Potential impacts of climate and anthropogenic-induced changes on DOM dynamics among the major Chinese rivers

Abstract

Dissolved organic matter (DOM) is closely linked to human activities in drainage basins and plays a crucial role in maintaining ecosystem functioning and reflecting environmental quality. However, the impacts of climate and anthropogenic-induced changes on DOM in riverine systems under increasingly warming conditions still need to be better understood, particularly at large regional scales. To address this knowledge gap, we analyzed a dataset containing 386 published measurements for nine major Chinese river systems, examining dissolved organic carbon (DOC) concentrations and optical properties of chromophoric DOM (CDOM) under diverse environmental conditions, including mean air temperature, precipitation, surface solar radiation, population density, and land use. Our findings indicate that riverine DOC concentrations are significantly higher in northern China (at 46.8%) than in the south. This disparity is primarily due to the high input of soil erosion-induced DOM from drying-affected lands (57.0%), farmland (49.1%), and forests in the north. The high temperate and strong hydrological conditions would lead to DOM degradation easily in the riverine system in the south of China. Our study highlights that various climatic and anthropogenic factors, such as agriculture, vegetation coverage, soil erosion, surface solar radiation, and precipitation, individually or in combination, can affect DOM dynamics in river systems. Therefore, considering alterations in DOM dynamics resulting from climate and environmental changes is crucial for carbon-neutral policies and sustainable river ecosystem assessments.

Keywords

River / Dissolved organic carbon / Land use / Climate and environmental change / Sustainable development

Declaration of Competing Interests

The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Acknowledgements

This research was funded by the National Natural Science Foundation of China (Grants No. 41925002, 42221001, 42230509) and received financial support from the Haihe Laboratory of Sustainable Chemical Transformations.

Supplementary materials

Supplementary material associated with this article can be found, in the online version, at doi:10.1016/j.geosus.2023.07.003.

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