Progress in graphdiyne-based membrane for gas separation and water puriﬁcation

Siyuan Li; Yasong Zhao; Dan Wang

doi:10.1016/j.chphma.2025.02.007

ChemPhysMater ›› 2025, Vol. 4 ›› Issue (3) :234 -250. DOI: 10.1016/j.chphma.2025.02.007

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research-article

Progress in graphdiyne-based membrane for gas separation and water puriﬁcation

Siyuan Li ^a
, Yasong Zhao ^a^,^*
, Dan Wang ^a^,^b^,^*

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Abstract

Membrane separation is an eﬃcient method with signiﬁcant applications across various ﬁelds. Graphdiyne (GDY), a novel carbon allotrope composed of sp and sp² hybridized carbon atoms, possesses unique physical and chemical properties that enable its application in catalysis, electronics, and sensing. Additionally, its two-dimensional planar structure and homogeneous pore distribution facilitate the adsorption and transport of various metal ions and gases, highlighting its potential in separation processes. This review summarizes the structure and properties of GDY, outlines its synthesis strategies, and describes its detailed applications in gas separation, heavy metal ion separation, organic separation, and desalination. Finally, the challenges associated with the separation of GDY-based materials are discussed.

Keywords

2D materials / Graphdiyne / Membrane / Separation

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Siyuan Li, Yasong Zhao, Dan Wang. Progress in graphdiyne-based membrane for gas separation and water puriﬁcation. ChemPhysMater, 2025, 4 (3) : 234-250 DOI:10.1016/j.chphma.2025.02.007

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Declaration of Competing Interest

The authors declare that they have no known competing ﬁnancial interests or personal relationships that could have appeared to inﬂuence the work reported in this paper.

CRediT authorship contribution statement

Siyuan Li: Writing – original draft, Investigation, Formal analysis. Yasong Zhao: Writing – review & editing, Formal analysis. Dan Wang: Writing – review & editing, Supervision, Funding acquisition, Conceptualization.

Acknowledgements

This study was ﬁnancially supported by the National Natural Science Foundation of China (Nos. 2022YFA1204502 and 52201284 ).

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