Buckwheat core derived nitrogen- and oxygen-rich controlled porous carbon for high-performance supercapacitors

Jun-ke Ou , Hong-wei Zhang , Ying Lei , Kai-yang Li , Bo Li , Hai-xin Deng , Hao Wang , Liang Zou

Journal of Central South University ›› 2023, Vol. 30 ›› Issue (2) : 419 -433.

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Journal of Central South University ›› 2023, Vol. 30 ›› Issue (2) : 419 -433. DOI: 10.1007/s11771-023-5249-0
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Buckwheat core derived nitrogen- and oxygen-rich controlled porous carbon for high-performance supercapacitors

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Abstract

We propose a simple and effective one-step activation route to prepare a hierarchically porous carbon with buckwheat core acting for precursor. The as-obtained porous carbon (BCPC-3) shows high specific surface area (805.91 m2/g) and high pore volume (0.60 cm3/g). As a supercapacitor electrode material for three-electrode, porous carbon delivers an ultrahigh capacitance of 330 F/g (at 0.5 A/g) in 6 mol/L KOH. In particular, it displays a capacitance of 140 F/g even when the current density increases to 100 A/g. In addition, in the two-electrode system, a symmetric supercapacitor based on buckwheat core with a controlled carbon structure can provide an output of 6.1 W·h/kg in a 6 mol/L KOH electrolyte. Therefore, this research offers a straightforward and cost-effective pathway for the fabrication of superior supercapacitor electrode materials.

Keywords

buckwheat core / porous carbon / supercapacitor

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Jun-ke Ou, Hong-wei Zhang, Ying Lei, Kai-yang Li, Bo Li, Hai-xin Deng, Hao Wang, Liang Zou. Buckwheat core derived nitrogen- and oxygen-rich controlled porous carbon for high-performance supercapacitors. Journal of Central South University, 2023, 30(2): 419-433 DOI:10.1007/s11771-023-5249-0

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