Metasurfaces are composed of periodic subwavelength nanostructures and exhibit optical properties that are not found in nature. They have been widely investigated for optical applications such as holograms, wavefront shaping, and structural color printing, however, electron-beam lithography is not suitable to produce large-area metasurfaces because of the high fabrication cost and low productivity. Although alternative optical technologies, such as holographic lithography and plasmonic lithography, can overcome these drawbacks, such methods are still constrained by the optical diffraction limit. To break through this fundamental problem, mechanical nanopatterning processes have been actively studied in many fields, with nanoimprint lithography (NIL) coming to the forefront. Since NIL replicates the nanopattern of the mold regardless of the diffraction limit, NIL can achieve sufficiently high productivity and patterning resolution, giving rise to an explosive development in the fabrication of metasurfaces. In this review, we focus on various NIL technologies for the manufacturing of metasurfaces. First, we briefly describe conventional NIL and then present various NIL methods for the scalable fabrication of metasurfaces. We also discuss recent applications of NIL in the realization of metasurfaces. Finally, we conclude with an outlook on each method and suggest perspectives for future research on the high-throughput fabrication of active metasurfaces.

Lens is a basic optical element that is widely used in daily life, such as in cameras, glasses, and microscopes. Conventional lenses are designed based on the classical refractive optics, which results in inevitable imaging aberrations, such as chromatic aberration, spherical aberration and coma. To solve these problems, conventional imaging systems impose multiple curved lenses with different thicknesses and materials to eliminate these aberrations. As a unique photonic technology, metasurfaces can accurately manipulate the wavefront of light to produce fascinating and peculiar optical phenomena, which has stimulated researchers’ extensive interests in the field of planar optics. Starting from the introduction of phase modulation methods, this review summarizes the design principles and characteristics of metalenses. Although the imaging quality of existing metalenses is not necessarily better than that of conventional lenses, the multi-dimensional and multi-degree-of-freedom control of metasurfaces provides metalenses with novel functions that are extremely challenging or impossible to achieve with conventional lenses.

Strong terahertz (THz) radiation provides a powerful tool to manipulate and control complex condensed matter systems. This review provides an overview of progress in the generation, detection, and applications of intense THz radiation. The tabletop intense THz sources based on Ti:sapphire laser are reviewed, including photoconductive antennas (PCAs), optical rectification sources, plasma-based THz sources, and some novel techniques for THz generations, such as topological insulators, spintronic materials, and metasurfaces. The coherent THz detection methods are summarized, and their limitations for intense THz detection are analyzed. Applications of intense THz radiation are introduced, including applications in spectroscopy detection, nonlinear effects, and switching of coherent magnons. The review is concluded with a short perspective on the generation and applications of intense THz radiation.

Manipulating circularly polarized (CP) electromagnetic (EM) waves at will is significantly important for a wide range of applications ranging from chiral-molecule manipulations to optical communication. However, conventional EM devices based on natural materials suffer from limited functionalities, bulky configurations, and low efficiencies. Recently, Pancharatnam–Berry (PB) phase metasurfaces have shown excellent capabilities in controlling CP waves in different frequency domains, thereby allowing for multi-functional PB meta-devices that integrate distinct functionalities into single and flat devices. Nevertheless, the PB phase has intrinsically opposite signs for two spins, resulting in locked and mirrored functionalities for right CP and left CP beams. Here we review the fundamentals and applications of spin-decoupled metasurfaces that release the spin-locked limitation of PB metasurfaces by combining the orientation-dependent PB phase and the dimension-dependent propagation phase. This provides a general and practical guideline toward realizing spin-decoupled functionalities with a single metasurface for orthogonal circular polarizations. Finally, we conclude this review with a short conclusion and personal outlook on the future directions of this rapidly growing research area, hoping to stimulate new research outputs that can be useful in future applications.

In this paper, we review the past and recent works on generating intense terahertz (THz) pulses from photoconductive antennas (PCAs). We will focus on two types of large-aperture photoconductive antenna (LAPCA) that can generate high-intensity THz pulses (a) those with large-aperture dipoles and (b) those with interdigitated electrodes. We will first describe the principles of THz generation from PCAs. The critical parameters for improving the peak intensity of THz radiation from LAPCAs are summarized. We will then describe the saturation and limitation process of LAPCAs along with the advantages and disadvantages of working with wide-bandgap semiconductor substrates. Then, we will explain the evolution of LAPCA with interdigitated electrodes, which allows one to reduce the photoconductive gap size, and thus obtain higher bias fields while applying lower voltages. We will also describe recent achievements in intense THz pulses generated by interdigitated LAPCAs based on wide-bandgap semiconductors driven by amplified lasers. Finally, we will discuss the future perspectives of THz pulse generation using LAPCAs.

With strong electron–phonon coupling, the self-trapped excitons are usually formed in materials, which leads to the local lattice distortion and localized excitons. The self-trapping strongly depends on the dimensionality of the materials. In the three-dimensional case, there is a potential barrier for self-trapping, whereas no such barrier is present for quasi-one-dimensional systems. Two-dimensional (2D) systems are marginal cases with a much lower potential barrier or nonexistent potential barrier for the self-trapping, leading to the easier formation of self-trapped states. Self-trapped excitons emission exhibits a broadband emission with a large Stokes shift below the bandgap. 2D perovskites are a class of layered structure material with unique optical properties and would find potential promising optoelectronic. In particular, self-trapped excitons are present in 2D perovskites and can significantly influence the optical and electrical properties of 2D perovskites due to the soft characteristic and strong electron–phonon interaction. Here, we summarized the luminescence characteristics, origins, and characterizations of self-trapped excitons in 2D perovskites and finally gave an introduction to their applications in optoelectronics.

Additive manufacturing (AM), which is also known as three-dimensional (3D) printing, uses computer-aided design to build objects layer by layer. Here, we focus on the recent progress in the development of techniques for 3D printing of glass, an important optoelectronic material, including fused deposition modeling, selective laser sintering/melting, stereolithography (SLA) and direct ink writing. We compare these 3D printing methods and analyze their benefits and problems for the manufacturing of functional glass objects. In addition, we discuss the technological principles of 3D glass printing and applications of 3D printed glass objects. This review is finalized by a summary of the current achievements and perspectives for the future development of the 3D glass printing technique.

Highly efficient generation and arbitrary manipulation of spin-polarized terahertz (THz) radiation will enable chiral lightwave driven quantum nonequilibrium state regulation, induce new electronic structures, consequently provide a powerful experimental tool for investigation of nonlinear THz optics and extreme THz science and applications. THz circular dichromic spectroscopy, ultrafast electron bunch manipulation, as well as THz imaging, sensing, and telecommunication, also need chiral THz waves. Here we review optical generation of circularly-polarized THz radiation but focus on recently emerged polarization tunable spintronic THz emission techniques, which possess many advantages of ultra-broadband, high efficiency, low cost, easy for integration and so on. We believe that chiral THz sources based on the combination of electron spin, ultrafast optical techniques and material structure engineering will accelerate the development of THz science and applications.

There are a variety of elementary and collective terahertz-frequency excitations in condensed matter whose magnetic field dependence contains significant insight into the states and dynamics of the electrons involved. Often, determining the frequency, temperature, and magnetic field dependence of the optical conductivity tensor, especially in high magnetic fields, can clarify the microscopic physics behind complex many-body behaviors of solids. While there are advanced terahertz spectroscopy techniques as well as high magnetic field generation techniques available, a combination of the two has only been realized relatively recently. Here, we review the current state of terahertz time-domain spectroscopy (THz-TDS) experiments in high magnetic fields. We start with an overview of time-domain terahertz detection schemes with a special focus on how they have been incorporated into optically accessible high-field magnets. Advantages and disadvantages of different types of magnets in performing THz-TDS experiments are also discussed. Finally, we highlight some of the new fascinating physical phenomena that have been revealed by THz-TDS in high magnetic fields.

Faster and better wound healing is a critical medical issue. Because the repair process of wounds is closely related to revascularization, accurate early assessment and postoperative monitoring are very important for establishing an optimal treatment plan. Herein, we present an extended depth-of-field photoacoustic microscopy system (E-DOF-PAM) that can achieve a constant spatial resolution and relatively uniform excitation efficiency over a long axial range. The superior performance of the system was verified by phantom and in vivo experiments. Furthermore, the system was applied to the imaging of normal and trauma sites of volunteers, and the experimental results accurately revealed the morphological differences between the normal and traumatized skin of the epidermis and dermis. These results demonstrated that the E-DOF-PAM is a powerful tool for observing and understanding the pathophysiology of cutaneous wound healing.

Materials, where charge carriers have a linear energy dispersion, usually exhibit a strong nonlinear optical response in the absence of disorder scattering. This nonlinear response is particularly interesting in the terahertz frequency region. We present a theoretical and numerical investigation of charge transport and nonlinear effects, such as the high harmonic generation in topological materials including Weyl semimetals (WSMs) and a-T₃ systems. The nonlinear optical conductivity is calculated both semi-classically using the velocity operator and quantum mechanically using the density matrix. We show that the nonlinear response is strongly dependent on temperature and topological parameters, such as the Weyl point (WP) separation b and Berry phase {\phi }_{\mathrm{B}}. A finite spectral gap opening can further modify the nonlinear effects. Under certain parameters, universal behaviors of both the linear and nonlinear response can be observed. Coupled with experimentally accessible critical field values of 1{\mathrm{0}}^4-1{\mathrm{0}}^{\mathrm{5}}\mathrm{V/m}, our results provide useful information on developing nonlinear optoelectronic devices based on topological materials.

Dielectric metasurfaces-based planar optical spatial differentiator and edge detection have recently been proposed to play an important role in the parallel and fast image processing technology. With the development of dielectric metasurfaces of different geometries and resonance mechanisms, diverse on-chip spatial differentiators have been proposed by tailoring the dispersion characteristics of subwavelength structures. This review focuses on the basic principles and characteristic parameters of dielectric metasurfaces as first- and second-order spatial differentiators realized via the Green’s function approach. The spatial bandwidth and polarization dependence are emphasized as key properties by comparing the optical transfer functions of metasurfaces for different incident wavevectors and polarizations. To present the operational capabilities of a two-dimensional spatial differentiator in image information acquisition, edge detection is described to illustrate the practicability of the device. As an application example, experimental demonstrations of edge detection for different biological cells and a flower mold are discussed, in which a spatial differentiator and objective lens or camera are integrated in three optical pathway configurations. The realization of spatial differentiators and edge detection with dielectric metasurfaces provides new opportunities for ultrafast information identification in biological imaging and machine vision.

Circadian rhythms are considered a masterstroke of natural selection, which gradually increase the adaptability of species to the Earth’s rotation. Importantly, the nervous system plays a key role in allowing organisms to maintain circadian rhythmicity. Circadian rhythms affect multiple aspects of cognitive functions (mainly via arousal), particularly those needed for effort-intensive cognitive tasks, which require considerable top-down executive control. These include inhibitory control, working memory, task switching, and psychomotor vigilance. This mini review highlights the recent advances in cognitive functioning in the optical and multimodal neuroimaging fields; it discusses the processing of brain cognitive functions during the circadian rhythm phase and the effects of the circadian rhythm on the cognitive component of the brain and the brain circuit supporting cognition.

Due to the rise of 5G, IoT, AI, and high-performance computing applications, datacenter traffic has grown at a compound annual growth rate of nearly 30%. Furthermore, nearly three-fourths of the datacenter traffic resides within datacenters. The conventional pluggable optics increases at a much slower rate than that of datacenter traffic. The gap between application requirements and the capability of conventional pluggable optics keeps increasing, a trend that is unsustainable. Copackaged optics (CPO) is a disruptive approach to increasing the interconnecting bandwidth density and energy efficiency by dramatically shortening the electrical link length through advanced packaging and co-optimization of electronics and photonics. CPO is widely regarded as a promising solution for future datacenter interconnections, and silicon platform is the most promising platform for large-scale integration. Leading international companies (e.g., Intel, Broadcom and IBM) have heavily investigated in CPO technology, an inter-disciplinary research field that involves photonic devices, integrated circuits design, packaging, photonic device modeling, electronic-photonic co-simulation, applications, and standardization. This review aims to provide the readers a comprehensive overview of the state-of-the-art progress of CPO in silicon platform, identify the key challenges, and point out the potential solutions, hoping to encourage collaboration between different research fields to accelerate the development of CPO technology.

In this paper, we presented single mode terahertz quantum cascade lasers (THz QCLs) with sampled lateral grating emitting approximately 3.4 THz. Due to strong mode selection, the implementation of sampled lateral grating on THz QCL ridges can result in stable single longitudinal mode emission with a side-mode suppression ratio larger than 20 dB. The measured peak power of the grating laser is improved by about 11.8% compared to the power of devices with uniform distributed feedback gratings. Furthermore, the far-field pattern of the presented device is uninfluenced by grating structures.

Inverted perovskite solar cells (PVSCs) have recently made exciting progress, showing high power conversion efficiencies (PCEs) of 25% in single-junction devices and 30.5% in silicon/perovskite tandem devices. The hole transporting material (HTM) in an inverted PVSC plays an important role in determining the device performance, since it not only extracts/transports holes but also affects the growth and crystallization of perovskite film. Currently, polymer and self-assembled monolayer (SAM) have been considered as two types of most promising HTM candidates for inverted PVSCs owing to their high PCEs, high stability and adaptability to large area devices. In this review, recent encouraging progress of high-performance polymer and SAM-based HTMs is systematically reviewed and summarized, including molecular design strategies and the correlation between molecular structure and device performance. We hope this review can inspire further innovative development of HTMs for wide applications in highly efficient and stable inverted PVSCs and the tandem devices.

The dynamic control of the metasurface opens up a vital technological approach for the development of multifunctional integrated optical devices. The magnetic field manipulation has the advantages of sub-nanosecond ultra-fast response, non-contact, and continuous adjustment. Thus, the magnetically controllable metasurface has attracted significant attention in recent years. This study introduces the basic principles of the Faraday and Kerr effect of magneto-optical (MO) materials. It classifies the typical MO materials according to their properties. It also summarizes the physical mechanism of different MO metasurfaces that combine the MO effect with plasmonic or dielectric resonance. Besides, their applications in the nonreciprocal device and MO sensing are demonstrated. The future perspectives and challenges of the research on MO metasurfaces are discussed.

Metal halide perovskites are a class of materials that are ideal for photodetectors and solar cells due to their excellent optoelectronic properties. Their low-cost and low temperature synthesis have made them attractive for extensive research aimed at revolutionizing the semiconductor industry. The rich chemistry of metal halide perovskites allows compositional engineering resulting in facile tuning of the desired optoelectronic properties. Moreover, using different experimental synthesis and deposition techniques such as solution processing, chemical vapor deposition and hot-injection methods, the dimensionality of the perovskites can be altered from 3D to 0D, each structure opening a new realm of applications due to their unique properties. Dimensionality engineering includes both morphological engineering–reducing the thickness of 3D perovskite into atomically thin films–and molecular engineering–incorporating long-chain organic cations into the perovskite mixture and changing the composition at the molecular level. The optoelectronic properties of the perovskite structure including its band gap, binding energy and carrier mobility depend on both its composition and dimensionality. The plethora of different photodetectors and solar cells that have been made with different compositions and dimensions of perovskite will be reviewed here. We will conclude our review by discussing the kinetics and dynamics of different dimensionalities, their inherent stability and toxicity issues, and how reaching similar performance to 3D in lower dimensionalities and their large-scale deployment can be achieved.

The broad emission and high photoluminescence quantum yield of self-trapped exciton (STE) radiative recombination emitters make them an ideal solution for single-substrate, white, solid-state lighting sources. Unlike impurities and defects in semiconductors, the formation of STEs requires a lattice distortion, along with strong electron–phonon coupling, in low electron-dimensional materials. The photoluminescence of inorganic copper(I) metal halides with low electron-dimensionality has been found to be the result of STEs. These materials were of significant interest because of their lead-free, all-inorganic structures, and high luminous efficiencies. In this paper, we summarize the luminescence characteristics of zero- and one-dimensional inorganic copper(I) metal halides with STEs to provide an overview of future research opportunities.