correlation coefficient of 0.993 and a low limit of detection of 0.2 mg/dL. Furthermore, binding affinity increased dramatically, with the Langmuir constants of 14.29 µM−1 for the gold-GQD probe and 0.000 1 µM−1 for the gold-APTES-GQD probe, representing a 142 900-fold increase. The probe demonstrated notable reproducibility and repeatability with relative standard deviations of 0.166% and 0.013%, respectively, and exceptional temporal stability of 99.66%. These findings represented a transformative leap in plasmonic UA sensors, characterized by enhanced precision, reliability, sensitivity, and increased surface binding capacity, synergistically fostering unprecedented practicality.
In producing high-performance optical biosensors, the selected coupling agent and its fixation mode play an essential role as one of the decisive conditions for antibody incubation. In this work, we designed optical fiber biosensors by electrochemical polymerization to enable low detection limit (LOD) immunoassay. Based on the optical fiber lossy mode resonance (OF-LMR) achieved by In2O3-SnO2-90/10 wt% (ITO), we have simultaneously implemented the electropolymerized dopamine (ePDA) film on the ITO-coated fiber via the electrochemical method, utilizing the excellent electrical conductivity of ITO. After that, the immunoglobulin G (IgG) antibody layer was immobilized on the entire sensing region with the assistance of the ePDA film. The results of immunoassay were analyzed by recording the shift of the LMR resonance wavelength to verify the sensor performance. The LOD was evaluated as the lowest concentration of human IgG detected by the OF-LMR sensor, which was confirmed to be 4.20 ng·mL−1. Furthermore, the sensor achieved selective detection for specific antigens and exhibited a good recovery capability in chicken serum samples. The developed scheme provides a feasible opportunity to enhance the intersection of electrochemistry and optics subjects and also offers a new promising solution to achieve the immunoassay.