Energy & Environmental Materials >

2024 , Vol. 7 >Issue 1: 12515

DOI: https://doi.org/10.1002/eem2.12515

Hybrid 2D/3D Graphitic Carbon Nitride-Based High-Temperature Position-Sensitive Detector

  • Xuexia Chen ,
  • Dongwen Yang ,
  • Xun Yang ,
  • Qing Lou ,
  • Zhiyu Liu ,
  • Yancheng Chen ,
  • Chaofan Lv ,
  • Lin Dong ,
  • Chongxin Shan
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  • Henan Key Laboratory of Diamond Optoelectronic Materials and Devices, Key Laboratory of Material Physics, Ministry of Education, School of Physics and Microelectronics, Zhengzhou University, Zhengzhou 450052, China
louqing1986@zzu.edu.cn
ldong@zzu.edu.cn
cxshan@zzu.edu.cn

Received date: 17 Jun 2022

Revised date: 07 Aug 2022

Copyright

2022 2022 The Authors. Energy & Environmental Materials published by John Wiley & Sons Australia, Ltd on behalf of Zhengzhou University.
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Abstract

Ultraviolet position-sensitive detectors (PSDs) are expected to undergo harsh environments, such as high temperatures, for a wide variety of applications in military, civilian, and aerospace. However, no report on relevant PSDs operating at high temperatures can be found up to now. Herein, we design a new 2D/3D graphitic carbon nitride (g-C3N4)/gallium nitride (GaN) hybrid heterojunction to construct the ultraviolet high-temperature-resistant PSD. The g-C3N4/GaN PSD exhibits a high position sensitivity of 355 mV mm-1, a rise/fall response time of 1.7/2.3 ms, and a nonlinearity of 0.5% at room temperature. The ultralow formation energy of -0.917 eV atom-1 has been obtained via the thermodynamic phase stability calculations, which endows g-C3N4 with robust stability against heat. By merits of the strong built-in electric field of the 2D/3D hybrid heterojunction and robust thermo-stability of g-C3N4, the g-C3N4/GaN PSD delivers an excellent position sensitivity and angle detection nonlinearity of 315 mV mm-1 and 1.4%, respectively, with high repeatability at a high temperature up to 700 K, outperforming most of the other counterparts and even commercial silicon-based devices. This work unveils the high-temperature PSD, and pioneers a new path to constructing g-C3N4-based harsh-environment-tolerant optoelectronic devices.

Key words： graphitic carbon nitride; high-temperature stability; lateral photovoltaic effect; position-sensitive detectors; two-dimensional materials

Cite this article

Xuexia Chen , Dongwen Yang , Xun Yang , Qing Lou , Zhiyu Liu , Yancheng Chen , Chaofan Lv , Lin Dong , Chongxin Shan . Hybrid 2D/3D Graphitic Carbon Nitride-Based High-Temperature Position-Sensitive Detector[J]. Energy & Environmental Materials, 2024 , 7(1) : 12515 . DOI: 10.1002/eem2.12515

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